$^{15}$C: from Halo-EFT structure to the study of transfer, breakup and radiative-capture reactions
Laura Moschini, Jiecheng Yang, Pierre Capel

TL;DR
This paper develops a Halo EFT model for $^{15}$C to analyze its structure and reactions, including transfer, breakup, and radiative capture, with results consistent with experimental data and implications for astrophysical nucleosynthesis.
Contribution
The work introduces a single Halo EFT model at NLO for $^{15}$C that accurately describes multiple reactions and clarifies the nuclear-structure observables involved.
Findings
Good agreement with experimental reaction data
Confirmed ANC value for $^{15}$C ground state
Estimated radiative-capture cross section at astrophysical energy
Abstract
Aside from being a one-neutron halo nucleus, C is interesting because it is involved in reactions of relevance for several nucleosynthesis scenarios. The aim of this work is to analyze various reactions involving C, using a single structure model based on Halo EFT. To develop a Halo-EFT model of C at NLO, we first extract the ANC of its ground state by analyzing C(d,p)C transfer data at low energy. Using this Halo-EFT description, we study the C Coulomb breakup at high (605AMeV) and intermediate (68AMeV) energies using eikonal models with a consistent treatment of nuclear and Coulomb interactions at all orders, and proper relativistic corrections. Finally, we study the C(n,)C radiative capture. Our theoretical cross sections are in good agreement with experimental data for all reactions, thereby assessing the robustness of…
| (fm) | (MeV) | (fm-1/2) |
|---|---|---|
| 0.6 | -591.05 | 0.865 |
| 0.8 | -339.87 | 0.934 |
| 1.0 | -222.43 | 1.01 |
| 1.2 | -157.95 | 1.09 |
| 1.4 | -118.68 | 1.17 |
| 1.6 | -92.933 | 1.26 |
| 1.8 | -75.095 | 1.36 |
| 2.0 | -62.212 | 1.46 |
| (fm-1) | Ref. | Method |
|---|---|---|
| 1.48 0.18 | Trache et al. (2002) | Knockout |
| 1.89 0.11 | Timofeyuk et al. (2006) | Mirror symmetry |
| 2.14 | Pang et al. (2007) | Transfer |
| 1.74 0.11 | Summers and Nunes (2008a, b) | Coulomb breakup |
| 1.64 0.26 | Mukhamedzhanov et al. (2011) | Transfer |
| 1.88 0.18 | McCleskey et al. (2014) | Transfer |
| 1.59 0.06 | this work | Transfer |
| (fm) | (MeV) | (MeV fm-2) | (MeV) | (MeV fm-2) |
|---|---|---|---|---|
| 1.2 | -3.1995 | -71.3 | 169.299 | -92.368 |
| 1.5 | -92.814 | -2.70 | -91.000 | -9.000 |
| 2.0 | -80.827 | 2.70 | -94.916 | 2.53 |
| (keV) | (b) Reifarth et al. (2008) | (b) |
|---|---|---|
| 23.3 | ||
| 150 | ||
| 500 | ||
| 800 |
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15C: from halo effective field theory structure
to the study of transfer, breakup and radiative-capture reactions
Laura Moschini
Physique Nucléaire et Physique Quantique (C.P. 229)
Université libre de Bruxelles (ULB), 50 avenue F.D. Roosevelt, B-1050 Brussels, Belgium
Jiecheng Yang
Physique Nucléaire et Physique Quantique (C.P. 229)
Université libre de Bruxelles (ULB), 50 avenue F.D. Roosevelt, B-1050 Brussels, Belgium
Afdeling Kern-en Stralingsfysica, Celestijnenlaan 200d-bus 2418, 3001 Leuven, Belgium
Pierre Capel
Institut für Kernphysik, Johannes Gutenberg-Universität Mainz, Johann-Joachim-Becher Weg 45, D-55099 Mainz, Germany
Physique Nucléaire et Physique Quantique (C.P. 229)
Université libre de Bruxelles (ULB), 50 avenue F.D. Roosevelt, B-1050 Brussels, Belgium
Abstract
Background
Aside from being a one-neutron halo nucleus, 15C is interesting because it is involved in reactions of relevance for several nucleosynthesis scenarios.
Purpose
The aim of this work is to analyze various reactions involving 15C, using a single structure model based on halo effective field theory (Halo EFT) following the excellent results obtained in [P. Capel, D. R. Phillips, and H.-W. Hammer, Phys. Rev. C 98, 034610 (2018)].
Method
To develop a Halo-EFT model of 15C at next to leading order (NLO), we first extract the asymptotic normalization coefficient (ANC) of its ground state by analyzing transfer data at low energy using the method developed in [J. Yang and P. Capel, Phys. Rev. C 98, 054602 (2018)]. Using the Halo-EFT description of 15C constrained with this ANC, we study the 15C Coulomb breakup at high (605 MeV/nucleon) and intermediate (68 MeV/nucleon) energies using eikonal-based models with a consistent treatment of nuclear and Coulomb interactions at all orders, and which take into account proper relativistic corrections. Finally, we study the radiative capture.
Results
Our theoretical cross sections are in good agreement with experimental data for all reactions, thereby assessing the robustness of the Halo-EFT model of this nucleus. Since a simple NLO description is enough to reproduce all data, the only nuclear-structure observables that matter are the 15C binding energy and its ANC, showing that all the reactions considered are purely peripheral. In particular, it confirms the value we have obtained for the ANC of the 15C ground state: fm*-1*. Our model of 15C provides also a new estimate of the radiative-capture cross section at astrophysical energy: b.
Conclusions
Including a Halo-EFT description of 15C within precise models of reactions is confirmed to be an excellent way to relate the reaction cross sections and the structure of the nucleus. Its systematic expansion enables us to establish how the reaction process is affected by that structure and deduce which nuclear-structure observables are actually probed in the collision. From this, we can infer valuable information on both the structure of 15C and its synthesis through the radiative capture at astrophysical energies.
I Introduction
The nucleus 15C is interesting for various reasons. On a nuclear-structure viewpoint, 15C is one of the best known one-neutron halo nuclei Tanihata (1996); Riisager (2013). Due to its small one-neutron separation energy [ MeV], the ground state of 15C is mostly described as a two-body structure, in which the valence neutron is loosely bound in a orbital to a 14C in its ground state. Thanks to its loose binding and the fact that it sits in an orbital, the valence neutron exhibits a high probability of presence at a large distance from the other nucleons. It therefore forms like a diffuse halo surrounding a compact core Hansen and Jonson (1987). The existence of halos in some nuclei challenges our view of the nucleus, which is usually seen as a compact object with a nucleon density at saturation. Halo nuclei, including 15C, are thus the focus of many experimental and theoretical studies Tanihata (1996); Riisager (2013).
The study of 15C has also applications in nuclear astrophysics. Its synthesis through one-neutron radiative capture by 14C has been suggested to be part of neutron-induced CNO cycles, which take place in the helium-burning zone of asymptotic-giant-branch (AGB) stars Wiescher et al. (1999). This 14CC reaction is also the doorstep to the production of heavy elements in inhomogeneous big-bang nucleosynthesis Kajino et al. (1990) and it has been shown to be part of possible reaction routes in the nuclear chart during the process in Type II supernovæ Terasawa et al. (2001). It is therefore necessary to have a reliable estimate of the cross section for this radiative capture at astrophysical energy, and hence to better understand the structure of 15C.
Because 15C exhibits a short lifetime, its structure cannot be probed with usual spectroscopic techniques. This nucleus is therefore mostly studied through reactions. Transfer, such as , measured in both direct and inverse kinematics, has been used to infer the single-particle structure of 15C Goss et al. (1975); Cecil et al. (1975); Murillo et al. (1994); Mukhamedzhanov et al. (2011). In breakup, the lose binding of the valence neutron to the core is broken up during the collision of the nucleus on a target, hence revealing its internal core- structure. Various experimental campaigns have been set up to measure the inclusive breakup—also known as knockout—of 15C on light targets at intermediate beam energies Tostevin et al. (2002); Sauvan et al. (2004); Fang et al. (2004). In these measurements, only 14C is detected after the reaction, and information pertaining to the single-particle structure of 15C is inferred from the analysis of the parallel-momentum distribution of the core. In Refs. Pramanik et al. (2003); Nakamura et al. (2009), the Coulomb (exclusive) breakup of 15C has been measured. In that case, both the 14C core and the halo neutron are detected in coincidence after the dissociation of the 15C projectile on a Pb target. Being dominated by the Coulomb interaction, this reaction process is rather clean as it exhibits little dependence on the choice of the optical potentials used to describe the nuclear interaction between the projectile constituents (core and ) with the target.
In addition to its interest in the study of the halo structure of 15C, Coulomb breakup has also been suggested as an indirect method to deduce the cross section for the C radiative capture at low energies Baur et al. (1986, 2003). The idea behind the Coulomb-breakup method is that this dissociation, which is often described as resulting from the exchange of virtual photons between the projectile and the heavy target Winther and Alder (1979), can be seen as the time-reversed reaction of the radiative capture, where a (real) photon is emitted following the capture of a neutron by the core. Later analyses have shown that the breakup process is not that simple and that higher-order effects spoil this nice picture Esbensen et al. (2005); Capel and Baye (2005). However, it has been suggested that the Coulomb-breakup measurements could be used to infer the asymptotic normalization coefficient (ANC) of the 15C ground-state wave function Summers and Nunes (2008a, b). However, due to the aforementioned higher-order effects, a precise model of the reaction is needed in the analysis of the reaction Summers and Nunes (2008a); Esbensen (2009); Capel and Nollet (2017). Because the radiative capture C is a purely peripheral process Timofeyuk et al. (2006), a reliable estimate of this ANC can then be used to compute its cross section. Following LABEL:15CANC_2006, it has also been suggested to rely on the strong sensitivity of transfer reaction to the single-particle structure of the nucleus to measure the ANC of the 15C ground-state wave function for that purpose Mukhamedzhanov et al. (2011).
Since the radiative capture C has been measured directly by Reifarth et al. Reifarth et al. (2008), the 15C case provides the opportunity to test the validity of the different indirect methods listed above.
In the present work, we reanalyze the transfer Goss et al. (1975); Mukhamedzhanov et al. (2011), Coulomb-breakup Pramanik et al. (2003); Nakamura et al. (2009) and radiative-capture Reifarth et al. (2008) measurements using one single description of the one-neutron halo nucleus 15C. For this, we follow the recent idea developed in LABEL:CPH18 and include, within precise models of reactions, a description of the nucleus based on halo effective field theory (Halo EFT) Bertulani et al. (2002) (see Ref. LABEL:HJP17 for a recent review). Halo EFT exploits the natural separation of scales that is observed in halo nuclei—viz. the difference between the small size of the core and the large extension of the halo —to build an effective Hamiltonian constructed as an expansion in powers of the small parameter . This allows us to introduce, order by order, the different nuclear-structure parameters in the description of the nucleus within the reaction models, and thereby to deduce how each of them affects the reaction processes. This puts a strong constraint on what can be learned about the structure of 15C from transfer and breakup experiments and how this nuclear-structure information relates to the direct radiative-capture capture measurement of LABEL:Reifarth2008.
This article is structured as follows. In Sec. II we introduce the Halo EFT description of 15C and explain how it is fitted at next to leading order (NLO). Using this description, we reanalyze transfer measurements at Goss et al. (1975) and MeV Mukhamedzhanov et al. (2011) in Sec. III. In Sec. IV we use the same 15C structure to study its breakup at high (605 MeV/nucleon Pramanik et al. (2003)) and intermediate (68 MeV/nucleon Nakamura et al. (2009)) energy. In Sec. V, we study the radiative capture Reifarth et al. (2008). Finally, in Sec. VI, we summarize our results and provide the outlook for future work.
II Halo-EFT description of 15C
II.1 Single-particle structure of 15C
Being a one-neutron halo nucleus, 15C can be modeled as a neutron loosely bound to a 14C core. With the assumption that the 14C core is in its ground state (), the \mbox{\frac{1}{2}}^{+} ground state (g.s.) of 15C can be described by a 14C() configuration and its \mbox{\frac{5}{2}}^{+} excited state (e.s.) by a 14C(). These states have an energy relative to the one-neutron threshold of MeV and MeV, respectively.
To model this system, the core of mass and charge is assumed to be of spin and parity and we neglect its internal structure. The halo nucleus is thus of mass , with the neutron mass, and charge . Such a two-body structure is described by the internal Hamiltonian
[TABLE]
where is the - relative coordinate, is their reduced mass, and is the effective potential simulating their interaction. In partial wave , the eigenstates of read
[TABLE]
where is the total angular momentum resulting from the coupling of the orbital angular momentum with the spin of the halo neutron and is its projection. The eigenstates of of negative energy are discrete and correspond to the bound states of the two-body model of the projectile . These include physical - bound states of the system as well as Pauli forbidden states, which simulate the presence of neutrons within the core . We enumerate them by adding the number of nodes in the radial wave function to the other quantum numbers. They are normed to unity and their reduced radial wave function behaves asymptotically as
[TABLE]
where , whith the - binding energy, and is a spherical Bessel function of the third kind Abramowitz and Stegun (1970). The single-particle asymptotic normalization constant (SPANC) defines the strength of the exponential tail of the - bound-state wave function Blokhintsev et al. (1977). This SPANC will vary with the geometry of the potential used to simulate the - interaction McCleskey et al. (2014); Belyaeva et al. (2014); Timofeyuk (2014); Capel and Nunes (2006). The asymptotic behavior (3) is universal, therefore it exists also in the actual structure of the nucleus, viz. in the overlap wave function obtained within a microscopic calculation of the nucleus Capel et al. (2010); Timofeyuk (2014). Being affected by the inherent couplings between the different configurations in the actual structure of the nucleus, in particular those involving the core in one of its excited states, the true asymptotic normalization constant (ANC) of the overlap wave function of the physical state of spin and parity corresponding to the configuration in which the core is in its ground state, , differs from the SPANC obtained in the effective single-particle description considered here Capel et al. (2010); Timofeyuk (2014).
The positive-energy states describe the - continuum, i.e. the broken-up projectile. Their reduced radial parts are normalized according to
[TABLE]
where is the phaseshift at energy and ; and are spherical Bessel functions of the first and second kinds, respectively Abramowitz and Stegun (1970).
As mentioned above, the - interaction is described by an effective potential . In this study, following the idea developed in LABEL:CPH18, this potential is built within a Halo-EFT description of the nucleus Bertulani et al. (2002); Hammer et al. (2017). At the leading order (LO), this interaction consists of a simple contact term within the sole wave. As usual, this interaction is regularized with a Gaussian
[TABLE]
The range of the Gaussian corresponds to the scale of the short-range physics neglected in this Halo-EFT description. Changing its value will enable us to generate different single-particle wave functions to describe the 14C- system and hence test the sensitivity of our reaction calculations to the internal part of the wave function of the projectile. At LO, the only free parameter is adjusted to reproduce MeV within a orbit.
At next-to-leading order (NLO), the interaction is extended up to the waves and contains, in addition to the contact term its second-order derivative. For simplicity, we follow Ref. Capel et al. (2018) and use the equivalent following parametrisation of the interaction
[TABLE]
To constrain the potential parameters and in the wave, we need two structure observables: in addition to the binding energy of the state, we also use its ANC. Various groups have estimated this ANC from reaction data Trache et al. (2002); Timofeyuk et al. (2006); Pang et al. (2007); Summers and Nunes (2008a, b); Mukhamedzhanov et al. (2011); McCleskey et al. (2014). In this work, we use the method presented in LABEL:yang-capel to deduce this ANC from low-energy transfer data selected at forward angle (see Sec. II.2).
Unlike 11Be, 15C does not exhibit any low-lying bound or resonant \mbox{\frac{3}{2}}^{-} or \mbox{\frac{1}{2}}^{-} states to which we could fit the effective interaction (6) in the waves. Therefore, true to the spirit of Halo-EFT, we set this interaction to 0 in the and partial waves. Interestingly, this treatment is in agreement with preliminary results obtained in an ab initio calculation of 15C performed within the no-core shell model with continuum (NCSMC), which predicts negligible phaseshifts at low 14C- energies in both waves Navrátil (2018).
At NLO, the interaction is nil in higher partial waves. Since the \mbox{\frac{5}{2}}^{+} excited bound state of 15C plays a role in the radiative capture (see Sec. V), we follow the idea of LABEL:CPH18 and go beyond NLO to include a state at MeV. The potential in that partial wave is chosen similar to that of Eq. (6). We fit the depths and to reproduce the experimental binding energy of the \mbox{\frac{5}{2}}^{+} state and the ANC deduced from transfer data.
II.2 Extraction of the ANC of the 15C bound states from the analysis of low-energy transfer reactions
To obtain a reliable estimate of the ANC of both bound states of 15C, we follow the idea developed in Ref. Yang and Capel (2018) and reanalyze 14CC transfer data. In that reference, it was found that transfer reactions are purely peripheral when they are performed at low beam energy (viz. MeV) and when the data are selected at forward angles. Within these experimental conditions, the transfer cross section scales perfectly with the square of the final state ANC . That value can then be reliably extracted from a comparison between reaction calculations performed using a single-particle description of the nucleus similar to the one presented in Sec. II.1 and experimental data Yang and Capel (2018).
We therefore need 14CC transfer data measured at low energies, and which contain enough data points at forward angles for this extraction of the ANC of 15C to be statistically meaningful. Two experiments satisfying the low-energy condition have been performed: one at the University of Notre Dame at MeV Goss et al. (1975), and another at the Nuclear Physics Institute of the Czech Academy of Sciences at MeV Mukhamedzhanov et al. (2011). Unfortunately, the former contains only one point at , which we deem not enough for this extraction. Fortunately, although performed at a slightly higher energy, the latter experiment contains six points at , which seems enough to constrain the ANC within proper peripheral conditions (see below).
Following the method presented in LABEL:yang-capel, we couple a leading order (LO) Halo-EFT description of 15C with a finite-range adiabatic distorted wave approximation (FR-ADWA) model Johnson and Tandy (1974). This model provides a reliable description of transfer reactions at these energies Nunes and Deltuva (2011); Upadhyay et al. (2012). As in LABEL:yang-capel, we consider the CH89 global potential Varner et al. (1991) to generate the optical potentials in the incoming (-14C) and outgoing (-15C) channels. The Reid soft core potential Reid (1968) is used to compute the deuteron bound state. The deuteron adiabatic potentials are obtained with the frontend code of TWOFNR Igarashi and Toyama (2008) and the transfer calculations are performed using FRESCO Thompson (1988). We illustrate here the results for the ground state, the method to extract the ANC of the excited state is analogous, though less efficient because it corresponds to a 14C- bound state (see Ref. Yang and Capel (2018) for the details).
We first build eight Gaussian potentials at the LO of Halo-EFT [see Eq. (5)] considering different ranges between fm and fm. For each width the depth is adjusted to reproduce the neutron binding energy in the 15C final state (see Table 1). These potentials provide different single-particle radial wave functions with very different SPANCs , but also a significant change in the surface part of the nucleus, i.e. in the range fm, see Fig. 1. This is the corner stone of the method developed in LABEL:yang-capel, because it is known that transfer reactions can be sensitive to that region Pang et al. (2007); Timofeyuk (2014). Using single-particle wave functions that strongly differ, not only in their SPANC, but also in their shape within that surface region will enable us to accurately determine the conditions under which the reaction is purely peripheral, and thus under which a reliable estimate of the actual ANC of the nucleus can be inferred.
With this input, we compute within the FR-ADWA Johnson and Tandy (1974) the corresponding theoretical differential cross section for the transfer to the 15C g.s. at MeV Mukhamedzhanov et al. (2011), expressed as a function of the relative direction between the proton and the 15C in the outgoing channel. These results are displayed in Fig. 2(a) for the eight g.s. wave functions shown in Fig. 1. At forward angles, the cross sections exhibit a huge sensitivity to the choice of the 14C- wave function. They seem to scale with the square of the SPANC, as one would expect if the process were purely peripheral Yang and Capel (2018). To confirm this, we have plotted the transfer cross section scaled by in Fig. 2(b). In this way, the spread in the results is significantly reduced at forward angles.
To precisely determine within which angular range the data should be limited to select strictly peripheral conditions, we remove the major angular dependence by considering the ratio
[TABLE]
where the transfer cross section computed using the 14C- Gaussian potential of range , scaled by the square of the corresponding SPANC , is divided by the result obtained with fm, which is at the center of the range in . The results are displayed in Fig. 2(c). We see that all ratios fall very close to one another at small angles, confirming the peripherality of the reaction when data measured at low beam energy are selected in the forward direction. To define an angular range in which the reaction can be considered as peripheral, we consider a maximum of difference [horizontal black dotted lines in Fig. 2(c)]. In this case, this happens only at very forward angles, viz. when . There are six data points within this angular region in this experiment Mukhamedzhanov et al. (2011). Note that there is no data available within this angular range in the case of the experiment performed at the lower energy MeV Goss et al. (1975).
Having determined the angular region within which the process is purely peripheral, we extract the value of the ANC for each of the single-particle wave function shown in Fig. 1. This is done by scaling, through a minimization, the corresponding theoretical cross section to the data selected at Yang and Capel (2018). The ANCs obtained in this way are shown in Fig. 3 as a function of the potential width . The error bars correspond to the uncertainty in the minimization. Despite the huge changes in the radial wave functions observed in Fig. 1, the ANCs extracted are nearly independent of ; they fall within 4% from each other. This is similar to what was obtained for 11Be (see Fig. 8 of LABEL:yang-capel), hence confirming the validity of the method.
To deduce an estimate of the actual ANC , we average the results and get fm*-1/2* ( fm*-1*) displayed as the horizontal red dashed line and gray band in Fig. 3. Following the same process, we obtain for the e.s. an estimate of the ANC of fm*-1/2*.
We compare our estimate with values extracted from the analysis of other experiments in Table 2. Though on the lower end of the range, the ANC we obtain agrees with most of the others. Our value is within the uncertainty band of the ANC extracted from knockout measurements in LABEL:15CANC_2002, which is not surprising because that reaction is mostly peripheral Hebborn and Capel (2019). Compared to the value extracted from the width of the \mbox{\frac{1}{2}}^{+} ground state of the proton-unbound mirror nucleus 15F, our seems too low. However, as explained in LABEL:Muk10, that resonant state being quite broad, its width used in this analysis might be marred with significant uncertainty. In LABEL:15CANC_2007, Pang et al. have used the aforementioned 14CC transfer data measured at MeV Goss et al. (1975), which have not enough points at forward angles to be purely peripheral. Its large value is most likely due to that issue. Note also that the normalization of the MeV data has been questioned in LABEL:17MeVdp. Interestingly, we are in excellent agreement with the value obtained by Summers and Nunes in their analysis Summers and Nunes (2008a, b) of the Coulomb breakup cross section of 15C measured at RIKEN Nakamura et al. (2009). Since this reaction is very peripheral Capel and Nunes (2007); Capel and Nollet (2017), this is not surprising (see Sec. IV.2). Our ANC is also perfectly compatible with the value extracted from the same data at MeV in LABEL:17MeVdp. The we have obtained is on the lower end of the uncertainty range of the value extracted from the C and C transfer experiments in LABEL:15CANC_2014. However, these experiments have been performed at energies corresponding to MeV, where the reaction is not fully peripheral Yang and Capel (2018), which may explain the slight disagreement with our ANC.
The value we have obtained from the method developed in LABEL:yang-capel is therefore in good agreement with most of the values cited in the literature, and the differences we observe with previous analyses can be explained from uncertainties in these analyses. Incidentally, as was observed in our previous analysis of the transfer Yang and Capel (2018), this ANC for the ground state of 15C is in excellent agreement with the fm*-1* obtained by Navrátil et al. in the aforementioned ab initio calculation of this one-neutron halo nucleus Navrátil (2018). The present work will therefore provide a stringent test of the value predicted in that NCSMC calculation.
II.3 Halo-EFT description of 15C at NLO
Having inferred a reliable value of the ANC for the 15C g.s., we can now proceed as suggested in LABEL:CPH18 and adjust a NLO Halo-EFT potential (6) to describe this nucleus within our reaction models. In the partial wave, the two depths of the Gaussian potential are fitted to reproduce the experimental binding energy of the halo neutron to the core and our ANC. As in Refs. Capel et al. (2018); Moschini and Capel (2019), we perform this fit for three different ranges to test the sensitivity of our reaction calculations to the short-range physics of the 14C- overlap wave function. The depths obtained by these fits are listed in Table 3.
As mentioned earlier, the interaction in the wave is set to zero, in agreement with preliminary results of the ab initio calculations Navrátil (2018). In Table 3, we also provide the depths for 14C- potentials in the partial wave, which are fitted to reproduce the binding energy and ANC of the \mbox{\frac{5}{2}}^{+} excited bound state of 15C. This goes beyond the NLO of Halo EFT, but it will enable us to check the influence of the presence of that state in the 15C spectrum in reaction calculations Capel et al. (2018).
Figure 4 displays the single-particle radial wave functions generated by the three potentials of Table 3. By construction, they exhibit the identical behavior in the asymptotic region, viz. for fm. However, as expected, the three wave functions exhibit significant differences at short distances, which will enable us to test the sensitivity to the short-range physics of 15C of the various reactions we consider in the following.
III Transfer reaction 14CC
We start our analysis of the reactions involving 15C using the NLO description developed in Sec. II.3 by looking at how it behaves in transfer reactions. We consider the low-energy reactions measured at MeV Mukhamedzhanov et al. (2011) and MeV Goss et al. (1975). We use the same FR-ADWA model Johnson and Tandy (1974) and potentials employed to extract the ANC in the previous section.
Figure 5 displays the cross sections for the C transfer reaction obtained at (a) MeV and (b) MeV. The results of the FR-ADWA calculations for each of the three ranges of the Gaussian NLO potential (6) are shown in the same colors and line types as the corresponding radial wave functions in Fig. 4. The green band shows the uncertainty in the cross sections, obtained with the Gaussian potential of range fm, related to the uncertainty in the ANC we have extracted in Sec. II.2. For comparison, we also show the results obtained with the LO description of 15C using fm (purple dashed line).
At MeV, without much surprise, the agreement of our NLO calculations with the data is perfect at forward angle since this is the region within which the fit has been performed in Sec. II.2. The transfer cross section obtained with the LO description of 15C misses the data by a factor that corresponds to the value of the ANC, which is not fitted at this order. This confirms the importance of fitting both the energy and the ANC of the bound state to correctly reproduce the data. All three NLO 14C- potentials provide the same cross section in the angular range of peripherality of the reaction, viz. . The agreement between the different wave functions actually extends beyond that range. At larger angles, however, the transfer cross sections obtained with the three different single-particle wave functions differ from one another, confirming that, at large angles, the reaction is sensitive to the short-range physics in 15C. The uncertainty band encompasses the error bars of the forward-angle data, but cannot explain the discrepancy between our calculations and the experimental points at large angles. This shows the limit of the present approach: Halo-EFT provides a proper low-energy—viz. large distances—description of the projectile, but, by construction, does not account for the details of the internal part of the 15C wave function. Hopefully, including a more precise wave function of the projectile could improve the description of the data at large angles. This could be done, e.g., using the overlap wave function provided by the ab initio calculation of Navrátil et al. Navrátil (2018). Alternatively, one could use a more elaborated two-body model of 15C, e.g., including core-excitation Gómez-Ramos et al. (2015).
IV Coulomb breakup of 15C
We now turn to the Coulomb breakup of 15C. As mentioned in the Introduction, this reaction has been measured on a lead target twice at two different energies. First at GSI at 605 MeV/nucleon by Datta Pramanik et al. Pramanik et al. (2003) and second at RIKEN at 68 MeV/nucleon by Nakamura and his collaborators Nakamura et al. (2009). These two experiments are similar to those performed previously on the one-neutron halo nucleus 11Be Palit et al. (2003); Fukuda et al. (2004), which were recently successfully analyzed using a Halo-EFT description of 11Be Capel et al. (2018); Moschini and Capel (2019). We therefore follow these references and apply the same models of the reaction using the NLO description of 15C detailed in Sec. II.3.
IV.1 Breakup of 15C on lead at MeV/nucleon
To analyze the breakup cross section of 15C measured on Pb at GSI at 605 MeV/nucleon Pramanik et al. (2003), we follow what we did in LABEL:MC19 and use an eikonal-based model of the reaction Glauber (1959); Baye and Capel (2012), which properly accounts for special relativity.
In that model, the projectile is described by the two-body system introduced in Sec. II: a core , to which a neutron is loosely bound, and which interact through the NLO Halo-EFT potential adjusted in Sec. II.3. The target is seen as a structureless body of mass and charge , which interacts with the projectile constituents and through the potentials and , respectively. We solve the problem within the Jacobi set of coordinates composed of the internal coordinate of the projectile [see Eq. (1)] and the relative coordinate of the projectile center of mass to the target . The latter is explicitly decomposed into its longitudinal and transverse components relative to the incoming beam axis.
At this high beam energy, the use of the eikonal approximation is fully justified as well as the usual adiabatic—or sudden—treatment of the projectile dynamics during the reaction, i.e., we neglect the change in the projectile internal energy in comparison with its kinetic energy. To properly account for special relativity, we follow Satchler Satchler (1992) and derive the eikonal wave function, which describes the projectile-target relative motion, from the Klein-Gordon equation expressed within the - center-of-momentum (CM) frame Satchler (1992); Pang (2014). Within this description of the reaction, the three-body wave function exhibits the following asymptotic behavior
[TABLE]
where is the initial - momentum, is the eikonal phase that accounts for the interaction between the target and the projectile constituents, and is the wave function of the projectile ground state, in which it is assumed to be initially. Formally, the eikonal phase reads Glauber (1959); Baye and Capel (2012)
[TABLE]
where is the - relative velocity. This phase can be interpreted semi-classically by seeing the projectile following a straight-line trajectory at fixed impact parameter along which its wave function accumulates a complex phase due to its interaction with the target. It is composed of three terms: . The first , with , the Sommerfeld parameter of the reaction, simply describes the Coulomb scattering of the projectile by the target Bertulani and Danielewicz (2004). It does not depend on , and hence does not contribute to the breakup of . The second
[TABLE]
is the Coulomb term that contributes to the excitation of the projectile. This phase diverges because the infinite range of the Coulomb interaction is not compatible with the sudden approximation, which assumes that the collision takes place in a short time. To solve this issue, we use the Coulomb correction to the eikonal model (CCE) detailed in Refs. Margueron et al. (2003); Capel et al. (2008). In that correction, the diverging eikonal Coulomb phase (10) is replaced at the first order by the first order of the perturbation theory Capel et al. (2008)
[TABLE]
For the first-order estimate of the Coulomb phase, we consider the relativistic expression limited to the E1 term Winther and Alder (1979)
[TABLE]
where 111Note the difference with LABEL:MC19, where we had considered for the calculation of the velocity of the projectile in the CM rest frame. Note also the correct formulation of our equation (12) with the factor (check Eq. (2.15) of Ref. Winther and Alder (1979)). These corrections have little effect on our results..
The third term of the eikonal phase corresponds to the nuclear interaction. At low and intermediate energies, it is usually described by optical potentials fitted to reproduce elastic-scattering cross sections. At high energy, and especially for exotic nuclei, it is difficult to find appropriate potentials. Therefore, we rely on the optical limit approximation (OLA) of the Glauber theory Glauber (1959); Bertulani and Danielewicz (2004), which has been successfully used in previous studies Horiuchi et al. (2010); Moschini and Capel (2019). In that approximation, the nuclear eikonal phase is obtained by averaging a profile function , which simulates the nucleon-nucleon interaction, over the density of the colliding nuclei
[TABLE]
where stands for either or , the two constituents of the projectile, and where and are the transverse components of the internal coordinate of the target () and (), respectively. In our three-body model of the reaction, the nuclear eikonal phase thus reads
[TABLE]
We consider the usual form of the profile function
[TABLE]
where is the total cross section for the collision, corresponds to the ratio of the real to the imaginary part of the -scattering amplitude, and is the slope of elastic differential cross section. These parameters are isospin dependent, which means that, in practice, the OLA phase (13) splits into four terms. For the parameters of Eq. (15) we use the values provided in Ref. Abu-Ibrahim et al. (2008) for an energy of 650 MeV. The densities used in Eq. (13) for the 14C core and the 208Pb target are approximated by the two-parameter Fermi distributions of Ref. Chamon et al. (2002), in which the authors study a systematization of nuclear densities based on charge distributions extracted from electron-scattering experiments as well as on theoretical densities derived from Dirac-Hartree-Bogoliubov calculations. For , we consider a Dirac delta function.
The breakup cross sections obtained with this model of reaction are displayed in Fig. 6 as a function of the relative energy between the 14C core and the neutron after dissociation. To enable the comparison with the experimental data of LABEL:Dat03, all theoretical cross sections have been folded with the experimental energy resolution, which we have considered identical to the one provided by Palit et al. in the analysis of the Coulomb breakup of 11Be measured at GSI Palit et al. (2003). The calculations performed with all three 14C- potentials listed in Table 3 are shown. The sensitivity of our calculations to the uncertainty in the 15C g.s. ANC extracted in Sec. II.2 is shown by the green band. The result of the calculation obtained without relativistic corrections is displayed as the purple dashed line. This clearly demonstrates the significance of these corrections at this beam energy.
Let us first note that our theoretical predictions are in excellent agreement with the data at all energies. As expected, we do not note any appreciable difference between the calculations performed with the different Halo-EFT wave functions (see Fig. 4). This result confirms that this reaction is purely peripheral, in the sense that it is sensitive only to the tail of the projectile wave function and not to its interior. The excellent agreement with the data observed in this reaction observable suggests that the ANC we have extracted from the transfer data, combined with the choice of a nil interaction in the 14C- partial waves, is valid structurewise Capel and Nollet (2017). Accordingly, the predictions of the ab initio calculations of Navrátil et al. seem correct Navrátil (2018).
In a subsequent test, we have analyzed how the inclusion of the 15C e.s.—described here as a bound state (see Sec. II.1)—affects our breakup calculations. The presence of that state in the 15C spectrum has no significant effect upon this reaction process; calculations performed with the Halo-EFT descriptions of 15C beyond NLO, which include this state, are nearly identical to those shown in Fig. 6. This is reminiscent of what has been observed in LABEL:CPH18 in the analysis of the RIKEN Coulomb breakup experiment of 11Be Fukuda et al. (2004), in which the presence of the \mbox{\frac{5}{2}}^{+} resonance, also described within the partial wave, is barely noticeable in the cross section. This result is not surprising in a reaction that is strongly dominated by an E1 transition from the bound state towards the continuum. The existence of a state in the low-energy spectrum of the projectile is more clearly seen in nuclear-dominated reactions, where quadrupole transitions are more significant Capel et al. (2018); Hebborn and Capel (2019). Therefore, for this Coulomb-dominated reaction, a Halo-EFT expansion limited to NLO is sufficient: the bound state would actually appear only at the next order (i.e. next to next to leading order, N2LO), and it has nearly no influence in our breakup calculations. This hence suggests that staying at NLO with a potential fitted to the ANC and binding energy of the g.s. in the wave and a nil potential in the wave, is enough to describe the experimental energy distributions for the breakup of 15C.
IV.2 Breakup of 15C on lead at MeV/nucleon
The Coulomb breakup of 15C has also been measured on Pb at RIKEN at MeV/nucleon by Nakamura et al. Nakamura et al. (2009). To reanalyze these data using the Halo-EFT description of 15C developed in Sec. II.3, we consider the dynamical eikonal approximation (DEA) Baye et al. (2005); Goldstein et al. (2006). This model of reaction is also based on the eikonal approximation, however, it does not include the usual adiabatic approximation, which means that it properly includes the dynamics of the projectile during the collision, which has been shown to matter at this intermediate beam energy Esbensen et al. (2005); Capel and Baye (2005); Summers and Nunes (2008a); Esbensen (2009). Besides having proved to be very efficient in the description of various observables measured in the breakup of one-neutron Goldstein et al. (2006) and one-proton Goldstein et al. (2007) halo nuclei, the model has been shown to be in excellent agreement with other breakup models on this very reaction Capel et al. (2012).
Following LABEL:CPH18, we include the 14C- Halo-EFT potentials within the DEA and compute the breakup cross section at the RIKEN energy. To describe the nuclear interaction between the projectile constituents and the target, we follow LABEL:CEN12 and consider optical potentials found in the literature. The 14C-Pb potential is obtained from the scaling of an 16O-Pb potential fitted to reproduce the elastic-scattering cross section of these nuclei at 94 MeV/nucleon Roussel-Chomaz et al. (1988). We simply scale the radius of the potential by to account for the mass difference between 16O and 14C and ignore the difference in beam energy. We use the Bechetti and Greenlees global nucleon-target optical potential to simulate the -Pb interaction Becchetti and Greenlees (1969). Note that the details of these interactions are provided in the supplemental material of LABEL:CEN12.
The results of these calculations are shown in Fig. 7 as a function of the 14C- continuum energy . We consider the two angular cuts under which the experimental data have been measured, i.e., , which includes the entire significant angular range, and , the forward-angle selection. To allow for a direct comparison with the data of LABEL:Nak09-15C, the results of our calculations have been folded with the experimental energy resolution. The green band shows the effect of the uncertainty on the ANC.
As in our analysis of the GSI experiment Pramanik et al. (2003), we obtain an excellent agreement with the data on the whole energy spectrum. All three NLO 14C- potentials lead to identical cross sections showing that, at this energy also, the reaction is purely peripheral and that the ANC we have extracted from the low-energy transfer data and the nil phaseshift in the 14C- waves are consistent with this other set of data. Our analysis hence independently confirms the value of the ANC extracted by Summers and Nunes from this same Coulomb breakup cross section Summers and Nunes (2008a, b). The slightly larger ANC they have obtained (see line 4 of Table 2) is probably due to their use of a non-zero interaction in the wave, which tends to reduce these contributions to the breakup Capel and Nunes (2006); Capel and Nollet (2017); Capel et al. (2018). Since there is no experimental observable upon which to constrain the phaseshift in these partial waves, we have to rely on theoretical hypotheses. We have made a choice consistent with what we have done in the 11Be case Capel et al. (2018) and with preliminary ab initio predictions Navrátil (2018). As shown in LABEL:CN17, for the Coulomb breakup of loosely bound wave nuclei, it is the combination of ANC in the g.s. and phaseshift in the continuum that matters, especially at low energy in the 14C- continuum and forward scattering angle. The excellent agreement with the data displayed in Figs. 5, 6, and 7 justifies our choice. However, the uncertainty in the data is not sufficiently small to disprove the choice made in LABEL:SN08. Using their choice of 14C- potentials would most likely provide as good an agreement with experiment as ours. Incidentally, this also confirms the ab initio prediction of Navrátil et al. for the ANC of the 15C g.s.
In addition to these NLO calculations, we have also performed another set of calculations going beyond NLO by including the e.s. in the 15C spectrum as a bound state. The results, not shown here for clarity, are identical to those displayed in Fig. 7, confirming that in Coulomb-dominated reactions the details in the description of the waves are irrelevant, and that an NLO Halo-EFT description of the projectile is sufficient.
V Radiative capture
As mentioned in the Introduction, the radiative capture of a neutron by 14C to form a 15C nucleus [] plays a significant role in various astrophysical sites, from the possible inhomogeneous big-bang nucleosynthesis Kajino et al. (1990) to neutron-induced CNO cycles in AGB stars Wiescher et al. (1999) and possible role in Type II supernovæ Terasawa et al. (2001). It is therefore useful for models of these astrophysical phenomena to have a reliable estimate of this reaction rate. Unfortunately it is difficult to measure directly: both reactants are radioactive and, although 14C targets can be provided, obtaining purely monochromatic neutron beams is not simple. This is why indirect techniques, such as the Coulomb-breakup method Baur et al. (1986, 2003), have been proposed. Nevertheless, recently, Reifarth et al. have taken up the gauntlet and performed a direct measure of this radiative capture Reifarth et al. (2008).
In Sec. IV, we have shown that the Halo-EFT description of 15C at NLO was sufficient to describe the breakup cross sections measured at GSI Pramanik et al. (2003) and RIKEN Nakamura et al. (2009). As expected from the analyses published in Refs. Summers and Nunes (2008a); Esbensen (2009); Capel and Nollet (2017), this model of 15C should also provide a good estimate for the radiative-capture cross section at low energy. In this section, we compare our prediction with the data of Reifarth et al. Reifarth et al. (2008).
The radiative-capture is dominated by the E1 transition from the waves in the 14C- continuum towards the ground state of 15C. A small contribution comes also from the capture from the continuum waves to the excited state of the nucleus. Since these two contributions cannot be disentangled in the experiment of Reifarth et al. we use the Halo-EFT description of 15C beyond NLO to include this excited state in our model of the reaction. To perform the calculations, we proceed as in LABEL:CN17.
The radiative-capture cross section obtained in this way is displayed in Fig. 8 as a function of the relative energy between the neutron and the 14C nucleus in the entrance channel. The three 14C- Gaussian potentials provide identical cross sections, confirming that this reaction is purely peripheral Timofeyuk et al. (2006). The effect of the ANC uncertainty is shown by the green band. The contribution due to the capture towards the e.s. is, as observed elsewhere Reifarth et al. (2008); Esbensen (2009); Capel and Nollet (2017), of the order of 5%. The details of the description of this state, and especially the accuracy of its ANC extracted from transfer data, are thus completely negligible in this analysis. We have checked that the contribution of the E2 term to the radiative capture is orders of magnitude lower than the E1. The cross section displayed in Fig. 8 is in excellent agreement with prior predictions Timofeyuk et al. (2006); Summers and Nunes (2008b); Rupak et al. (2012); Capel and Nollet (2017) and the ab initio prediction of Navraátil et al. Navrátil (2018). It is however slightly lower than what has been obtained in the analysis of the direct experiment Reifarth et al. (2008).
To properly confront these results with the data measured by Reifarth et al. Reifarth et al. (2008), we need to account for the distribution of the neutron energy in the incoming beam Capel and Nollet (2018). The values averaged over the neutron distributions shown in Fig. 3 of LABEL:Reifarth2008 are provided in Table 4 alongside the experimental data.
The experimental values are the ones provided in Table V of LABEL:Reifarth2008. The theoretical cross sections are the one obtained using the 14C- potentials listed in Table 3 of the present article. These values include the small contribution of the capture to the bound state that simulates the \mbox{\frac{5}{2}}^{+} e.s. of 15C. The uncertainty provided for the theoretical value corresponds to the uncertainty on the ANC of the g.s. of 15C. The sensitivity to the range of the Gaussian potential (6) is smaller than the precision provided here.
Our theoretical predictions are usually in good agreement with the experimental values of Reifarth et al. Reifarth et al. (2008). The only significant difference is observed at the lowest energy point, where our prediction lies two sigma lower than the measured cross section. This seems to be an issue for most of the indirect estimates of this cross section Timofeyuk et al. (2006); Summers and Nunes (2008b); Esbensen (2009); Rupak et al. (2012); Capel and Nollet (2017). Therefore, either there is some new physics not considered in the single-particle descriptions used in these references and in the present study, or there is some systematic uncertainty, which has not been well accounted for in the analysis of the experiment. The cross section we derive from our Halo-EFT description of 15C at the single astrophysical energy keV is b, which is slightly lower than what other groups obtain Reifarth et al. (2008); Timofeyuk (2014); Summers and Nunes (2008a).
Within our study, this is the only one oddity in the analysis of various reaction observables, which are all peripheral, and in particular with Coulomb-breakup cross sections, which are sensitive to the same nuclear-structure observables as the radiative capture, viz. the ANC of the g.s. of 15C and the phaseshift in the 14C- waves Capel and Nollet (2017). We therefore believe that they are well constrained within our model of 15C. The E1 strength this model predicts, and upon which both the Coulomb-breakup and the radiative-capture cross sections depend, should thus be quite reliable. Figure 9 provides this as a function of the relative energy between the 14C and the neutron in the continuum. The value we obtain from our NLO 14C- potentials are compared with the E1 strength inferred from the Coulomb-breakup measurement by Nakamura et al. Nakamura et al. (2009). We observe that the latter is systematically lower than the deduced from our Halo-EFT model of 15C, even though we are in perfect agreement with their Coulomb-breakup cross sections (see Fig. 7). This difference is due to higher-order effects, which are neglected in the analysis of the RIKEN data. As already shown in Refs. Summers and Nunes (2008a); Esbensen (2009); Capel and Nollet (2017), these effects are significant and cannot be ignored in the reaction model. This is the reason why the RIKEN prediction of the cross section for the radiative capture 14C(,)15C underestimates the direct measurement or Reifarth et al. (see Fig. 3 of Ref. Nakamura et al. (2009)). A comparison with that observable within the ab initio model of Navrátil et al. would be interesting to confirm our prediction.
VI Summary and outlook
The exotic nucleus 15C raises interests in various fields. It exhibits a one-neutron halo Tanihata (1996); Riisager (2013), and its synthesis through the radiative capture of a neutron by 14C takes place in various astrophysical sites Wiescher et al. (1999); Kajino et al. (1990); Terasawa et al. (2001). It is therefore interesting to better understand its structure and to provide astrophysicists with reliable cross sections for the radiative capture at low energies.
In this work, we have reanalyzed various reactions involving 15C using one single description of that nucleus. Following the work initiated in LABEL:CPH18, we have considered a Halo-EFT description of that one-neutron halo nucleus. Once coupled to a precise model of reactions, this very systematic expansion enables us to accurately determine the observables that affect the reaction process and hence, which can be probed through experimental measurements Capel et al. (2018); Yang and Capel (2018); Moschini and Capel (2019).
Using a LO Halo-EFT Hamiltonian (5), we have reanalyzed the transfer data at low energy Mukhamedzhanov et al. (2011) within the framework of the FR-ADWA Johnson and Tandy (1974). Following the results of LABEL:yang-capel, focusing on the forward-angle region, enables us to select purely peripheral data, from which a reliable estimate of the ANC of the g.s. of 15C has been inferred. The value obtained fm*-1/2* ( fm*-1*) is in good agreement with previous work Trache et al. (2002); Timofeyuk et al. (2006); Pang et al. (2007); Summers and Nunes (2008a, b); Mukhamedzhanov et al. (2011); McCleskey et al. (2014) and with preliminary ab initio predictions Navrátil (2018).
The ANC hence obtained coupled to the binding energy of the valence neutron to the 14C provides us with two nuclear-structure observables, upon which we have constrained a Halo-EFT Hamiltonian at NLO. This Hamiltonian has then be used within precise models of reactions to reanalyze transfer data Goss et al. (1975); Mukhamedzhanov et al. (2011), Coulomb-breakup cross sections measured at high Pramanik et al. (2003) and intermediate Nakamura et al. (2009) energies, and cross sections for the radiative capture Reifarth et al. (2008). In all cases, we observe a very good agreement with experiment without the need for any additional adjustment.
By showing that all these experiments can be described at the NLO of the Halo-EFT expansion, these analyses indicate that the core-neutron binding energy and the ground-state ANC are the sole nuclear-structure observables that need to be constrained to reproduce these data. These reactions are therefore purely peripheral, in the sense that they probe only the tail of the projectile wave function and not its interior. Especially, no need is found for a renormalisation of the projectile wave function, confirming that no spectroscopic factor can be extracted from such measurements Capel and Nunes (2007); Capel et al. (2018). Going beyond NLO, we have found that the presence of the bound excited state of 15C in its description has no effect in Coulomb-breakup calculations.
From this NLO description of 15C we have been able to infer a reliable estimate of the E1 strength from the \mbox{\frac{1}{2}}^{+} ground state of 15C to its 14C- continuum. This leads to excellent agreement with the measurements of both the 15C Coulomb breakup Pramanik et al. (2003); Nakamura et al. (2009) and the radiative capture Reifarth et al. (2008). Accordingly, we suggest as a cross section for the latter process at astrophysical energy the value b.
The excellent results obtained within this framework confirms the interest of coupling a Halo-EFT description of the nucleus to existing precise models of reactions Capel et al. (2018). They also drive us to extend this idea to other reactions, like knockout Hebborn and Capel (2019). Hopefully, the model developed herein and in LABEL:CPH18 will enable us to reproduce existing data on 15C and 11Be Tostevin et al. (2002); Sauvan et al. (2004); Fang et al. (2004). We also plan to apply this model to other halo nuclei, like 19C and 31Ne.
Acknowledgements.
This project has received funding from the European Union’s Horizon 2020 research and innovation programme under grant agreement No 654002, the Deutsche Forschungsgemeinschaft within the Collaborative Research Centers 1044 and 1245, and the PRISMA (Precision Physics, Fundamental Interactions and Structure of Matter) Cluster of Excellence. J. Y. is supported by the China Scholarship Council (CSC). P. C. acknowledges the support of the State of Rhineland-Palatinate.
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