Non-destructive study of collision cascade damage in self-ion irradiated tungsten using HR-EBSD and ECCI

TL;DR

This study demonstrates the use of advanced SEM techniques, ECCI and HR-EBSD, for non-destructive, multi-scale analysis of irradiation-induced defects and strain fields in tungsten, revealing microstructural evolution with dose.

Contribution

It introduces a non-destructive SEM-based approach combining ECCI and HR-EBSD for detailed analysis of irradiation damage in tungsten, overcoming limitations of traditional TEM methods.

Findings

Damage microstructure evolves from nano-scale defects to string structures with dose.

Significant heterogeneity in lattice strains appears at 0.1 dpa and saturates at 0.32 dpa.

SEM techniques enable rapid, multi-scale, non-destructive characterization of irradiation damage.

Abstract

Understanding defect production and evolution under irradiation is a long-standing multi-scale problem. Conventionally, experimental examination of irradiation-induced defects (IIDs) has mainly relied on transmission electron microscopy (TEM), which offers high spatial resolution but requires destructive sample preparation. Furthermore, limited field of view and low strain sensitivity make multi-scale characterisation and quantitative strain measurements difficult. Here we explore the potential of using advanced techniques in the scanning electron microscope (SEM) to non-destructively probe irradiation damage at the surface of bulk materials. Electron channelling contrast imaging (ECCI) is used to image nano-scale irradiation-induced defects in 20 MeV self-ion irradiated tungsten, the main candidate material for fusion reactor armour. The results show an evolution of the damage microstructure from uniformly and randomly distributed nano-scale defects at 0.01 dpa (displacement per atom) to string structures extending over hundreds of nanometres at 1 dpa. Cross-correlation based high-resolution EBSD (HR-EBSD) is used to probe the lattice strain fields associated with IIDs. While there is little strain fluctuation at 0.01 dpa, significant heterogeneity in the lattice strains is observed at 0.1 dpa, increasing with dose until saturation at 0.32 dpa. The characteristic length scale of strain fluctuations is ~500 nm. Together, ECCI and HR-EBSD reveal a transition from a structure where defects are disordered to a structure with long-range order driven by elastic interactions between pre-existing defects and new cascade damage. This study demonstrates that SEM provides an attractive tool for rapid throughput, non-destructive, multi-scale and multi-aspect characterisation of irradiation damage.