Theoretical Atto-nano Physics

TL;DR

This paper provides a comprehensive theoretical overview of the emerging field of atto-nano physics, exploring how ultrashort laser pulses interact with nanoscale systems and affect electron dynamics and related phenomena.

Contribution

It introduces the theoretical tools to understand laser-matter interactions at the intersection of attosecond and nanoscale physics, highlighting the effects of spatially inhomogeneous fields.

Findings

Modified electron dynamics due to inhomogeneous fields

Impact on above-threshold ionization processes

Influence on high-order harmonic generation

Abstract

Two emerging areas of research, attosecond and nanoscale physics, have recently started to merge. Attosecond physics deals with phenomena occurring when ultrashort laser pulses, with duration on the femto- and sub-femtosecond time scales, interact with atoms, molecules or solids. The laser-induced electron dynamics occurs natively on a timescale down to a few hundred or even tens of attoseconds (1 attosecond=1 as=10$^{-18}$ s), which is of the order of the optical field cycle. For comparison, the revolution of an electron on a $1s$ orbital of a hydrogen atom is $\sim152$ as. On the other hand, the second topic involves the manipulation and engineering of mesoscopic systems, such as solids, metals, and dielectrics, with nanometric precision. Although nano-engineering is a vast and well-established research field on its own, the combination with intense laser physics is relatively recent. We present a comprehensive theoretical overview of the tools to tackle and understand the physics that takes place when short and intense laser pulses interact with nanosystems, such as metallic and dielectric nanostructures. In particular, we elucidate how the spatially inhomogeneous laser-induced fields at a nanometer scale modify the laser-driven electron dynamics. Consequently, this has an important impact on pivotal processes such as above-threshold ionization and high-order harmonic generation. The deep understanding of the coupled dynamics between these spatially inhomogeneous fields and matter configures a promising way to new avenues of research and applications. Thanks to the maturity that attosecond physics has reached, together with the tremendous advance in material engineering and manipulation techniques, the age of atto-nano physics has begun, but it is still in an incipient stage.