Resolved Sideband Cooling of a Levitated Nanoparticle in the Presence of Laser Phase Noise
Nadine Meyer, Andres de los Rios Sommer, Pau Mestres, Jan Gieseler,, Vijay Jain, Lukas Novotny, Romain Quidant

TL;DR
This paper explores how laser phase noise impacts resolved sideband cooling of levitated nanoparticles, identifying phase noise as a key obstacle and proposing strategies to achieve motional ground state cooling.
Contribution
It investigates the role of laser phase noise in limiting cooling efficiency and suggests methods to overcome this obstacle for ground state cooling of levitated nanoparticles.
Findings
Achieved minimal temperatures of 10 mK limited by phase noise
Identified phase noise as the main obstacle in reaching motional ground state
Proposed strategies for ground state cooling despite phase noise
Abstract
We investigate the influence of laser phase noise heating on resolved sideband cooling in the context of cooling the center-of-mass motion of a levitated nanoparticle in a high-finesse cavity. Although phase noise heating is not a fundamental physical constraint, the regime where it becomes the main limitation in Levitodynamics has so far been unexplored and hence embodies from this point forward the main obstacle in reaching the motional ground state of levitated mesoscopic objects with resolved sideband cooling. We reach minimal center-of-mass temperatures comparable to mK at a pressure of mbar, solely limited by phase noise. Finally we present possible strategies towards motional ground state cooling in the presence of phase noise.
Peer Reviews
No public reviews on file for this paper yet. If you reviewed it on a platform where reviews are public (OpenReview, ICLR, NeurIPS, ICML), you can paste yours below so the community can read it here.
Videos
No videos yet. Explain this paper in a talk, walkthrough, or lecture? Add one.
Resolved-Sideband Cooling of a Levitated Nanoparticle in the
Presence of Laser Phase Noise
Nadine Meyer
ICFO Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain
Andrés de los Rios Sommer
ICFO Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain
Pau Mestres
ICFO Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain
Jan Gieseler
ICFO Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain
Vijay Jain
Photonics Laboratory, ETH Zürich, 8093 Züurich, Switzerland
Lukas Novotny
Photonics Laboratory, ETH Zürich, 8093 Züurich, Switzerland
Romain Quidant
ICFO Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology, 08860 Castelldefels (Barcelona), Spain
ICREA-Institució Catalana de Recerca i Estudis Avançats, 08010 Barcelona, Spain
(March 9, 2024)
Abstract
We investigate the influence of laser phase noise heating on resolved sideband cooling in the context of cooling the center-of-mass motion of a levitated nanoparticle in a high-finesse cavity. Although phase noise heating is not a fundamental physical constraint, the regime where it becomes the main limitation in Levitodynamics has so far been unexplored and hence embodies from this point forward the main obstacle in reaching the motional ground state of levitated mesoscopic objects with resolved sideband cooling. We reach minimal center-of-mass temperatures comparable to mK at a pressure of mbar, solely limited by phase noise. Finally we present possible strategies towards motional ground state cooling in the presence of phase noise.
Optomechanics, Levitodynamics, phase noise heating
pacs:
Valid PACS appear here
Among the numerous optomechanical systems, Levitodynamical systems excel with an extreme level of isolation from the environment, rendering Q-factors exceeding Gieseler et al. (2013). This makes them an attractive alternative to membranes and nanobeams Tsaturyan et al. (2014); Reinhardt et al. (2016); Norte et al. (2016); Ghadimi et al. (2018) for probing macroscopic quantum phenomena at room temperature Marshall et al. (2003); Kleckner et al. (2008); Romero-Isart et al. (2010, 2011). In addition, Levitodynamics offers unique possibilities unavailable in conventional clamped systems, including free fall Hebestreit et al. (2018a), rotation Arita et al. (2013); Kuhn et al. (2017); Monteiro et al. (2018); Reimann et al. (2018) and engineered potentials Rondin et al. (2017). These unique features make them ideal candidates for enhanced sensing applications Hempston et al. (2017), out of equilibrium thermodynamics Gieseler and Millen (2018) and matter wave interferometry Bateman et al. (2014); Wan et al. (2016).
Thus far, the motional ground state (GS) of levitated nanoparticles remains elusive. The lowest phonon occupation of tens of phonons, has been achieved with continuous measurement and active feedback cooling Gieseler et al. (2012); Jain et al. (2016); Tebbenjohanns et al. (2019); Conangla et al. (2019); Li et al. (2011). In contrast to these active schemes, passive optomechanical cooling provides a way to cool to the GS without continuous measurement, provided that the cavity linewidth is narrower than the mechanical frequency. This so-called sideband cooling technique was originally developed for atomic systems and in combination with cryongenics it has been used for GS cooling () in a range of optomechanical systems.
First Levitodynamics experiments demonstrated 1D sideband cooling Kiesel et al. (2013); Asenbaum et al. (2013); Millen et al. (2015) from room temperature down to 0.3K Fonseca et al. (2016). Here we demonstrate 1D resolved sideband cooling of a levitated nanoparticle reaching temperatures of at a pressure of mbar, a regime where we will show that phase noise heating is indeed the limiting factor. The phonon occupation of the mechanical oscillator yields , an occupation less than in previous experiments Fonseca et al. (2016) and comparable to minimal temperatures reached in coherent scattering Vuletić et al. (2001); Gonzalez-Ballestero et al. (2019); Windey et al. (2019); Delić et al. (2019). Next to the well-known decoherence due to thermal noise and photon recoil Jain et al. (2016), we investigate in detail the influence of frequency noise of the cavity field, also called phase noise, on the phonon occupation. Phase noise decoherence has so far been largely overlooked in Levitodynamics Delić et al. (2019) despite being previously observed in other platforms Schliesser et al. (2008); Safavi-Naeini et al. (2013) where it seriously complicates the creation of low phonon states Rabl et al. (2009); Diósi (2008).
Understanding the limitations of sideband cooling techniques with actively driven cavities is essential for many protocols to generate entanglement Riedinger et al. (2018); Hong et al. (2017), non-classical correlations Riedinger et al. (2016) or achieve coherent quantum control Verhagen et al. (2012). Controlling the mechanical motion of mesoscopic systems on the single phonon quantum level has been achieved only recently Chan et al. (2011); Teufel et al. (2011).
By using an external cavity, the center-of-mass (COM) motion of an atom, ion, molecule Vuletić and Chu (2000); Leibrandt et al. (2009), or mesoscopic particle can be controlled and therefore cooled. The presence of a polarizable object inside the cavity induces a position-dependent dispersive change in optical path length, altering the intracavity intensity which then acts back on the particle motion. Coherently driving the cavity with a red(blue) detuned light field enhances(reduces) anti-Stokes scattering versus Stokes scattering, thus cooling(heating) the COM motion.
The interaction Hamiltonian for a particle moving along the axis of an optical cavity is Aspelmeyer et al. (2014); Kiesel et al. (2013) where () is the photon annihilation (creation) operator and () is the phonon annihilation (creation) operator. The single photon optomechanical coupling strength can be enhanced by the driving field as , being the intracavity photon number. The single photon optomechanical coupling strength is sinusoidally modulated due to the intracavity standing wave and given as
[TABLE]
where is the resonance frequency shift induced by a particle placed at the center of an empty cavity, with , being the cavity resonance frequency, the polarizability of the particle with radius nm and refractive index . The cavity volume is , cm the cavity length, m the cavity waist, the cavity field wave vector, nm the cavity wavelength and the position of the particle from the center along the cavity axis. The particle mass is inferred from the particle density , and the particle mechanical frequency is obtained from the particle displacement power spectral density (PSD). The optomechanical damping rate is then given by Aspelmeyer et al. (2014)
[TABLE]
with the cavity linewidth kHz (FWHM). The optomechanical damping rate depends strongly on position along the cavity axis through , the intracavity photon number and detuning from the cavity resonance . In the resolved sideband regime () the maximum cooling rate equals at optimal red detuning , enabling an optomechanical damping rate in the kHz-regime in state-of-the-art cavities.
In addition to the coupling rate to the thermal bath , shot noise radiation pressure heating (SNRP) due to the cavity field () and the trapping field () are additional decoherence sources (see Eq.(6) - (8)). As shown in section C, the additional phonon occupation due to the SNRP of the cavity light field () does not depend on the intra-cavity photon number, while the SNRP of the trapping light field acts as an additional thermal bath. The latter causes only a small relative offset and will therefore be negelected in the following. Moreover, heating effects due to classical laser intensity noise show a much smaller heating effect Jain compared to SNRP and will therefore also be neglected.
In the regime where the thermal mechanical damping is the main decoherence source, the final phonon occupation of the mechanical oscillator is
[TABLE]
where is the initial thermal phonon occupation. We neglect the contribution from the thermal photon occupation of the undriven cavity, since for optical frequencies. puts an ultimate limit on the minimum phonon number for . As a consequence the GS can only be reached in the resolved sideband regime () where . The COM temperature is then (solid lines in Fig.2 - 4).
In Fig. 1 the experimental setup is displayed. A silica nanoparticle is levitated in an optical tweezers trap Mestres et al. (2015) with a wavelength , power and focusing lens . The trap is mounted on a 3D piezo system allowing for precise 3D positioning of the particle inside the high finesse Fabry-Pérot cavity with a cavity finesse and free spectral range FSR = GHz (for more details see supplementary A). Due to tight focusing, the nanoparticle eigenfrequencies are non-degenerate. The maximum single photon optomechanical coupling strength is , which puts GS cooling seemingly into reach by simply increasing the intracavity photon number to , corresponding to a feasible intracavity power of W.
In our experiments we vary the cavity input power , the detuning and the position along the cavity axis in low and high vacuum, respectively. In the following, points represent data and solid lines are theoretical predictions according to eq.(2). The intracavity photon number, used for theoretical predictions, is calculated from the transmitted cavity power. At low pressure, we apply parametric feedback cooling (PFC) along , preventing particle loss and limiting the particle displacement to the linear regime of the optical trap. Experimentally we deduce from the area of the particle displacement PSD equal to Hebestreit et al. (2018b), as shown in Fig.2(a).
Fig.2(b) shows the pressure dependence of at optimal detuning and intracavity power of . At pressures below 1mbar, we observe the expected linear decrease of . At , cooling becomes ineffective and the temperature levels off with a constant final minimum temperature of , in contrast to theoretical expectations (solid line).
Figs. 3 and 4 show measurements at high pressure (red ) and low pressure (blue ), respectively. In Fig.3 we investigate versus for various cavity input powers ranging from - at high pressure () and - at low pressure (). At high pressure (Fig.3(a-c)) features a clear minimum at . The experimental results agree well with the theory, and only for high cavity input powers of we observe a deviation. In contrast, at low pressure the data deviates from the theory and the optimal detuning is farther away from resonance as shown in Fig.3(e-g). Our minimum temperature is , corresponding to a minimal phonon number . The dependence of at a nominal optimal detuning versus cavity input power is summarized in Fig.3(d) and (h) for high and low pressure respectively. At high pressure decreases as expected with increasing power (solid line). This is in strong contrast to the low pressure regime, where measurements deviate from theoretical predictions, which yield a minimal temperature of K at maximum input power mW (Fig.3(h)).
In Fig.4 we probe versus particle position along the cavity axis . We step the optical tweezers trap in increments of over a total distance exceeding . The cavity detuning is kept at a constant optimal value of and at constant intracavity power W. At high pressure (Fig.4(a)) we observe a sinusoidal dependence of the temperature on position as expected from the optomechanical coupling strength (see Eq.(1)). While the minimum temperature of agrees well with the theory (solid line), the maximum temperature differs by a factor of 2 from the expected room temperature of . We attribute this to the particle motion at K, which is and thus a significant fraction of the intracavity standing wave .
In the low pressure regime the situation is quite different (Fig.4 (b-d)). Periodic behaviour is only observed for the lowest cooling powers . Once the intracavity power is increased to , starts losing its position dependence. The minimum temperature mK persists over a broad region and looses its position-dependence for .
Altogether, as long as the dominant heating source is thermal noise, our observations are consistent with theory (see Eq.(2)). Laser phase noise becomes significant below mbar preventing further cooling. The heating at low pressures cannot be explained by thermal heating (Fig.2) or by photon radiation pressure (see supplementary C).
Phase noise stems from a combination of cavity instability and phase noise of the driving laser. It translates into amplitude noise of the intracavity field. This has two effects on the system Rabl et al. (2009): First, the optomechanical coupling strength changes due to its dependence on the intracavity photon number . However, for a laser linewidth of the coupling strength varies as and hence the dependence on intracavity field variations is negligible. Second, the conversion of phase to amplitude fluctuations inside the cavity gives rise to a stochastic force driving the mechanical oscillator. This leads to an additional phonon occupation , which scales linearly with the intracavity photon number and the phase noise PSD at the mechanical frequency . Including phase noise, the total final phonon occupation is
[TABLE]
where the first two terms derive from Eq.(2) and the last term accounts for phase noise. Eq.(3) reproduces the data well (half-solid line), assuming the specified phase noise at 10kHz of . The shaded area covers a range of and to account for the 1/ decrease in phase noise at higher frequencies Numata et al. (2018) and additional phase noise contributions related to setup instabilities respectively. In general, phase noise heating increases near the cavity resonance due to high intracavity photon numbers (see Eq.(3)) and dominates at low pressure. This leads to a shift in optimal detuning towards and the opposite power dependence at high and low pressure. The trap SNRP is largely negligible (dotted line in Fig.3(e-h) and Eq.(5)). The optimum intracavity photon number depends on the phase noise level. Consequently, the minimum phonon occupation in presence of phase noise (see supplementary C) is
[TABLE]
The experimental minimum phonon occupation of , stands in good agreement with the theoretical prediction of , corresponding to mK and mK respectively.
In conclusion, we experimentally and theoretically investigated the influence of phase noise heating in resolved sideband cooling of a levitated nanoparticle in high vacuum where thermal heating is no longer the main limitation. Counter-intuitively, minimum temperatures are achieved at low intracavity power. Nevertheless, there are two approaches to continue towards GS cooling. Either the optomechanical coupling strength is increased by using a larger particle, a higher finesse or a smaller cavity volume Magrini et al. (2018), such that the cooling efficiency per photon improves. Alternatively the coupling to the environment has to be reduced by further lowering the pressure or the system’s phase noise (see Eq.(4)). Reducing the current phase noise of by a factor of 1500, GS cooling can be achieved with the experimental parameters given here. This condition can be relaxed by an additional factor of 100 for a larger particle of r = 250nm at a pressure of mbar. Note that, phase noise can be decreased with external filtering cavities acting as low pass filters Jayich et al. (2012); Safavi-Naeini et al. (2013). This reduces the phase noise by several orders of magnitude Hald and Ruseva (2005), opening up the road to GS cooling with levitated nanoparticles.
Acknowledgments. NM, ADLRS, PM, and RQ acknowledge financial support from the European Research Council through grant QnanoMECA (CoG - 64790), Fundació Privada Cellex, CERCA Programme / Generalitat de Catalunya, and the Spanish Ministry of Economy and Competitiveness through the Severo Ochoa Programme for Centres of Excellence in RD Grants No. SEV-2015-0522 and No. FIS2016-80293-R. This project has received funding from the European Union’s Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 713729. JG received funding from the European Union’s Marie Skłodowska-Curie program (SEQOO, H2020-MSCA-IF-2014, grant no. 655369) LN and VJ acknowledge support through the NCCR-QSIT program (Grant No. 51NF40-160591) by the Swiss National Science Foundation.
Appendix A Experiment
The experimental setup is displayed in Fig. 1. In order to control the detuning between the cavity resonance and the driving field , we drive the cavity with two laser fields originating from the same laser at . The first weak cavity field is used for locking the cavity via the Pound Drever Hall technique (PDH) on the TEM01 mode minimising additional heating effects through the photon recoil heating of the cavity lock field. The PDH errorsignal acts on the internal laser piezo and an external AOM. In order to prevent interference effects between light fields we cross polarize the lock and pump field and separate them in frequency space by one free spectral range (FSR) such that the total detuning between lock and pump field yields . The tunable EOM modulation is provided by a signal generator. The AOM is modulated at a constant frequency. The intracavity power can be deduced from the transmitted cooling light observed on a photo diode (PD) behind the cavity.
For additional control of the other two motional degrees of freedom () we apply standard parametric feedback cooling Gieseler et al. (2012) by modulating the trapping potential with a phase locked loop (PLL) at twice the particle mechanical frequencies via an AOM. This maintains the particle motion in the and direction in the linear regime, avoiding mechanical cross coupling with the mode, while keeping the particle trapped at high vacuum.
All particle information shown is gained in forward detection interfering the scattered light field with the trap reference beam. The highly divergent trap light is recollected with a collection lens (). We use three balanced in-loop detectors (IL) to monitor the oscillation of the particle in all three degrees of freedom and generate the feedback signal for the PFC Gieseler et al. (2012). Additionally an out-of-loop detector (OoL) in the -direction solely records data, avoiding noise squashing Conangla et al. (2019); Tebbenjohanns et al. (2019) and therefore an underestimation of the particle energy. The pressure can be varied between atmospheric pressure and mbar.
Appendix B Data acquisition and evaluation
The data time traces are acquired at 1MHz acquisition rate with a home-built balanced detector and calibrated at mbar. Each data point consists of N = 10 averages of which each one consists again of at least 100 averaged position PSDs of which each is based on individual 2ms time trace, corresponding to a total minimum measurement time of sec. In the region of interest of ROI = 10-20kHz the averaged PSD is summed up and the corresponding temperature where is the Boltzmann constant. The error bars are the standard deviation of the N averages.
Appendix C Phonon occupation
The oscillator mean phonon occupation is governed by its environment. It is coupled to several baths as e.g. the thermal environment, the photon bath of trap and cavity field and the cavity frequency noise leading to decoherence effects. Each of the baths has an individual occupation state and coupling rate to the resonator. The steady state phonon occupation can be expressed as the following:
[TABLE]
where the we only consider the case of a cooled oscillator with . In Eq.(5) the terms from left to right describe the residual phonon occupation due to 1) the quantum back action of the resolved sideband cooling , 2) the thermal bath , 3) the shot noise radiation pressure of the cavity light field , 4) the phase noise of the cavity light field and 5) the shot noise radiation pressure of the optical tweezers light field .
In the resolved sideband regime () we assume a maximum optomechanical coupling rate at the optimal detuning () Aspelmeyer et al. (2014). The coupling rate are given in the following.
The thermal bath couples as
[TABLE]
where is the mechanical quality factor, the thermal occupation number, the particle radius, the gas pressure and the velocity of the residual gas molecules.
The phase noise of the driving field is coupled as
[TABLE]
where is the PSD of the phase noise at the mechanical frequency and the cavity line width (FWHM).
The radiation pressure shot noise from the cavity and trap are coupled to the particle as
[TABLE]
From Eq.(5) to 9 we can see that on one hand and are independent from the intracavity photon number and will be neglected for the remainder of the manuscript. On the other hand and decrease and increase linearly with . only causes an small offset. Hence there exists an optimal intracavity photon number where the minimum phonon occupation is reached. This stands in contrast to the standard picture of sideband cooling where the phonon occupation monotonically decreases with the number of intracavity photons .
The optimal intracavity photon number where we reach the lowest phonon occupation is given as
[TABLE]
[TABLE]
where . The thermal environment and optical trap together can be interpreted as a thermal bath with a higher effective temperature and therefore higher phonon occupation . The additional phonon contribution due to the trap light only needs to be taken into account at the lowest . The lowest phonon occupation is reached when the phonons are equally distributed between the effective thermal bath and the phase noise heating ().
[TABLE]
In case of neglecting the trap radiation pressure (), the minimum reachable phonon occupation deviates by and yields . The theoretically predicted optimal intracavity power is 0mW which is in reasonable agreement with the experimental value of -mW (see Fig.4(b-c)).
The reference list from the paper itself. Each links out to its DOI / PubMed record.
- 1Gieseler et al. (2013) J. Gieseler, L. Novotny, and R. Quidant, Nature Physics 9 , 806 (2013) . · doi ↗
- 2Tsaturyan et al. (2014) Y. Tsaturyan, A. Barg, A. Simonsen, L. G. Villanueva, S. Schmid, A. Schliesser, and E. S. Polzik, Optics Express 22 , 6 (2014) .
- 3Reinhardt et al. (2016) C. Reinhardt, T. Müller, A. Bourassa, and J. C. Sankey, Physical Review X 6 , 021001 (2016) .
- 4Norte et al. (2016) R. A. Norte, J. P. Moura, and S. Gröblacher, Physical Review Letters 116 , 147202 (2016) .
- 5Ghadimi et al. (2018) A. H. Ghadimi, S. A. Fedorov, N. J. Engelsen, M. J. Bereyhi, R. Schilling, D. J. Wilson, and . T. J. Kippenberg, Science 360 , 764 (2018) .
- 6Marshall et al. (2003) W. Marshall, C. Simon, R. Penrose, and D. Bouwmeester, Physcal Review Letters 91 , 13 (2003) .
- 7Kleckner et al. (2008) D. Kleckner, I. Pikovski, E. Jeffrey, L. Ament, E. Eliel, J. van den Brink, and D. Bouwmeester, New Journal of Physics 10 , 095020 (2008) .
- 8Romero-Isart et al. (2010) O. Romero-Isart, M. L. Juan, R. Quidant, and J. I. Cirac, New Journal of Physics 12 , 033015 (2010) .
