# Tunable Isolated Attosecond X-ray Pulses with Gigawatt Peak Power from a   Free-Electron Laser

**Authors:** Joseph Duris, Siqi Li, Taran Driver, Elio G. Champenois, James P., MacArthur, Alberto A. Lutman, Zhen Zhang, Philipp Rosenberger, Jeff W., Aldrich, Ryan Coffee, Giacomo Coslovich, Franz-Josef Decker, James M., Glownia, Gregor Hartmann, Wolfram Helml, Andrei Kamalov, Jonas Knurr, Jacek, Krzywinski, Ming-Fu Lin, Megan Nantel, Adi Natan, Jordan O'Neal, Niranjan, Shivaram, Peter Walter, Anna Wang, James J. Welch, Thomas J. A. Wolf, Joseph, Z. Xu, Matthias F. Kling, Philip~H.~Bucksbaum, Alexander Zholents, Zhirong, Huang, James P. Cryan, Agostino Marinelli

arXiv: 1906.10649 · 2020-01-08

## TL;DR

This paper reports the creation of high-power, isolated soft X-ray attosecond pulses using a free-electron laser, enabling advanced studies of ultrafast electron dynamics with unprecedented intensity and spectral specificity.

## Contribution

It introduces a method to generate GW-scale, isolated soft X-ray attosecond pulses with significantly higher energy and power than previous sources.

## Key findings

- Generated soft X-ray attosecond pulses with gigawatt peak power.
- Pulse energy is six orders of magnitude larger than previous sources.
- Enables new ultrafast electron dynamics investigations.

## Abstract

The quantum mechanical motion of electrons in molecules and solids occurs on the sub-femtosecond timescale. Consequently, the study of ultrafast electronic phenomena requires the generation of laser pulses shorter than 1 fs and of sufficient intensity to interact with their target with high probability. Probing these dynamics with atomic-site specificity requires the extension of sub-femtosecond pulses to the soft X-ray spectral region. Here we report the generation of isolated GW-scale soft X-ray attosecond pulses with an X-ray free-electron laser. Our source has a pulse energy that is six orders of magnitude larger than any other source of isolated attosecond pulses in the soft X-ray spectral region, with a peak power in the tens of gigawatts. This unique combination of high intensity, high photon energy and short pulse duration enables the investigation of electron dynamics with X-ray non-linear spectroscopy and single-particle imaging.

## Full text

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## Figures

21 figures with captions in the complete paper: https://tomesphere.com/paper/1906.10649/full.md

## References

64 references — full list in the complete paper: https://tomesphere.com/paper/1906.10649/full.md

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Source: https://tomesphere.com/paper/1906.10649