Generalized Elastodynamic Model for Nanophotonics

TL;DR

This paper introduces a comprehensive elastodynamic model for nanophotonics that accurately describes light-matter interactions at the nanoscale, incorporating spatial dispersion and interface effects without additional boundary conditions.

Contribution

It develops a self-consistent classical theory using elastodynamics to model non-local effects in nanostructured materials, unifying interface treatment across different material types.

Findings

The model converges to local boundary conditions in the low dispersion limit.

It provides a natural boundary condition derivation without extra hypotheses.

The approach accurately describes solid-solid and solid-vacuum interfaces.

Abstract

A self-consistent theory for the classical description of the interaction of light and matter at the nano-scale is presented, which takes into account spatial dispersion. Up to now, the Maxwell equations in nanostructured materials with spatial dispersion have been solved by the introduction of the so-called Additional Boundary Conditions. In this paper, we derive an approach where non-local effects are studied in a precise and uniquely defined way, thus allowing the treatment of all solid-solid interfaces (metals, semiconductors or insulators), as well as solid-vacuum interfaces in the same framework. The theory is based on the derivation of a potential energy for an ensemble of electrons in a given potential, where the deformation of the ensemble is treated as in a solid, including both shear and compressional deformations, instead of a fluid described only by a bulk compressibility like in the hydrodynamical approach. The derived classical equation of motion for the ensemble describes the deformation vector and the corresponding polarization vector as an elastodynamic field, including viscous forces, from which a generalized non-local constitutive equation for the dielectric constant is derived. Boundary conditions are identical to that of elastodynamics and they emerge in a natural way, without any physical hypothesis outside the current description, as it is commonly required in other non-local approaches. This description does not require the discontinuity of any component of the electric, magnetic or polarization fields and, consequently, no bounded currents or charges are present at the interface, which is a more suitable description from the microscopic point of view. It is shown that the method converges to the local boundary conditions in the low spatial dispersion limit for insulators and conductors, quantified by means of a parameter defined as the "characteristic length".