Bell correlations at Ising quantum critical points
Angelo Piga, Albert Aloy, Maciej Lewenstein, Ir\'en\'ee Fr\'erot

TL;DR
This paper demonstrates that Bell inequalities based on two-body correlations are violated near the quantum-critical point of the Ising model with power-law interactions, revealing non-local quantum behavior at criticality.
Contribution
It introduces a permutationally invariant Bell inequality applicable to the Ising model with power-law interactions and shows its violation at quantum critical points using analytical and numerical methods.
Findings
Bell inequality violation occurs near the quantum-critical point.
Maximum violation is observed for infinite-range interactions ($=0$).
Quantum-critical correlations lead to squeezing of collective-spin fluctuations.
Abstract
When a collection of distant observers share an entangled quantum state, the statistical correlations among their measurements may violate a many-body Bell inequality, demonstrating a non-local behavior. Focusing on the Ising model in a transverse-field with power-law () ferromagnetic interactions, we show that a permutationally invariant Bell inequality based on two-body correlations is violated in the vicinity of the quantum-critical point. This observation, obtained via analytical spin-wave calculations and numerical density-matrix renormalization group computations, is traced back to the squeezing of collective-spin fluctuations generated by quantum-critical correlations. We observe a maximal violation for infinite-range interactions (), namely when interactions and correlations are themselves permutationally invariant.
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Bell correlations at Ising quantum critical points
Angelo Piga
ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Av. Carl Friedrich Gauss 3, 08860 Barcelona, Spain
Albert Aloy
ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Av. Carl Friedrich Gauss 3, 08860 Barcelona, Spain
Maciej Lewenstein
ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Av. Carl Friedrich Gauss 3, 08860 Barcelona, Spain
ICREA-Institució Catalana de Recerca i Estudis Avançats, Lluis Companys 23, 08010 Barcelona, Spain
Irénée Frérot
ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, Av. Carl Friedrich Gauss 3, 08860 Barcelona, Spain
Abstract
When a collection of distant observers share an entangled quantum state, the statistical correlations among their measurements may violate a many-body Bell inequality, demonstrating a nonlocal behavior. Focusing on the Ising model in a transverse-field with power-law () ferromagnetic interactions, we show that a permutationally invariant Bell inequality based on two-body correlations is violated in the vicinity of the quantum-critical point. This observation, obtained via analytical spin-wave calculations and numerical density-matrix renormalization group computations, is traced back to the squeezing of collective-spin fluctuations generated by quantum-critical correlations. We observe a maximal violation for infinite-range interactions (), namely when interactions and correlations are themselves permutationally invariant.
Introduction. Nonlocal correlations, witnessed by the violation of Bell inequalities (BIs), mark the strongest departure from classical physics that correlated quantum systems may exhibit Brunner et al. (2014). To violate a BI, entanglement among the individual degrees of freedom is necessary (albeit not sufficient Werner (1989)). Such quantum correlations are typically fragile against thermalization, especially when considering many degrees of freedom. Nevertheless, thermalization is not always detrimental to entanglement: indeed, quantum critical points (QCPs) Sachdev (2011) represent a special instance of equilibrium states, where multipartite entanglement is stabilized at all length scales Hauke et al. (2016), a feature intrinsically robust at finite temperature in the quantum-critical regime Hauke et al. (2016); Gabbrielli et al. (2018); Frérot and Roscilde (2019). In addition to entanglement, are there QCPs which stabilize also nonlocal correlations among the individual components of the system? An important result from quantum information theory shows that all non-product pure states, including those at QCPs, possess bipartite nonlocal correlations Gisin (1991). Demonstrating and quantifying the presence of nonlocal correlations among a macroscopic number of degrees of freedom is, in general, a very challenging task Brunner et al. (2014). Nonetheless, a permutationally invariant Bell inequality (PIBI) involving only first and second moments of collective observables was derived recently Tura et al. (2014, 2015), which is especially revelant for a collection of qubits. The preparation, in a Bose-Einstein condensate (BEC), of massively entangled states of two-level atoms violating this inequality, was subsequently reported Schmied et al. (2016).
In the BEC experiment Schmied et al. (2016), violatation of the PIBI was achieved through the dynamical generation of spin-squeezed states Schmied et al. (2016); Pezzè et al. (2018). On the other hand, spin squeezing is known to be present at the QCP of the transverse-field ferromagnetic (FM) Ising model (TFIM), at least for a sufficiently large number of spatial dimensions Frérot and Roscilde (2018); Gabbrielli et al. (2018). Here, we investigate nonlocal correlations at the QCP of the TFIM with power-law decaying () interactions, interpolating between infinite-range () and nearest-neighbour () interactions. Besides its fundamental interest as a paradigmatic model for quantum phase transitions, this model has been implemented in various quantum simulators Bernien et al. (2017); Zhang et al. (2017); Chang et al. (2018). We first establish spin squeezing as a necessary condition to violate the PIBI derived in ref. Tura et al. (2014, 2015), in a Bell scenario involving identical measurement settings on all qubits. Based on numerical density-matrix renormalization group (DMRG) and analytical linear spin-wave (LSW) computations, we show that spin squeezing is a generic feature close to the QCP, leading to a maximal violation for in the thermodynamic limit. Interestingly, the violation of the PIBI is maximal for all-to-all interactions, where the semi-classical spin-wave theory is exact. Bipartite entanglement entropy (EE), on the other hand, shows the opposite behavior, being maximal for nearest-neighbour interactions.
Bell inequality violation and spin squeezing. We consider a -qubits quantum state, and a Bell scenario in which every qubit can be projectively measured along two possible directions and . We aim at certifying the nonlocal nature of the resulting correlations, relying on 1- and 2-body expectation values. More specifically, we consider BIs involving symmetric combinations of such correlators, namely and with , where , and the vector of Pauli matrices. In Tura et al. (2014), the following BI was established
[TABLE]
which must be fulfilled by any statistical model obeying Bell locality hypothesis. Given a quantum state, we look for optimal measurement directions in order to maximally violate inequality (1). This optimization can be performed analytically. First, introducing , defining the collective spin , and using elementary spin algebra, Eq. (1) can be recast in the equivalent form Schmied et al. (2016)
[TABLE]
where and are the first and second moments of the collective spin along, respectively, directions and , scaled to the coherent spin state values.
Notice that measuring the collective spin projectively along and does not realize a Bell scenario, but witnesses the ability to prepare many-spin states exhibiting nonlocality if the spins are individually measured along and Schmied et al. (2016). Indeed, Eqs. (1) and (2) have a different status. On the one hand, Eq. (1) allows for a device-independent test of nonlocality, valid even if individual measurement axes are not well-controlled, and even if the individual systems are actually not qubits but have an arbitrary physical structure. The only assumption leading to Eq. (1) – beyond Bell locality hypothesis – is that two possible measurement settings can be freely chosen on each party, each of which yielding two possible outcomes Tura et al. (2014, 2015). On the other hand, Eq. (2) relies on extra physical assumptions: applicability of quantum-mechanical spin algebra and correct calibration of measurement axes Schmied et al. (2016).
We define as the mean spin direction: . If , then , precluding violation of Eq. (2) for large . Hence, axis must be chosen perpendicular to . Then, the minimal value of is obtained if is along the direction of minimal variance of . Violation of inequality (2) then requires (namely, spin squeezing Kitagawa and Ueda (1993); Pezzè et al. (2018)), while maintaining the largest possible spin length (). Then, we choose , yielding . The minimal is
[TABLE]
achieved for . The second measurement direction is . Maximal violation of inequality (2) is achieved for perfect squeezed states ( and ), possible only for .
Ferromagnetic Ising model. We investigate violation of Eqs. (1) and (2) at the QCP of the TFIM, with power-law FM interactions:
[TABLE]
where , and are spin operators. and run over the sites of a dimensional square lattice of size , and denotes the position of spin . We introduced , and, to have a well-defined thermodynamic limit also for , we normalized the interaction term to . Mean-field theory predicts a QCP for , separating paramagnetic (PM) (for ) from FM phases (). The exact QCP is in general at ; in the nearest-neigbour limit, Sachdev (2011). In the PM phase, spins are aligned along ; in the FM phase, they sponteneously align along , with in mean-field theory. At the QCP, fluctuations of the magnetization along diverge as a power-law with the system size, namely with a critical exponent . On the other hand, due to the presence of the transverse-field, the system maintains a finite magnetization along , so that . In virtue of Heisenberg inequality for the collective spin, this opens the possibility for squeezing the fluctuations of , as . While quantum-critical spin squeezing is indeed present when Dusuel and Vidal (2004); Frérot and Roscilde (2018), for nearest-neighbour interactions it is present for but absent in Liu et al. (2013); Frérot and Roscilde (2018). FM power-law interactions increase the connectivity of the Ising model, and can be viewed as effectively increasing the physical dimension of the system. Hence, we may expect spin squeezing, as well as the resulting violation of inequality (1), to exhibit a non-trivial behavior when varying the power-law exponent at the QCP. In particular, in , we may expect a violation for small values of , but not in the nearest-neighbour limit . This scenario is indeed confirmed by our numerical DMRG results 111 Our DMRG algorithm for long-range interactions follows Crosswhite et al. (2008); Fröwis et al. (2010). , consistently with LSW analytical predictions.
DMRG results in one dimension. On Fig. 1(a), we plot the maximal violation of the BI [Eq. (1)], as a function of the transverse-field and of . For values of , nonlocal correlations are detected in the vicinity of the QCP, with maximal violation for . For , no violation is detected, consistently with the quasi-absence of spin squeezing at the nearest-neighbour QCP Liu et al. (2013); Frérot and Roscilde (2018). Fig. 1(b) shows von Neumann half-chain EE. Regardless of , for , EE is maximal at the QCP. The quantum-critical origin of the BI violation is demonstrated on Fig. 1(b), as maximal EE and maximal violation of Eq. (1) occur for the same transverse-field in the thermodynamic limit. On Fig. 2, we plot, varying power-law exponent and system size , the maximal violation of Eq. (1) obtained at the finite-size precursor of the QCP (defined as the value of for which is minimal). For and , LSW theory (detailed below) predicts that . Due to strong finite-size effects, our extrapolation for does not exactly match this prediction (see inset of Fig. 2). However, increasing , we clearly see a weakening violation of Eq. (1), up to where no violation is detected any more.
In Aloy et al. (2019), it was proven that -producible states 222 A state is -producible if it is a mixture of tensor products of states involving at most spins Tóth (2012); Hyllus et al. (2012). The entanglement depth is the minimal value of such that is -producible. cannot violate the PIBI by more than a certain bound . Therefore, observing a violation exceeding certifies an entanglement depth of at least . Such bounds are indicated on Fig. 1(a, inset). In particular, a violation , as observed at the critical point for , certifies a diverging entanglement depth Aloy et al. (2019).
Linear spin-wave theory. Given that FM power-law interactions harden quantum fluctuations about the mean-field ground state, LSW theory is expected to give accurate predictions, especially for small . In fact, we show that LSW theory even becomes exact in the thermodynamic limit for . In the following, we choose FM order along . After Holstein-Primakoff (HP) mapping of spin operators to bosonic modes 333 HP mapping: ; ; . Expressions are valid up to ordrer . are bosonic operators which, in Fourier space, read: . , we obtain the LSW Hamiltonian:
[TABLE]
valid up to second order in HP operators. We introduced in the PM phase, and in the FM phase. In terms of HP operators at wave-vector , and are defined as and , such that , and . The LSW Hamiltonian of Eq. (5) is diagonalized by the Bogoliubov rotation , such that . Written as in Eq. (5), the physical meaning of LSW mapping is especially transparent. Indeed, the two quadratures and represent collective-spin fluctuations in the two directions transverse to the mean spin orientation, namely (in LSW approximation): and , with and . Within LSW theory, their fluctuations are simply harmonic, and sectors corresponding to different wave-vectors decouple from each other. Finally, Eq. (5) allows one to directly read the eigenfrequencies of collective-spin fluctuations, namely . Approaching the QCP at , becomes gapless, implying diverging fluctuations of the quadrature (and, correspondingly, squeezing of the quadrature). In terms of collective-spin degrees of freedom (), one indeed finds
[TABLE]
Divergence of order parameter fluctuations (here, ) is a generic signature of critical phase transitions (quantum or thermal). Squeezing of fluctuations transverse to the order parameter (namely of ), on the other hand, is a genuine signature of quantum criticality without a classical analog Frérot and Roscilde (2018). Here, it signals the presence of genuine multipartite entanglement at the QCP Pezzé and Smerzi (2009); Frérot and Roscilde (2018); Gabbrielli et al. (2018), yielding maximal violation of the multipartite BI Eq. (1). LSW theory predicts perfect squeezing of fluctuations at the QCP (), so that from Eq. (3), the minimal value of is simply
[TABLE]
At LSW level, BI violation at the QCP has thus a very transparent interpretation, involving solely the reduction of the mean spin length by quantum fluctuations.
LSW predictions are reliable as long as the mean spin length, , is moderately reduced by occupation of HP bosonic modes, namely . We find . For , for Frérot et al. (2017), so that , and . In other words, all quantum fluctuations apart from those of the collective spin are effectively frozen out. For any , we find : LSW theory is asymptotically exact at any finite detuning from the QCP. The situation is different for . On the one hand, away from the QCP, is gapped, so that is always finite. The only possible instance of (infrared) divergence is then at the QCP, where with dynamical exponent Frérot et al. (2017). The condition for infrared divergence of is then equivalent to the divergence of at low , i.e. to the condition , met only for () in , where logarithmic divergence occurs. Otherwise, converges for to a finite value, which must satisfy for LSW theory to be reliable 444 For , for at the QCP; for , : LSW is always reliable for . In , for at the QCP, but already for , indicating a strong effect of quantum fluctuations for large . We complement LSW by DMRG calculations in . .
Remarkably, for , in the thermodynamic limit, corresponding to the maximal possible violation of the considered BI Tura et al. (2014). This property is illustrated on Fig. 2 in , and on Fig. 3(a) in , where is plotted across the phase diagram. It may seem surprising that the limit of infinite-range interactions, leading to a complete suppression of quantum fluctuations at in the ground state, is identified as maximally nonlocal. Indeed, in contrast, as shown on Fig. 3(c), bipartite EE is strongly suppressed for , obeying at most a scaling for Latorre et al. (2005) instead of a (area-law) scaling. This feature should be understood as a specificity of the (permutationally invariant) BI we have considered, rather than an intrinsic property of the many-body state. In general, for all , we always find maximal violation of the PIBI at criticality, where bipartite EE is also maximal [Fig. 3(b)], demonstrating the quantum-critical origin of the correlations leading to non-locality detection. Finally, we notice that for , in contrast to , nonlocal correlations are detected at the QCP for any value of . This observation is consistent with the presence of spin-squeezing for nearest-neighbour interactions in Frérot and Roscilde (2018).
Discussion. We investigated the violation of a permutationally invariant Bell inequality (PIBI, Eq. (1)) induced by a quantum critical point (QCP). We identified spin squeezing – in a general sense – as a necessary ingredient to violate the PIBI when identical measurements are performed on a collection of qubits. Focusing on the ground state of the ferromagnetic TFIM, we showed that power-law decaying interactions favor the development of spin squeezing at the QCP, leading to a maximal violation of the PIBI in the limit of infinite-range interactions. Our results are relevant to various experimental platforms implementing the quantum Ising model with power-law interactions, like trapped ions Zhang et al. (2017), Rydberg atoms Bernien et al. (2017) and nano-photonic structures Chang et al. (2018). In particular, BI violation is expected to be robust against thermal noise Frérot and Roscilde (2018); Gabbrielli et al. (2018) and particle losses Tura et al. (2014).
Beyond the Ising model considered in this paper, we expect our results to hold for critical points corresponding to the spontaneous breaking an Ising symmetry – for any range of interactions in , and for sufficiently long-range power-law interactions in . Extending our study to higher-order symmetries [U(1), SU(2), etc.] is however a non-trivial task, which may require the derivation of novel BIs.
Being invariant under the permutation of any of the parties involved in the Bell scenario, the BI we have considered is especially suited to investigate nonlocal correlations in -body states themselves permutationally invariant. This absence of spatial structure was indeed realized in the BEC experiment, where atoms share one spatial mode, as well as in the ground-state of all-to-all interacting models. However, general quantum-critical states, like conventional many-body states, do usually have a non-trivial spatial structure. As the PIBI only depends on the two-body reduced density-matrix averaged over all pairs, the possibility to capture nonlocal features of QCPs is thus not obvious. The spatial structure of entanglement, on the other hand, is rather revealed through bipartite Schmidt decomposition, capturing entanglement at a many-body level. Developing further conceptual and technical tools to investigate nonlocal correlations in spatially structured many-body states is an important challenge for ongoing studies Wang et al. (2017).
Acknowledgements.
Acknowledgements. We thank T. Roscilde, J. Tura, M. Fadel and E. Tirrito for insightful discussions. We acknowledge the Spanish Ministry MINECO (National Plan 15 Grant: FISICATEAMO No. FIS2016-79508-P, SEVERO OCHOA No. SEV-2015-0522, FPI), European Social Fund, Fundació Cellex, Generalitat de Catalunya (AGAUR Grant No. 2017 SGR 1341 and CERCA Programme), ERC AdG OSYRIS and NOQIA, and the National Science Centre, Poland-Symfonia Grant No. 2016/20/W/ST4/00314. IF acknowledges the Fundació Cellex through a Cellex-ICFO-MPQ postdoctoral fellowship, the Spanish MINECO (QIBEQI FIS2016-80773-P, Severo Ochoa SEV-2015-0522), and the Generalitat de Catalunya (SGR 1381 and CERCA Programme)
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