Peering into the darkness: vison-generated photon mass in quantum spin ice

TL;DR

This paper develops a theoretical framework to predict the dynamical photon mass in quantum spin ice, revealing how thermally activated visons create a measurable mass gap in neutron scattering experiments.

Contribution

It introduces a new method to calculate vison dynamics and their impact on the photon spectrum in quantum spin ice, including the effects of temperature-dependent vison plasma formation.

Findings

Visons induce a temperature-dependent mass gap in the photon spectrum.

The mass gap is detectable in energy-resolved neutron scattering spectra.

Visons do not cause confinement of static spinons.

Abstract

Describing experimental signatures of quantum spin ice has been the focus of many theoretical efforts, as definitive experimental verification of this candidate quantum spin liquid is yet to be achieved. Gapped excitations known as visons have largely eluded those efforts. We provide a theoretical framework, which captures their dynamics and predicts new signatures in the magnetic response. We achieve this by studying the ring-exchange Hamiltonian of quantum spin ice in the large-$s$ approximation, taking into account the compact nature of the emergent $U(1)$ gauge theory. We find the stationary solutions of the action -- the instantons -- which correspond to visons tunneling between lattice sites. By integrating out the instantons, we calculate the effective vison Hamiltonian, including their mass. We show that in the ground state virtual vison pairs simply renormalise the speed of light. At low temperatures, however, thermally activated visons form a Debye plasma and introduce a mass gap in the photon spectrum, equal to the plasma frequency, which we calculate as a function of temperature. We demonstrate that this dynamical mass gap should be visible in energy-resolved neutron scattering spectra but not in the energy-integrated ones. We also show that it does not lead to confinement of static spinons.