Structural disorder on small scales softens hierarchical structures

TL;DR

This study reveals that structural disorder at small scales significantly affects the rigidity and mechanical properties of hierarchical filamentous networks, despite similar large-scale scaling behaviors.

Contribution

It demonstrates that small-scale disorder influences network rigidity and surface structure, providing new insights into the mechanical behavior of hierarchical materials.

Findings

Small-scale disorder reduces network rigidity.

Disorder increases surface node fraction.

Large-scale scaling of stiffness remains unaffected.

Abstract

Hierarchically structured materials, which possess distinct features on different length scales, are ubiquitous in nature and engineering. In many cases, one structural level may be ordered while another structural level may be disordered. Here, we investigate the impact of structural disorder on the mechanical properties of hierarchical filamentous structures. Through simulations of networks with two hierarchical levels, we show that disorder does not change how stiffness scales with the mean coordination number - the average number of bonds per node - on large and small length scales. However, we find that network rigidity and stiffness depend strongly on the presence or absence of disorder on the small length scale, but not on the large length scale. In fact, the amount of material necessary for a fully connected, network ordered on the small scale is insufficient to create even a marginally rigid network with small-scale disorder. We trace these phenomena back to a difference in the maximum mean coordination number on the small scale. While single length scale ordered and disordered networks have similar mean coordination numbers in the interior and on surfaces, we find that disorder strongly impacts the structure of surfaces, resulting in a larger fraction of surface nodes on the small scale. While this effect increases in strength as large scale bonds become narrower, it persists even for bonds that are wider than they are long (i.e., aspect ratios < 1).