# Extreme Ultraviolet Time- and Angle-Resolved Photoemission Spectroscopy with 21.5 meV Resolution using High-Order Harmonic Generation from a Turn-Key Yb:KGW Amplifier

## TL;DR

This paper presents a high-resolution time- and angle-resolved photoemission spectroscopy setup using high-order harmonic generation from a Yb:KGW laser, enabling detailed studies of quantum materials with 21.5 meV energy resolution.

## Contribution

The work introduces a robust, tunable repetition rate HHG-based photoemission system achieving 21.5 meV energy resolution without a monochromator, suitable for studying quantum materials.

## Key findings

- Achieved 21.5 meV energy resolution in photoemission.
- Demonstrated effective single-harmonic isolation at 21.8 eV.
- Measured electronic structures in topological materials.

## Abstract

Characterizing and controlling electronic properties of quantum materials require direct measurements of non-equilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for time- and angle-resolved photoemission spectroscopy using high-order harmonic probe pulses generated by a robust, moderately high power (20 W) Yb:KGW amplifier with tunable repetition rate between 50 and 150 kHz. By driving high-order harmonic generation (HHG) with the second harmonic of the fundamental 1025 nm laser pulses, we show that single-harmonic probe pulses at 21.8 eV photon energy can be effectively isolated without the use of a monochromator. The on-target photon flux can reach 5 x 10^10 photons/second at 50 kHz, and the time resolution is measured to be 320 fs. The relatively long pulse duration of the Yb-driven HHG source allows us to reach an excellent energy resolution of 21.5 meV, which is achieved by suppressing the space-charge broadening using a low photon flux of 1.5 x 10^8 photons/second at a higher repetition rate of 150 kHz. The capabilities of the setup are demonstrated through measurements in the topological semimetal ZrSiS and the topological insulator Sb2-xGdxTe3.