Quantum Theory of Near-field Optical Imaging with Rare-earth Atomic Clusters

TL;DR

This paper develops a quantum theoretical framework for near-field optical imaging using rare-earth atomic clusters, enabling simultaneous detection of electric and magnetic local density of states, enhancing the interpretation of SNOM experiments.

Contribution

It introduces a quantum model coupling rare-earth ions with photonic nanostructures, allowing detailed analysis of electric and magnetic dipolar transitions in near-field imaging.

Findings

The formalism can describe light intensity from ED and MD transitions in scanning configurations.

Simulations show the model's usefulness for interpreting experimental SNOM data.

The approach accounts for external parameters like laser properties and probe size.

Abstract

Scanning near-field optical imaging (SNOM) using local active probes provides in general images of the electric part of the photonic local density of states. However, certain atomic clusters can supply more information by simultaneously revealing both the magnetic (m-LDOS) and the electric (e-LDOS) local density of states in the optical range. For example, nanoparticles doped with rare-earth elements like europium or terbium provide both electric dipolar (ED) and magnetic dipolar (MD) transitions. In this theoretical article, we develop a quantum description of active systems (rare earth ions) coupled to a photonic nanostructure, by solving the optical Bloch equations together with Maxwell's equations. This allows us to access the population of the emitting energy levels for all atoms excited by the incident light, degenerated at the extremity of the tip of a near-field optical microscope. We show that it is possible to describe the collected light intensity due to ED and MD transitions in a scanning configuration. By carrying out simulations on different experimentally interesting systems, we demonstrate that our formalism can be of great value for the interpretation of experimental configurations including various external parameters (laser intensity, polarization and wavelength, the SNOM probe size, the nature of the sample ...).