Room temperature nanocavity laser with interlayer excitons in 2D heterostructures

TL;DR

This paper demonstrates the first room temperature interlayer exciton laser using MoS2/WSe2 heterostructures, operating in the infrared range and compatible with silicon photonics, enabled by long exciton lifetimes.

Contribution

It introduces the first room temperature interlayer exciton laser in 2D heterostructures, showcasing infrared emission and relaxed cavity quality requirements.

Findings

First room temperature interlayer exciton laser in 2D heterostructures

Infrared emission compatible with silicon photonics

Long exciton lifetime reduces cavity quality factor needs

Abstract

Atomically thin layered two dimensional (2D) material has provided a rich library for both fundamental research and device applications. One of the special advantages is that, bandgap engineering and controlled material response can be achieved by stacking different 2D materials. Recently several types of excitonic lasers have been reported based on Transition metal dichalcogenide (TMDC) monolayers, however, the emission is still the intrinsic energy bandgap of the monolayers and lasers harnessing the flexibility of Van der Waals heterostructures have not been demonstrated yet. Here, we report for the first time a room temperature interlayer exciton laser with MoS2/WSe2 heterostructures. The onset of lasing action was identified by a combination of distinct kink in the 'L-L' curve and the noticeable collapse of spectral linewidth. Different from visible emission of intralayer excitons for both MoS2 and WSe2, our interlayer exciton laser works in the infrared range, which is fully compatible with the well-established technologies in silicon photonics. Thanks to the long lifetime of interlayer excitons, the requirement of the cavity quality factor is relaxed by orders of magnitude. The demonstration of room temperature interlayer exciton laser might open new perspectives for the development of coherent light source with tailored optical properties on silicon photonics platform.