# Magnetic proximity in a van der Waals heterostructure of magnetic insulator and graphene

**Authors:** Bogdan Karpiak, Aron W. Cummings, Klaus Zollner, Marc Vila, Dmitrii Khokhriakov, Anamul Md Hoque, Andr\'e Dankert, Peter Svedlindh, Jaroslav Fabian, Stephan Roche, Saroj P. Dash

arXiv: 1908.05524 · 2025-06-06

## TL;DR

This paper demonstrates that stacking a ferromagnetic insulator with graphene induces out-of-plane magnetic interactions, significantly affecting spin transport and enabling potential applications in spintronics and quantum devices.

## Contribution

It provides experimental and theoretical evidence of proximity-induced ferromagnetism and anisotropic spin textures in graphene within a van der Waals heterostructure.

## Key findings

- Proximity-induced ferromagnetic exchange in graphene.
- Modification of spin transport due to magnetic anisotropy.
- Enhanced lifetime of perpendicular spins.

## Abstract

Engineering two-dimensional material heterostructures by combining the best of different materials in one ultimate unit can offer a plethora of opportunities in condensed matter physics. Here, in the van der Waals heterostructures of the ferromagnetic insulator Cr2Ge2Te6 and graphene, our observations indicate an out-of-plane proximity-induced ferromagnetic exchange interaction in graphene. The perpendicular magnetic anisotropy of Cr2Ge2Te6 results in significant modification of the spin transport and precession in graphene, which is ascribed to the proximity-induced exchange interaction. Furthermore, the observation of a larger lifetime for perpendicular spins in comparison to the in-plane counterpart suggests the creation of a proximity-induced anisotropic spin texture in graphene. Our experimental results and density functional theory calculations open up opportunities for the realization of proximity-induced magnetic interactions and spin filters in 2D material heterostructures and can form the basic building blocks for future spintronic and topological quantum devices.

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Source: https://tomesphere.com/paper/1908.05524