Why phonon scattering in glasses is universally small at low temperatures
Herve M. Carruzzo, Clare C. Yu

TL;DR
This paper offers a new theoretical explanation for the universal smallness of phonon scattering in glasses at low temperatures, aligning well with experimental data across various glass types.
Contribution
It introduces a model with a broad distribution of phonon-TLS couplings that accounts for the universal phonon scattering behavior in glasses at low temperatures.
Findings
Good agreement between theory and experiment for various glasses.
Exponential renormalization of tunneling matrix elements.
Reduction of TLS density of states due to TLS-TLS interactions.
Abstract
We present a novel view of the standard model of tunneling two level systems (TLS) to explain the puzzling universal value of a quantity, , that characterizes phonon scattering in glasses below 1 K as reflected in thermal conductivity, ultrasonic attenuation, internal friction, and the change in sound velocity. Physical considerations lead to a broad distribution of phonon-TLS couplings that (1) exponentially renormalize tunneling matrix elements, and (2) reduce the TLS density of states through TLS-TLS interactions. We find good agreement between theory and experiment for a variety of individual glasses.
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Taxonomy
TopicsMaterial Dynamics and Properties · Spectroscopy and Quantum Chemical Studies · Glass properties and applications
