Is the surface fluid during surface melting, a study of the surface shear modulus of solid Gallium

TL;DR

This study introduces a novel method to measure the surface shear modulus of solid Gallium, revealing that it abruptly vanishes near the premelting temperature, providing new insights into surface melting phenomena.

Contribution

The paper presents a new measurement technique for surface shear modulus and applies it to Gallium, uncovering the abrupt change near premelting, which was not previously observed.

Findings

Surface shear modulus vanishes abruptly near premelting

Surface melting begins about 9K below melting temperature

New measurement method for surface shear properties

Abstract

Melting of 3D solids is often preceded by a melting of their surface, a distinct process which begins at a temperature lower than the melting temperature. Until now, surface melting was investigated mostly by diffraction or other non-contact techniques, revealing how the surface becomes progressively disordered with temperature. We designed a method to measure an effective shear modulus of the surface, another property which should change at melting. This property was not measured before. We applied this method to surface melting of Gallium, and found that this surface shear modulus vanishes abruptly near the onset of premelting, about 9K below melting temperature.