Pressure-induced suppression of charge density wave and emergence of Superconductivity in 1T-VSe2

TL;DR

This study investigates how high pressure affects charge density wave suppression and induces superconductivity in 1T-VSe2, revealing electronic structural changes and potential spin-fluctuation mechanisms.

Contribution

It provides the first detailed analysis of pressure-induced suppression of CDW and emergence of superconductivity in 1T-VSe2, highlighting electronic structure evolution.

Findings

CDW order enhances up to 240K at 12 GPa

Superconductivity appears at ~15 GPa with Tc ~4K

Electronic structure changes occur at 6 GPa and 12 GPa

Abstract

We report pressure evolution of charge density wave (CDW) order and emergence of superconductivity (SC) in 1T-VSe2 single crystal by studying resistance and magnetoresistance behavior under high pressure. With increasing quasi-hydrostatic pressure the CDW order enhances with increase ofthe ordering temperature up to 240K at 12 GPa. Upon further increase of pressure, the resistance anomaly due to CDW order gets suppressed drastically and superconductivity emerges at ~15 GPa, with the onset critical temperature (Tc) ~ 4K. The pressure dependence of Tc is found negligible, different from the significant increase or a dome-shape seen in iso-structural layered diselenide superconductors. The high pressure magnetoresistance and Hall measurements suggest successive electronic structural changes with Fermi surface modifications at 6 GPa and 12GPa. From the observed negative magnetoresistance in this pressure range and absence of coexisting CDW and SC phases, we propose that intra-layer spin-fluctuation can play a role in the emergence of superconductivity in the high pressure phase.