Experimental observation of coupled valley and spin Hall effect in p-doped WSe2 devices

TL;DR

This paper reports the experimental observation of coupled valley and spin Hall effects in p-doped WSe2 devices, demonstrating out-of-plane spin polarization and its detection, advancing spintronic applications with 2D materials.

Contribution

It provides the first experimental evidence of coupled valley and spin Hall effects in monolayer WSe2, enabling out-of-plane spin polarization without external magnetic fields.

Findings

Electrical generation of out-of-plane spin polarization in WSe2

Detection of spin signals via nonlocal spin valve on graphene

Confirmation of coupled valley and spin Hall effects in 2D TMDs

Abstract

Giant spin Hall effect (GSHE) has been observed in heavy metal materials such as Ta, Pt, and W, where spins are polarized in the surface plane and perpendicular to the charge current direction. Spins generated in these materials have successfully switched magnets with in-plane magnetic anisotropy (IMA) and perpendicular magnetic anisotropy (PMA) through spin orbit torque (SOT) mechanism. It is generally accepted that PMA magnets are preferred over IMA magnets in data storage applications owing to their large thermal stability even at ultra scaled dimensions. However, SOT switching of PMA magnets by conventional GSHE materials requires either a small external magnetic field, a local dipolar field, or introducing tilted anisotropy to break the symmetry with respect to the magnetization. To deterministically switch a PMA without any additional assistance, nonconventional GSHE materials that can generate spins with polarization perpendicular to the surfaces are needed. Several monolayer transition metal dichalcogenides (TMDs) have been predicted to generate such out of plane spins due to their 2D nature and unique band structures. Interestingly, opposite spins are locked to their respective sub-band in each K valley of the TMD valence band with substantially large energy splitting, which enables polarized spins to be accessible through electrical gating and spatially separated by electric field through the valley Hall effect (VHE). Therefore, spatial separation and accumulation of spins in these 2D TMDs are uniquely referred to as coupled valley and spin Hall effect. Here, we report an experiment of electrical generation of spin current with out of plane polarization in monolayer WSe2 and detection of spin signals through a nonlocal spin valve structure built on a lateral graphene spin diffusion channel that partially overlaps with WSe2.