Time-resolving magnetic scattering on rare-earth ferrimagnets with a bright soft-X-ray high-harmonic source

TL;DR

This paper introduces a tabletop high-harmonic generation source enabling time-resolved X-ray magnetic scattering at the Tb N edge, revealing femtosecond dynamics of magnetic domains with high spatial resolution.

Contribution

It presents the first laboratory-scale setup for time-resolved X-ray resonant magnetic scattering at the N edge using high-harmonic generation, achieving high photon flux and femtosecond resolution.

Findings

Resolved femtosecond magnetic domain dynamics in Co/Tb alloys.

Observed magnetic domain expansion with domain wall velocity similar to spin transfer torque.

Achieved highest photon flux in 100-220 eV range using helium HHG.

Abstract

We demonstrate the first time-resolved X-ray resonant magnetic scattering (tr-XRMS) experiment at the N edge of Tb at 155 eV performed using a tabletop high-brightness high-harmonic generation (HHG) source. In contrast to static X-ray imaging applications, such optical-pump X-ray-probe studies pose a different set of challenges for the ultrafast driver laser because a high photon flux of X-rays resonant with the N edge must be attained at a low repetition rate to avoid thermal damage of the sample. This laboratory-scale X-ray magnetic diffractometer is enabled by directly driving HHG in helium with terawatt-level 1 um laser fields, which are obtained through pulse compression after a high-energy kHz-repetition-rate Yb:CaF2 amplifier. The high peak power of the driving fields allows us to reach the fully phase-matching conditions in helium, which yields the highest photon flux (>2x10^9 photons/s/1% bandwidth) in the 100-220 eV spectral range, to the best of our knowledge. Our proof-of-concept tr-XRMS measurements clearly resolve the spatio-temporal evolution of magnetic domains in Co/Tb ferrimagnetic alloys with femtosecond and nanometer resolution. In addition to the ultrafast demagnetization, we observe magnetic domain expansion with a domain wall velocity similar to that induced by spin transfer torque. The demonstrated method opens up new opportunities for time-space-resolved magnetic scattering with elemental specificity on various magnetic, orbital and electronic orderings in condensed matter systems.