Effective viscosity of a polydispersed suspension
Matthieu Hillairet (IMAG), Di Wu

TL;DR
This paper derives the first order correction to the effective viscosity of a suspension with arbitrarily shaped particles, using homogenization and an extended reflection method, applicable even as particle number increases.
Contribution
It introduces a novel homogenization approach and extends the method of reflections to handle suspensions with many particles of arbitrary shapes, providing convergence results.
Findings
Derived the first order correction to effective viscosity.
Extended the method of reflections for multiple particles.
Proved convergence for small volume fractions regardless of particle count.
Abstract
We compute the first order correction of the effective viscosity for a suspension containing solid particles with arbitrary shapes. We rewrite the computation as an homogenization problem for the Stokes equations in a perforated domain. Then, we extend the method of reflections to approximate the solution to the Stokes problem with a fixed number of particles. By obtaining sharp estimates, we are able to prove that this method converges for small volume fraction of the solid phase whatever the number of particles. This allows to address the limit when the number of particles diverges while their radius tends to 0. We obtain a system of PDEs similar to the Stokes system with a supplementary term in the viscosity proportional to the volume fraction of the solid phase in the mixture.
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Effective viscosity of a polydispersed suspension
Matthieu Hillairet
Institut Montpelliérain Alexander Grothendieck, CNRS, Univ. Montpellier, France
and
Di Wu
School of Mathematical Sciences, Peking University, Beijing 100871, P.R. China.
Abstract.
We compute the first order correction of the effective viscosity for a suspension containing solid particles with arbitrary shapes. We rewrite the computation as an homogenization problem for the Stokes equations in a perforated domain. Then, we extend the method of reflections [11, 16] to approximate the solution to the Stokes problem with a fixed number of particles. By obtaining sharp estimates, we are able to prove that this method converges for small volume fraction of the solid phase whatever the number of particles. This allows to address the limit when the number of particles diverges while their radius tends to We obtain a system of PDEs similar to the Stokes system with a supplementary term in the viscosity proportional to the volume fraction of the solid phase in the mixture.
1. Introduction
When a viscous fluid transports solid particles, the particles modify in return the properties of the fluid. For instance, the rheological properties of the fluid are altered. In his seminal paper [5], Einstein addresses the computation of the effective viscosity of the mixture, having in mind it could help recovering the size of the transported particles. He obtains then the formula:
[TABLE]
Here stands for the (bulk) viscosity of the incompressible fluid alone, denotes the viscosity of the mixture and stands for the volume fraction of the solid suspension of spheres. Einstein formula has been the subject of numerous studies: analysis of Einstein ”formal” computations [1, 14, 2, 9], computation of second order expansion [10, 4, 7]. We refer the reader also to [13] for a comprehensive picture on the possible phenomena influencing the effective viscosity of a suspension. Most of these studies consider homogeneous suspensions. However, as mentioned in [13], a formula for the effective viscosity depending only on the volume fraction is hopeless to describe general suspensions, the factor in the above formula being in particular valid for a suspension of spheres a priori. In this paper, we provide a method for the computation of an effective viscosity allowing a distribution of shapes for the particles in the suspension.
A second motivation of the paper is to obtain a ”local” formula for the effective viscosity similar to [1, 16]. To be more precise, we rephrase now the computation of an effective viscosity, as depicted in [3], into a homogenization problem. We consider an incompressible newtonian fluid occupying the whole space and transporting a cloud made of particles. We neglect the particle and fluid inertia so that computing an effective viscosity amounts to understand the behavior of the system when it is submitted to a strain flow (where is a symmetric trace-free matrix). This reduces to the following stationary problem. We denote by the fluid velocity-field/pressure. The domain of the -th solid particle is the smooth bounded open set and its center of mass is The motion of is associated to a pair of translational/rotational velocities . Introducing the viscosity of the fluid, the unknowns are computed by solving the problem
[TABLE]
In this system, we introduced the fluid stress-tensor Under the assumption that the fluid is newtonian, it reads:
[TABLE]
The zero source terms on the right-hand side of the first equation in (2) and both equations of (4) are reminiscent of the intertialess assumption. The second equation of (3) must be understood as
[TABLE]
In the last equations (4) the symbol stands for the normal to By convention, we assume that it points inwards the solid and outwards the fluid domain that we denote in what follows:
[TABLE]
Under the assumption that the do not overlap, existence/uniqueness of a solution to (2)-(3)-(4) falls into the scope of the classical theory for the Stokes equations (see [6, Section V]). We give a little more details in the next section. We only mention here that the pressure is unique up to a constant. But, this has no impact on our computations and we consider the pressure as being uniquely defined below (this problem could be fixed by assuming that one mean of the pressure has a fixed value). Our aim is to tackle the asymptotics of this solution when the are small and many. To make this statement quantitative, we introduce further assumptions regarding the . Namely, we assume that there exists a diameter centers and shapes (meaning smooth bounded connected open sets of ) such that
[TABLE]
Then, we prescribe that the solid domains remain in a compact set and that there is no-overlap between the particles:
[TABLE]
With these conventions, we note that the total volume of the solid phase is at most so that, globally, in the volume the volume fraction of the solid phase is controlled by However, the separation assumption (H2) implies that we have also a uniform local control of the solid phase volume fraction by We use also constantly below that, with (H1)-(H2), we obtain
In order to derive an effective viscosity for the mixture, the classical point of view proposed in [5, 3] is to compute the rate of work of the viscous stress tensor on the boundary of the domain containing the solid particles:
[TABLE]
and to compare the excess with respect to the value that would yield in case there is no particle. In brief, the analysis of Einstein – in the case the are spheres of radius filling a bounded domain – relies on splitting the solution into Here is the pure strain applied on the boundaries at infinity:
[TABLE]
(this is a solution to the Stokes equations on since is trace-free) while the term compensates the trace of the boundary conditions on the that cannot be matched by a suitable pair in (3). Namely, one may write:
[TABLE]
Since is symmetric the latter linear term in the boundary condition cannot be compensated by a rigid rotation. Under the assumption that the holes are well-separated one provides the approximation:
[TABLE]
where is the solution to the Stokes problem (2) outside with boundary condition on (and vanishing boundary conditions at infinity). With this formula at-hand, one obtains that
[TABLE]
Via conservation arguments related to the divergence form of the Stokes equation, the boundary integrals involved in can be transformed into integrals over the boundaries of It is then possible to apply the explicit value of the solution Summing the contributions of all the particles leads finally to the first order expansion:
[TABLE]
leading to formula (1). We refer the reader to [3, p.246] for more details on this computation.
Herein, we show that solutions to (2)-(3)-(4) are close to solutions to the continuous analogue:
[TABLE]
Here the symbol stands for with an application that maps to the matrix . This linear mapping measures the collective reaction of the particles to the strain induced by We emphasize that we allow this mapping to depend on the space variable To be more precise, we explain now the computation of For arbitrary let denote by the unique solution to
[TABLE]
In this system, we have but we drop the index of the symbol for legibility. We note that are also unknowns in this problem. But they are the lagrange multipliers of the constraint (8), so that we may retain only as the solution. We associate to this solution:
[TABLE]
where stands for the orthogonal projection (w.r.t. matrix contraction) on the space of symmetric trace-free matrices . As shown in Section 2 below the matrix encodes the far-field decay of the solution in the sense that:
[TABLE]
at infinity (where contains vector-fields build up from the Green-function for the Stokes problem). Due to the linearity of the Stokes equations, we have that, for fixed the mapping is linear and thus given by a mapping (such a mapping can be identified with a matrix). We set then:
[TABLE]
We shall obtain below – under assumption (H1)-(H2)– that independent of the shape The mapping-function has then support in with so that it is bounded independent of Then, one can think as a possible weak limit if the parameter was tending to .
For instance, in the case are spheres of radius (so that is a sphere of radius ) comparing the expansion (9) with the explicit solutions to the Stokes problem (see [8, p. 39]) we obtain that so that
[TABLE]
In this case, the convergence of reduces to the convergence of the distribution of centers If the empirical measures associated to the distribution of centers converges to some we obtain, with the volume fraction of particles :
[TABLE]
We give herein a quantitative result with explicit stability bounds for the distance between solutions to the perforated problem (2)-(3)-(4) and to the continuous problem (5)-(6). We restrict below to functions in classes
[TABLE]
Here is a given parameter related to the volume fraction We identify the space of linear mappings with With the notations introduced before, a precise statement of our main result is the following theorem
Theorem 1.1**.**
Let (H1)-(H2) be in force and denote by the unique solution to (2)-(3)-(4). Let and denote by the unique solution to (5)-(6).
Under the assumption that is sufficiently small and that for arbitary there exists a constant depending only on for which:
[TABLE]
where
Several comments are in order. First, In (11), the norm on the right-hand side must be understood componentwise. Second, in the particular case of spheres, we can compute via (10) so that, we obtain a fully rigorous justification of the system:
[TABLE]
that has been obtained previously in [16, 1]. Finally, the restriction on exponent is reminiscent of the singularity of solutions to (7), corresponding to the gradient of the Green function for the Stokes problem on i.e. like . This singularity allows an -space for in dimension 3. In particular, this restriction can be removed when measuring the distance between and outside the particle domain (see [16] in the case of spheres).
As in the original proof of Einstein, Theorem 1.1 relies on two main properties. First, each particle in the cloud behaves as if it was alone in the strain flow Second, there is an underlying additivity principle which implies that the action of the cloud of particles on the fluid is the sum of the undividual actions of the different particles. In the two next sections, we justify the first of these two properties by extending Einstein computations to general suspensions. Broadly, a first guess for a solution to (2)-(3)-(4) could be
[TABLE]
This yields a solution to (2) and (4) which does not fulfill the boundary conditions (3) on So, we apply the linearity of the Stokes problem and introduce a first corrector:
[TABLE]
Again the candidate is a solution to (2) and (4) but does not match boundary conditions (3). So, we proceed with compensating again the non rigid part of the velocity-field on the boundaries This starts a process known as the ”method of reflections”. It has been studied in other contexts in [11, 15, 12] and extended to the problem of effective viscosity for a suspension of spheres in [16]. Herein, we modify a bit the method by correcting only the first order term in the expansion of the boundary values of on
[TABLE]
This enables to rely on the semi-explicit solutions to (7) and relate the final computations with the associated However, this does not rule out the key-difficulty of the process. Indeed, the method of reflections leads to the iterative formula:
[TABLE]
with a kernel wich decays generically like A priori, the above iterative formula entails then the bound:
[TABLE]
which yields that must be small w.r.t. for the method to converge (see assumption (2.3) in [16]). We remove this difficulty herein by showing that there exists a Calderòn-Zygmund operator underlying the above recursive formula. This enables to rule out the limitation on with respect to the number of particles. These computations are explained in the two next sections. Section 2 is devoted to the analysis of the problem (7)-(8). The Section 3 builds up on this analysis to study the convergence of the method of reflections and compute error estimates between the sequence of approximated solutions and the exact solution to (2)-(3)-(4).
The two last sections are devoted to the proof of the additivity principle and to complete the proof of Theorem 1.1. Once the method of reflections is proved to converge, we have an expansion of the solution to (2)-(3)-(4) in terms of the parameter We prove that there exits an equivalent expansion of the solution to (5)-(6) w.r.t. so that there is a correspondance between the first terms in the expansions of both solutions. We emphasize that, as classical with the weak-formulation of the Stokes problem, one obtains estimates on the difference of velocity-fields Regularity properties of the Stokes problem entail then similar properties for the pressures.
Through the paper, we use the following conventions. In the space of matrices we denote by the set of symmetric matrices and its subspace containing only the trace-free ones. We denote the orthogonal projection from onto with respect to the matrix contraction.
Concerning function spaces, we use classical notations for Lebesgue and Sobolev spaces. We also introduce the Beppo-Levi space and its divergence-free variant:
[TABLE]
In the whole paper, we denote and the fundamental solution to the Stokes equation in the whole space , which can be written
[TABLE]
for We collect in the vector
We also introduce the Bogovskii operator defined for arbitrary mean-free . It is well-known that this is continuous with values in and characterized by in . In particular, we denote for any .
2. Analysis of the Stokes problem
In the whole section, we suppose that has smooth boundaries Given a trace-free let consider the following problem:
[TABLE]
It is classical that, given alternatively a matrix and there exists a unique solution (with ) and (with ) to (14) in . The mapping
[TABLE]
is then linear and symmetric positive definite. In particular, there exists a unique solution to the problem:
[TABLE]
The candidate is then a solution to (14)-(15). By difference and integration by parts, we obtain uniqueness of a velocity-field solution which enables to recover that the pressure is unique up to a constant also. Since matches a velocity-field of the form on it is classical to extend by the field corresponding to this boundary value on yielding a vector-field Straightforward integration by parts arguments show that this extended realizes:
[TABLE]
In particular, we note that the set on which the minimum is computed on the right-hand side increases when decreases. Since we assume in this section, we infer a uniform bound for by the minimum reached for This yields that
[TABLE]
(and thus also) with a constant uniform in
One may proceed similarly to show that, under the assumption (H1)-(H2), the problem (2)-(3)-(4) admits a unique solution such that
[TABLE]
Furthermore, the velocity-field of this solution can be extended to the whole to yield a vector-field that realizes:
[TABLE]
In particular, under assumptions (H1)-(H2) we can construct an extension on of the field that matches on each of the (and thus on ) by truncating and lifting the divergence terms. Straightforward computations show that we have then:
[TABLE]
so that there exists a uniform constant for which:
[TABLE]
Before going to the main result of this section, we prepare the proof with a control on momenta of the trace of
[TABLE]
on This is the content of the following preliminary lemma:
Lemma 2.1**.**
There exists an absolute constant such that:
[TABLE]
We recall that stands for the orthogonal projection from onto With this lemma, we obtain that the linear mappings
[TABLE]
are uniformly bounded whatever
Proof.
Because of the linearity of the Stokes equations and of the stress tensor, the mapping from to :
[TABLE]
is also linear. So, let an orthonormal basis of , and the corresponding velocity-fields solution to the Stokes problem (14)-(15). Then, the mapping is represented in this basis by the matrix :
[TABLE]
Our proof reduces to obtaining that for arbitrary in So, let fix by integrating by parts, we have that
[TABLE]
so that:
[TABLE]
where we applied (16) to obtain the last inequality. This concludes the proof. ∎
We continue the analysis of (14)-(15) by providing pointwise estimates on . The content of the following theorem is reminiscent of [6, Section V.3]:
Proposition 2.2**.**
Let be the unique solution to (14)-(15). There exists a vector field depending on and , such that for any ,
[TABLE]
where for with:
[TABLE]
Moreover, there exists a constant independent of for which:
[TABLE]
Before giving a proof of this proposition, we note that for large , we have:
[TABLE]
Consequently the splitting that we obtain in the above proposition corresponds to the extraction of the leading order term () at infinity. A second crucial remark induced by this proposition is that the amplitude of both terms (the leading term and remainder ) do not depend asymptotically on the shape
Proof.
Let such that in and in . We recall that stands for the Bogovskii operator lifting the divergence on the annulus .
By standard ellipticity arguments are on Let define
[TABLE]
Up to a mollifying argument that we skip for conciseness, we may assume that The pair satisfies then the Stokes equation on with source term where:
[TABLE]
Since and we have uniqueness of -solutions to the Stokes equations on we may use the Green function to compute . This entails that, for each we have:
[TABLE]
In particular, for and (where coincides with ), a Taylor expansion yields:
[TABLE]
Concerning , we notice that
[TABLE]
Hence . To analyse , we denote:
[TABLE]
and
[TABLE]
First, for arbitrary skew-symmetric matrix , there holds:
[TABLE]
On the right-hand side, we have, since is symmetric and is skew-symmetric:
[TABLE]
We also notice that
[TABLE]
To obtain the last equality, we use that since is skew-symmetric, there is a vector such that and:
[TABLE]
Therefore we obtain that . Consequently, we have
[TABLE]
Since is symmetric, we deduce that:
[TABLE]
So, we set and we turn to show (19) and . To this end, we notice that is completely fixed by its action on matrices So, let fix We have
[TABLE]
Applying that again, we obtain
[TABLE]
Since is trace-free, the last pressure term vanishes. We rewrite the first term on the right-hand side:
[TABLE]
This entails that:
[TABLE]
We recall that pressure term do vanish since is trace-free. Concerning the first integral on the right-hand side, we notice again that:
[TABLE]
We are then in position to apply Lemma 2.1 which yields that
[TABLE]
for an absolute constant We proceed with the second integral. We notice that for any and on . Hence
[TABLE]
where we applied that to obtain the last identity. Gathering the previous computations we obtain that, for arbitrary , there holds:
[TABLE]
This concludes the proof of (19). Recalling that , and applying the explicit computation of the last integral in this latter identity, we obtain also
To finish the proof, we handle the last term for . We prove the required estimate for the extension to arbitrary being obvious. Given , and , we can find with such that:
[TABLE]
Asymptotic properties of entail then that Therefore, we have, thanks to the uniform bound (16) and the embedding
[TABLE]
This ends the proof of the proposition. ∎
We end this section by having a look to the interactions between the decomposition in Proposition 2.2 with scaling properties of the Stokes problem (14)-(15). Indeed, for any , standard scaling arguments imply that:
[TABLE]
Consequently for arbitrary we have:
[TABLE]
This entails that and
[TABLE]
We can then compare remainder terms. This yields:
[TABLE]
3. Approximation of the solution to the -particle problem
In this section, we fix large and We provide an approximation via the method of reflections for the solution to
[TABLE]
We recall that the method of reflections consists in matching the boundary conditions on each particle by solving a Stokes system around each particle, gluing together the local solutions into one approximation and iterating the process, since by gluing the local solutions we alter the boundary values of the approximation. More precisely, we first define
[TABLE]
Given and assuming that a vector-field and matrices are constructed we set:
[TABLE]
Correspondingly, we compute a sequence of approximate pressure:
[TABLE]
The factor is introduced here since solves a Stokes system without viscosity.
The motivation of these definitions is the following remark. For each the flow cancels the first order symmetric term of the leading part of the boundary value of on each . For instance, for , we notice that on , it holds:
[TABLE]
which implies that:
[TABLE]
Since is very small, meaning that , by Proposition 2.2 and (21), we have that for each and any :
[TABLE]
where since on On the other hand, by Taylor expansion, for any and any ,
[TABLE]
Hence in the reflection method, we aim at canceling the symmetric gradient . By a direct iteration, we obtain that, for any and there holds:
[TABLE]
The purpose of this section is twofold. First, we show that the method of reflections converges. We quantify then how close the family of approximations are to the velocity-field solution to (23)-(24)-(25).
We start with the convergence of the method. Since the correctors are fixed with respect to the family of matrices this amounts to prove that this family of matrices defines a converging series (in for arbitrary ). This is the content of the following proposition which relies mostly on item (1) of Lemma A.2 in Appendix A:
Proposition 3.1**.**
There exists sufficiently small such that, for and , there exists a constant depending on and , but independent of , such that
[TABLE]
Proof.
Let We first notice that, by Proposition 2.2, there exists symmetric matrices such that
[TABLE]
We remark then that, for , is homogeneous in with degree . Moreover satisfies that
[TABLE]
where for each , is harmonic in . We can apply then Lemma A.2 to the computation of the components of by choosing and for each This yields that, for sufficiently small and arbitrary
[TABLE]
However, by Proposition 2.2, there exists an absolute constant (independent of and other parameters) such that This completes the proof of the proposition. ∎
We proceed with the analysis of the quality of the sequence of approximations .
Proposition 3.2**.**
Let sufficiently small. There exists a constant , such that for and there holds
[TABLE]
Proof.
By substracting the equations satisfied by and we obtain that satisfies:
[TABLE]
and
[TABLE]
As for boundary conditions, we note that by definition of , we have that
[TABLE]
Thanks to (17) and extending the velocities and inside the particle domains with their boundary values, we have that On the boundaries, reorganizing the terms involved in see also (29), we have that there exists vectors for which:
[TABLE]
where we have with:
[TABLE]
and
[TABLE]
We notice that for each , the formula defining can be extended to . We also mention that again classical integration by parts arguments yield that realizes
[TABLE]
The proof of our theorem then reduces to construct divergence-free vector-fields that match (up to a rigid vector-field) on for each . Indeed, since is divergence-free and using the minimizing principle of (33), we have then:
[TABLE]
So, we define:
[TABLE]
Here, we denoted such that on and in , is the mean-value of over . Clearly, our candidate matches the condition
[TABLE]
For the next computations, we introduce also and the mean-values of and over respectively so that .
By the scaling properties of the Bogovskii operator, we obtain that
[TABLE]
where
[TABLE]
and
[TABLE]
Here, it is standard that the Poincaré-Wirtinger inequality entails that and . Hence, we only need to bound and .
We deal with first. According to the definition of and (see Proposition 2.2), for each , we have
[TABLE]
As in the proof of Proposition 3.1, for each , is homogeneous in with degree such that
[TABLE]
where for each , is harmonic in . By the definition of and applying Lemma A.2 by choosing and for each and Proposition 3.1, we have
[TABLE]
Up to restrict the size of we obtain that:
[TABLE]
Now we turn to deal with . By the definition of , we have that for any ,
[TABLE]
We notice here – since the minimum distance between two ’s is lager than which is much larger than (for small ) – that, for each and for any , there holds:
[TABLE]
where
[TABLE]
Therefore we obtain, with a direct Young inequality for convolution:
[TABLE]
which combined with Proposition 3.1, yields that:
[TABLE]
where we have chosen sufficiently small so that the series converges. Combining (34)-(35), we obtain the expected result. ∎
4. Approximation of the target system
In this section, we fix and (for some small ) and we analyse the properties of the asymptotic problem
[TABLE]
We note that is a gain a simple factor in this equation so that we only treat the case below. This system is associated with the weak formulation:
Find such that:
[TABLE]
Since has compact support, for sufficiently small we have that so that construction of a weak solution falls into the scope of the Lax-Milgram theorem. Hence, under the assumption that is sufficiently small we have existence and uniqueness of a satisfying
- •
- •
there exists for which (36) holds true (in ),
and consequently, the pressure exists and is unique up to a constant. We focus now – as in the previous section for the problem in a perforated domain – on a possible expansion of the solution in terms of ”powers of ”. Namely, for small the matrix can be seen as a perturbation of the identity so that one may look for a solution to (36)-(37) by iterating the mapping solving the system:
[TABLE]
starting form Again, it is standard by introducing a weak formulation and Lax-Milgram arguments that there exists a unique velocity-field satisfying
- •
- •
there exists a pressure such that
[TABLE]
The main result of this section is the following proposition which compares the velocity-field with
Proposition 4.1**.**
Under the assumption that is sufficiently small, there exists a constant such that
[TABLE]
Proof.
This proof is a straightforward application of fixed-point arguments. First, let prove that the mapping is a contraction on Indeed, for arbitrary given the weak formulation for the Stokes problem, we have that satisfies:
[TABLE]
Setting and recalling that is divergence-free we obtain that
[TABLE]
Consequently, fix Then and the mapping is a contraction that admits a unique fixed point. This yields a solution to (36)-(37). Furthermore, this solution is obtained by iterating the mapping from So the sequence converges to (in ) while, by definition, Similar energy estimates yield that
[TABLE]
Standard arguments with contractions then yield that
[TABLE]
This concludes the proof. ∎
5. Proof of main result
We end the paper with a proof of Theorem 1.1. In the whole section, we assume that we are given a perforated domain such that (H1)-(H2) hold true. We are also given with simultaneously (see (H1)-(H2) for the definitions of and ). Restrictions on are introduced throughout the section. Finally, we fix a matrix
We recall that Theorem 1.1 is a stability estimate between the solutions to two problems. The first one is the Stokes problem in a perforated domain (2)-(3)-(4) that we studied in Section 3. We restrict at first so that Proposition 3.2 holds true. We have then a sequence of approximations to the velocity-field solution to (2)-(3)-(4). The second problem is the continuous analogue (5)-(6) that we studied in Section 4. We assume also that is sufficiently small so that Proposition 4.1 holds true. We have then an approximation to the velocity-field solution to (5)-(6).
The purpose of Theorem 1.1 is to compute a bound from above for To this end, we fix and (with the notations of Proposition 3.2) and write
[TABLE]
The two error terms and have been estimated previously in Proposition 3.2 and Proposition 4.1 respectively. So, we proceed in the next subsection with estimating and shall combine the various partial results in the last subsection to complete the proof of our theorem.
5.1. Computing
We recall that is constructed via the method of reflections:
[TABLE]
By the definition of and Proposition 2.2, we have the following decomposition, for any
[TABLE]
where
[TABLE]
and
[TABLE]
We start with computing
Proposition 5.1**.**
Let and there exists for which:
[TABLE]
where
Proof.
By Proposition 2.2, we know that each component of can be written as:
[TABLE]
In this identity, we recall that given by (19), and that with
[TABLE]
corresponding to the fundamental solution of Stokes equation in . According to the fact that for any
[TABLE]
with and applying Lemma A.1, we obtain that for any and , for any
[TABLE]
We proceed by remarking that:
[TABLE]
Furthermore, since is harmonic on for and there holds:
[TABLE]
On the other hand, by uniqueness of the solution to the Stokes problem defining (in ), we know that is computed with Green’s function for the Stokes problem. This yield componentwise:
[TABLE]
We note that this quantity is well-defined since has compact support and is homogeneous of degree so that it is for arbitrary Eventually, the th component of can be rewritten as
[TABLE]
since Concerning the first term on the right-hand side of this equality, let denote any component of By assumption, we have then so that it can be written , where and are and
[TABLE]
Therefore, we have on
[TABLE]
where, by Calderón Zygmund inequality, the right-hand side of this identity is well defined and satisfies.
[TABLE]
As for the second term in we can apply a classical Young inequality for convolution to obtain:
[TABLE]
Finally, applying the embedding we have:
[TABLE]
We conclude by applying again that so that
[TABLE]
∎
We proceed by computing error estimates for This is the content of the following proposition:
Proposition 5.2**.**
Let and there exists for which:
[TABLE]
where
Proof.
We recall that
[TABLE]
Since by Proposition 2.2, we know that for any and , when
[TABLE]
Therefore, on , we have:
[TABLE]
Consequently, denoting we obtain
[TABLE]
where we applied Proposition 3.2 to pass from the second to the last line together with the remark that ∎
5.2. End of the proof
Let containing (for simplicity) and . By (40) we have
[TABLE]
Since and by the embedding and Proposition 3.2, we have the bounds
[TABLE]
With a similar chain of inequalities, we obtain by applying Proposition 4.1
[TABLE]
Finally, concerning , we recall that we have simultaneously (where we denote ) and with the notations of the previous subsection. This entails that:
[TABLE]
The two last terms of the right-hand side are controlled respectively by (42) and (46):
[TABLE]
where As for the first term, we first bound
[TABLE]
Here, it is straightforward from (39) that:
[TABLE]
As for we have, by Proposition 3.2 and uniform estimate (18) that:
[TABLE]
Via a straightforward bound on the volume of the we conclude that:
[TABLE]
Combining (47) and (48) yields
[TABLE]
since, as we have
Finally, we have proven:
[TABLE]
This concludes the proof.
Acknowledgement.
The authors would like to thank David Gérard-Varet for many fruitful discussions. The authors are partially supported by ANR Project IFSMACS ANR-15-CE40-0010. The first author is also supported by ANR Project SingFlow ANR-18-CE40-0027 and Labex Numev Convention grants ANR-10-LABX-20.
Appendix A Tools for the method of reflections
In this appendix, we give some technical tools that are involved in the method of reflections. We start with a representation formula generalizing the mean-value formula for harmonic functions.
Lemma A.1**.**
Suppose that . Let be a domain in and in . Then for arbitrary and such that we have:
[TABLE]
Proof.
This lemma must be part of the folklore. We give a proof for completeness. Let
[TABLE]
After differentiation and integration by parts, we obtain:
[TABLE]
Since when we infer that:
[TABLE]
Then, if we have:
[TABLE]
Integrating by parts and applying the formula we derived above for and , we obtain:
[TABLE]
This concludes the proof. ∎
Relying on this formula, we analyze the behavior of the recursive formula for the method of reflections (26). We recall that we consider here a set of centers of mass and parameters such that where We include the recursive formula in the following more general framework. We assume we are given homogeneous of degree and we suppose that where is harmonic in and homogeneous with degree . We look then at quantities of the form
[TABLE]
where are given and arbitrary and is a multi-index in The crucial result underlying the method of reflections is the following lemma:
Lemma A.2**.**
Let small and Then, there exists a constant such that the following properties hold true:
- (1)
if , then
[TABLE] 2. (2)
if and we denote on , there holds:
[TABLE]
Proof.
We split the proof into two parts corresponding to the two items in the lemma.
Part 1. This part is the proof of the first statement of the above lemma. By definition of we notice that in . Hence according to Lemma A.1 and the fact that is harmonic in , we obtain that
[TABLE]
where
[TABLE]
[TABLE]
and
[TABLE]
For the next computations, we introduce:
[TABLE]
and fix
Step 1. In this part we deal with . By definition, we have that
[TABLE]
In order to apply Calderón-Zygmund inequality, we split the above quantity into two parts: where
[TABLE]
We note that for any ,
[TABLE]
which implies that
[TABLE]
Therefore, we have:
[TABLE]
and
[TABLE]
On the other hand, by Calderón-Zygmund inequality we have:
[TABLE]
Hence we obtain that:
[TABLE]
Now we turn to deal with . At first, we notice that for any and , there holds:
[TABLE]
(where represents the symmetric difference between sets). Since is -homogeneous, this implies that for any , we have:
[TABLE]
We denote the right-hand side of this inequality. Again by Hölder inequality, we obtain that
[TABLE]
and
[TABLE]
On the other hand, by a standard Young inequality for convolution, we have
[TABLE]
Therefore we obtain that
[TABLE]
By combing (53) and (54), we obtain finally that,
[TABLE]
Step 2. Now we turn to handle . We recall that
[TABLE]
Since is harmonic outside , we have for each and ,
[TABLE]
which implies that
[TABLE]
We also notice that
[TABLE]
Therefore we obtain that
[TABLE]
By a similar argument as before, we obtain that
[TABLE]
which implies that, since :
[TABLE]
Step 3. At last we deal with . We recall that
[TABLE]
Again by the fact that is harmonic in for any , we obtain that for and :
[TABLE]
By a similar argument as in step 2, we obtain that
[TABLE]
and we conclude that:
[TABLE]
By combining (55), (56) and (57), we obtain the expected result since :
[TABLE]
The first statement of the lemma is proved.
Part 2. In this part we give a proof for the second item. By definition of and Lemma A.1, we have that for any
[TABLE]
According to the fact that is harmonic outside the origin, the second term on the right side of the above equation can be written as
[TABLE]
for any . Therefore for any , we have:
[TABLE]
where is defined in (52).
Now we start to prove (51). By the above argument and since the are disjoint, we have
[TABLE]
In order to control the right-hand side of the above inequality, we first notice that for each any and
[TABLE]
By similar arguments as in Part 1 of the proof, we obtain that
[TABLE]
and
[TABLE]
Therefore we have
[TABLE]
Now we turn to deal with the second term of the right side of (58). We first notice that for any and , there holds:
[TABLE]
Since we obtain via a standard Young inequality for convolutions that
[TABLE]
Finally, combining (58), (59) and (60) and remarking that , we have that
[TABLE]
This ends the proof of the second item and the proof of the lemma. ∎
The reference list from the paper itself. Each links out to its DOI / PubMed record.
- 1[1] Y. Almog and H. Brenner. Global homogenization of a dilute suspension of spheres.
- 2[2] H. Ammari, P. Garapon, H. Kang, and H. Lee. Effective viscosity properties of dilute suspensions of arbitrarily shaped particles. Asymptot. Anal. , 80(3-4):189–211, 2012.
- 3[3] G. Batchelor An introduction to fluid dynamics. Cambridge University Press, 1967.
- 4[4] G. Batchelor and J. Green. The determination of the bulk stress in a suspension of spherical particles at order c 2 superscript 𝑐 2 c^{2} . J. Fluid Mech. , 56:401–427, 1972.
- 5[5] A. Einstein. Eine neue bestimmung der moleküldimensionen. Ann. Physik. , 19:289–306, 1906.
- 6[6] G. P. Galdi. An introduction to the mathematical theory of the Navier-Stokes equations. Vol. I , volume 38 of Springer Tracts in Natural Philosophy . Springer-Verlag, New York, 2011. Linearized steady problems.
- 7[7] D. Gérard-Varet and M. Hillairet , Analysis of the viscosity of dilute suspensions beyond Einstein’s formula , Preprint.
- 8[8] E. Guazzelli and J. F. Morris , A Physical Introduction To Suspension Dynamics , Cambridge Texts In Applied Mathematics, 2012.
