Quantitative analysis of $p$-wave three-body losses via cascade process
Muhammad Waseem, Jun Yoshida, Taketo Saito, and Takashi Mukaiyama

TL;DR
This paper develops a rate equation model to analyze three-body losses in $p$-wave interacting fermions, explaining experimental results and extending to two-dimensional traps, revealing a proportionality to the scattering area.
Contribution
It introduces a theoretical rate equation model for $p$-wave three-body losses and verifies it experimentally in both 3D and 2D systems, including the weakly interacting regime.
Findings
The model explains experimental data above the universal scaling law.
In 2D traps, the loss coefficient scales with the cube of the scattering area.
The theoretical predictions match experimental results in both 3D and 2D configurations.
Abstract
We describe the three-body loss coefficient of identical fermions with -wave interactions using a set of rate equations in which three-body recombination happens via an indirect process. Our theoretical treatment explains experimental results just above the universal scaling law regime of weak interactions. Furthermore, we theoretically extend and experimentally verify the rate equation model for the case of atoms trapped in two dimensions. Moreover, we find that the three-body loss coefficient in a two-dimensional trap is proportional to in the weakly interacting regime, where is the scattering area. Our results are useful in understanding three-body physics with -wave interactions.
Peer Reviews
No public reviews on file for this paper yet. If you reviewed it on a platform where reviews are public (OpenReview, ICLR, NeurIPS, ICML), you can paste yours below so the community can read it here.
Videos
No videos yet. Explain this paper in a talk, walkthrough, or lecture? Add one.
Quantitative analysis of -wave three-body losses via cascade process
Muhammad Waseem1
Jun Yoshida2,3
Taketo Saito2,3
Takashi Mukaiyama4
1Karachi Institute of Power Engineering, Pakistan Institute of Engineering and Applied Sciences (PIEAS)
Islamabad, Karachi, 75780, Pakistan
2Department of Engineering Science, University of Electro-Communications, Tokyo 182-8585, Japan
3Institute for Laser Science,University of Electro-Communications, Chofugaoka, Chofu, Tokyo 182-8585, Japan
4Graduate School of Engineering Science, Osaka University, 1-3, Machikaneyama, Toyonaka, Osaka 560-8531 Japan
Abstract
We describe the three-body loss coefficient of identical fermions with -wave interactions using a set of rate equations in which three-body recombination happens via an indirect process. Our theoretical treatment explains experimental results just above the universal scaling law regime of weak interactions. Furthermore, we theoretically extend and experimentally verify the rate equation model for the case of atoms trapped in two dimensions. Moreover, we find that the three-body loss coefficient in a two-dimensional trap is proportional to in the weakly interacting regime, where is the scattering area. Our results are useful in understanding three-body physics with -wave interactions.
I introduction
Many-body quantum systems such as ultracold atoms offer great control and versatility due to Feshbach resonances, which allow accurate control of interatomic interactions via external magnetic fields. Such resonances occur when the kinetic energy of two colliding atoms in an open channel and the energy of bound-state atoms in the closed channel potential become degenerate. Higher partial wave interactions across these resonances, such as -wave Feshbach resonances, have specific features and signatures unlike their -wave counterparts vg ; cheng ; sukjin ; victor ; lev , for example, anisotropic phases of -wave condensates cheng ; lev and the possibility of observing different quantum phase transitions across -wave Feshbach resonances due to rich -wave order parameters vg ; victor ; lev . Some of these phase transitions across the -wave Feshbach resonances for fermions are similar to the phases of superfluid 3He lev11 .
The -wave Feshbach resonances in ultracold fermionic gases have been observed experimentally regal ; zhang . These -wave Feshbach resonances have been widely used to explore inelastic collision losses regal ; zhang ; ticknor ; chevy ; gun ; fed ; russian ; waseem2 ; yoshida ; waseem3 ; elk , the creation of -wave Feshbach molecules zhang ; gab ; inada ; waseem , the binding energies of -wave Feshbach molecules gab ; fuch , the determination of scattering parameters naka , and -wave contacts ueda1 ; thy ; yao ; lio . Following the advancement of -wave few-body physics, an impressive amount of theoretical effort was devoted to the case of identical Fermions near a -wave Feshbach resonance in three dimensions esry1 ; suno ; suno2 ; jona ; jesper ; jpd ; bratpra and in two dimensions lev ; nishida ; nishida12 ; nishida13 ; nishida14 ; nikolaj ; marish ; jpd2d ; zen1 ; zen2 ; maxim ; sjj ; hui ; petrov2 . On the experimental side, three-body loss coefficients as a function of interaction strength and temperature were measured in three-dimensional (3D) traps regal ; zhang ; yoshida ; waseem3 . The experiments conducted in Ref. yoshida successfully verified the temperature threshold behavior of at the low-temperature () limit and the scattering volume scaling law of three-body loss coefficients, , but only for relatively weak interactions. Since the first experimental study of spin-polarized interacting Fermi gases in two dimensions using a -wave Feshbach resonance gun , systematic studies of two-body spin relaxation losses waseem2 and the creation of the -wave Feshbach molecules in the angular momentum state have been performed waseem . A systematic understanding of three-body collision losses of identical fermions confined in a two-dimensional (2D) trap is also needed in experiments due to its importance in stability fed ; lev and few-body physics nishida ; nikolaj .
In this paper, we present a quantitative analysis to explain the three-body loss coefficient of identical fermions with -wave interactions using a set of rate equations describing three-body recombination as an indirect process. Our theoretical model explains the experimental results only above the universal scaling law regime of weak interactions and requires only a single parameter representing a collision rate coefficient between a free atom and quasiresonant molecules. For cross verification of the rate equation model, we extend it to the case of atoms trapped in two dimensions and again find good agreement with experimental data above the weak interaction regime. Furthermore, we found that the three-body loss coefficient in a 2D trap is proportional to in the weakly interacting regime, where is the scattering area.
This article is organized as follows. Section II describes our theoretical treatment for three-body recombination losses as an indirect process. In Sec. III, we compare our theoretical discussion with experimental results. In Sec. IV, we present our conclusions and outlook regarding this work.
II Theoretical Model
Three-dimensional theory: We consider the narrow Feshbach resonance that occurs in a -wave collision between the lowest-energy hyperfine state of 6Li atoms located at a magnetic field strength of 159.17(5) G. The two-body -wave interactions are described by an effective-range expansion of the -wave scattering phase shift as Taylor ; naidon
[TABLE]
where is a relative wave vector and is the effective range defined as positive. The scattering volume plays a role analogous to that of -wave scattering length and varies as a function of the external magnetic field as . Here, and are the background scattering volume and resonance width in the magnetic field, respectively idz . We used the values [] and from our previous measurement naka , where is the Bohr radius. The energy of the molecular state relative to the threshold varies as where is the mass of a 6Li atom and is the momentum of the resonant bound state parametrized by the scattering volume and the effective range russian . The relative kinetic energy becomes equal to the energy of the molecular state relative to the threshold at resonance, where is the thermal relative wave number. Near the threshold, the finite lifetime of the molecular state due to coupling to the continuum is described by the energy-dependent resonance width victor ; thy .
In order to describe three-body recombination near the narrow -wave Feshbach resonance, we treated the loss of trapped atoms as an indirect successive process. A -wave Feshbach resonance can be considered as a bound quasimolecular state weakly coupled to a continuum above the resonance victor . Therefore, the rate coefficient for the generation of quasimolecules via two-body collision at temperature above the narrow -wave Feshbach resonance is lee
[TABLE]
where . Then, the rate coefficient of vibrational quenching of a molecule, , occurs through collision of the molecule with a third atom. The rate equations describing the time evolution of atomic number density and the density of quasiresonant molecules in the resonance state are
[TABLE]
Here, instead of having a term, with being the three-body loss coefficient in the rate equation for atomic density as a three-body loss term, the three-body loss is taken into account as a successive process of dimer creation followed by an atom-dimer collision. Assuming a steady-state condition of molecular density (), one obtains
[TABLE]
Under the further condition of fast molecular creation, , we obtain a steady-state rate equation of the atomic density in the following form:
[TABLE]
Substituting Eq. (2) into Eq. (5), we write the three-body loss coefficient in the following form:
[TABLE]
We assume that molecular creation is sufficiently fast that the three-body loss coefficient is directly related to the atom-dimer collision coefficient .
Quasi-2D theory: Next, we apply a similar theoretical treatment to the case of atoms trapped in a quasi-two-dimensional geometry. In quasi-2D geometry, atoms are confined in the axial () direction with frequency , and the interatomic separations in the other two directions ( and ) greatly exceed the axial extension of the atomic wave function given by the harmonic oscillator length . In this case, the two-body -wave interactions are described by a two-dimensional effective range expansion of the scattering phase shift as cai ; prico ; russian
[TABLE]
where is a relative wave vector defined for the 2D case. The scattering area , defined as , was used as a controllable length scale parameter to tune the interaction via external magnetic field. depends upon both the harmonic oscillator length and the 3D scattering parameters russian . The positive dimensionless effective range in two dimensions is , which also depends on the 3D effective-range parameter and the harmonic oscillator length russian .
For the 2D case, the rate for the generation of quasimolecules via two-body collisions at temperature is written as
[TABLE]
Here, is the thermal momentum in quasi-2D geometry and is the momentum of the resonant bound state parametrized by the scattering area and the effective range russian . The two-dimensional resonance energy width is , which can be obtained from the pole of the -wave scattering amplitude in two dimensions marish . Similar to the 3D case, we assume a steady-state condition for the molecular density and a condition of . Here, we denote the rate constant of vibrational quenching of molecules due to atom-dimer collisions with and atomic density with . Then, the three-body loss rate coefficient can be obtained in the form
[TABLE]
which again describes the three-body loss rate coefficient as a function of magnetic field detuning and the atomic temperature in terms of the atom-dimer rate coefficient .
III Experiments
Three-dimensional case: We first trapped 6Li atoms in the hyperfine ground state of and using a single-beam optical dipole trap as described in detail elsewhere naka . In brief, we performed evaporative cooling at 300 G magnetic field where the elastic collision cross section is at its maximum after capturing the atoms with a single-beam optical dipole trap. To prepare a single-component Fermi gas, we eliminated the atoms in the state by shining the resonant light for a duration of 50 s. Then, we ramped the magnetic field close to the -wave Feshbach resonance for the state located at 159.17 G to investigate the loss features. Here, we reduced the fluctuation in the magnetic field to 8 mG by stabilizing the current in the Feshbach coils using a bypass circuit added in parallel to the coils naka . The resonance magnetic field was determined from the sharp edge of the atomic loss feature naka . The doublet structure arising from the resonance shift between different angular momentum projections and appears in a -wave Feshbach resonance due to dipole-dipole interactions between the two atoms in a -wave molecular state ticknor . We treated the -wave Feshbach resonance as a single resonance due to overlap of the and resonances in 6Li chevy .
Near the -wave Feshbach resonance, the density of atom decay due to three-body recombination losses is governed by the following rate equation:
[TABLE]
where, is the one-body loss rate. Assuming that the atomic density profile is Gaussian, integrating Eq. (10) results in a rate equation that describes the decay of the total number of atoms, ,
[TABLE]
where is the mean-square atomic density, which we determined from the atomic density profile obtained from the absorption image. Here, is the mean trapping frequency.
Figure 1 shows the three-body loss coefficient as a function of the magnetic field detuning at K and m*-3* (solid circles), K and m*-3* (solid triangles), and K and m*-3* (solid squares), respectively. The vertical bars indicate the magnetic field detuning values at which . The dashed curves in Fig. 1 show the results of Eq. (6), which agree with the experimental data to the left of the vertical bars. To the right of the vertical bars, where (or equivalently (), the measured three-body loss coefficients show a different trend from Eq. (6). Therefore, the direct three-body recombination process dominates over the indirect three-body loss coefficient at small scattering volumes. In this small scattering volume limit, when yoshida , the three-body loss coefficient follows the universal scaling law of
[TABLE]
as shown by the black solid curves with dimensionless constant yoshida on the right side of the vertical bars. The above scaling law was first predicted by Suno et al., suno , and was experimentally confirmed in our previous work yoshida . During fitting, we fit the data of Fig. 1 to Eq. (6) in the nonuniversal regime (left side of the vertical bars) and to Eq. (12) in the universal scaling regime (right side of the vertical bars) with and the critical magnetic field detuning as free parameters at each temperature independently. We obtained consistent values of from all data sets, which gave ms from the average of all fits. The values of at the kink location consistently correspond to . In our case, the ratio , which indicates that three-body losses are due to the two successive processes of pair creation and collision with a third atom above the universal scaling regime described by Eq. (12).
The quantity is the ratio of the second term to the first term in Eq. (1). Revamping Eq. (1) shotan under the condition of , gives
[TABLE]
Multiplying the above expression with effective range , using the definition , and considering (because generally the wave vector shows the temperature dependence russian ), we obtained a convenient form of the effective range expansion:
[TABLE]
Hence, includes the contribution of the effective range term in the collisional phase shift and quantifies the closeness of the dimer bound-state energy level to the average collision energy of two atoms. In the limit of small in the far-resonant regime, the strength of the three-body losses due to Eq. (6) falls exponentially and becomes negligible compared to the direct three-body recombination losses described by Eq. (12). As a result, the three-body losses due to the universal scaling of Eq. (12) increase, starting to dominate at in our case. Furthermore, the effect of the effective range that is included in Eq. (6) becomes irrelevant when , which is consistent with previous observations suno ; yoshida . Our current theoretical description of the three-body loss coefficient above the universal scaling regime converges to a single physical parameter instead of two unknown parameters and yoshida .
Quasi-2D case: We prepared a 2D Fermi gas by adiabatically shining an optical lattice potential using a laser with a beam waist of 65 m at 1064 nm, as described elsewhere waseem ; waseem2 . We calibrated the lattice depth from measured radial trap frequencies with and without the retroreflection beam. The motion of atoms along the lattice direction is restricted because the axial energy is always kept higher than the thermal energy , where is the confinement frequency along the lattice direction. To make sure that all the atoms are in the lowest motional state in the lattice potential, we performed the adiabatic band-mapping technique waseem ; kohl . We verified that the percentage of the population in the first excited motional state along the axis is less than 10 by taking into account both the size of the Brillouin zone and our imaging resolution miranda . In our experiment, the magnetic field is parallel to the optical lattice beams. Therefore, only the -wave Feshbach resonance for symmetry becomes active because all atoms are in the motional ground state along the quantization direction gun ; waseem ; tan .
To extract the three-body loss constant in the quasi-2D system, the time evolution of the number of atoms per site, , is fitted to the solution of the rate equation,
[TABLE]
where is the mean-square atomic density per site with 2D mean trap frequency miranda . We performed all measurements in a thermal regime so that we can safely assume the atomic density profile as a Gaussian along the loosely confined axes. Solid circles in Fig. 2 show as a function of magnetic field detuning at K, m*-2*, and with a lattice depth of ( kHz). Here, K is the recoil energy of the 6Li atom. Similarly, in Fig. 2, solid squares indicate values K, m*-2*, and with a lattice depth of ( kHz). The vertical bars indicate the values of the magnetic field detuning at which . In Fig. 2, the dashed curves on the left side of the vertical bar show the theoretical results obtained from Eq. (9) with ms, in agreement with experimental data. The ratios for Fig. 2(a) and for Fig. 2(b) again indicate that the observed three-body losses are mainly due to indirect two-step processes when .
In the region where , the experimental data deviate from the indirect process given by Eq. (9). Therefore, we expect some universal scaling of the three-body loss rate coefficient similar to the 3D case. In the far-resonant region, the temperature threshold law can be written as jpd2d . Here, is a quantum number associated with the dominated lowest three-body continuum channel in the low-energy limit for three identical fermions in two dimensions jpd2d . Therefore, using the dimensional analysis together with the temperature threshold law similar to the 3D case, we expect the following scaling law:
[TABLE]
In analogy with -wave interactions kra , the dimensionless constant may have additional scattering area dependence. The super Efimov effect nishida might be reflected in a universal double-exponential scaling behavior of . We did not observe recombination loss peaks arising from triatomic super Efimov resonances as predicted for three identical fermions in the state confined in two dimensions nishida . Therefore, we consider a dimensionless constant as long as the threshold law and scattering area scaling law hold.
In Fig. 2, the blue solid curves show the scaling of at fixed temperature using in Eq. (16). In our experiment, we were restricted to confirming the threshold law of in two dimensions at fixed because it was not possible to introduce controlled changes in temperature at a fixed lattice depth comment . Therefore, we followed the method of displaying all results in dimensionless units yoshida . We plot as a function of in Fig. 3 to clearly demonstrate the scaling of Eq. (16) and the range over which it applies. The entire data set along with additional data taken at 2.0, 3.4, 4.7, and K merge into a single monotonic curve. Below , the flat region of zero slope with an intercept of best revealed the expected scaling law of Eq. (16) as shown by the dotted horizontal line in Fig. 3. The long dashed curve in Fig. 3 is the combined result from Eqs. (16) and (9). The scaling of Eq. (16) holds over a relatively small range in the weakly interacting limit. In our experiment, the lower limit of Eq. (16) scaling is restricted to , mainly due to the non-negligible contribution of one-body decay. After the upper limit at , the loss coefficient steeply increased similar to the 3D case, and was well described by Eq. (9).
IV Conclusion
In conclusion, we have quantitatively analyzed the three-body loss coefficient as a function of temperature and magnetic field using a theoretical model based on a two-step loss process. The model nicely explains the loss behavior just above the weak interaction limit, where the universal scaling law is expected to hold. The model reproduces the experimental three-body loss coefficient results in both 3D and quasi-2D geometries with a single parameter, i.e., an atom-molecule collision rate coefficient. In the weak-interaction limit, the three-body loss coefficient is explained by the scaling law, meaning that the three-body loss is dominated by the direct transition from the three free-atom-state into a deeply bound dimer and one free atom. Slightly above the scaling-law regime, the three-body loss coefficient deviates from the scaling law but the behavior can be explained by the model presented here, indicating that the universal scaling law breaks down because the Feshbach dimer creation gets faster and the three-body loss can be considered a two-step process of a Feshbach dimer creation and an atom-dimer collision.
Our results provide useful initial grounds for extending the understanding of three-body physics in the presence of -wave Feshbach resonances. In our current theoretical description, the atom-molecule collision rate coefficient is the only parameter and is theoretically more difficult to predict. We assumed that the atom-molecule rate coefficient is independent of the magnetic field due to the nonresonant nature of the relaxation process. However, its precise dependence on atom-molecule collision energy or temperature would be expected to vary over a wide range of temperatures, from a very few to a few hundred microkelvins. Understanding the atom-molecule rate coefficients as a function of collision energy near the -wave Feshbach resonance in both 3D and 2D cases is needed to fully understand atomic losses near the Feshbach resonance, which prevents the realization of the -wave superfluid.
ACKNOWLEDGMENT
This work was supported by a Grant-in-Aid for Scientific Research on Innovative Areas (Grant No. 24105006) and a Grant-in-Aid for Challenging Exploratory Research (Grant No. 17K18752). M.W. acknowledges the support of a Japanese government scholarship (MEXT).
The reference list from the paper itself. Each links out to its DOI / PubMed record.
- 1(1) V. Gurarie, L. Radzihovsky, and A. V. Andreev, Phys. Rev. Lett. 94 , 230403 (2005) .
- 2(2) C. -H. Cheng and S. -K. Yip, Phys. Rev. Lett. 95 , 070404 (2005) .
- 3(3) S. Yoon and G. Watanabe Phys. Rev. Lett. 119 , 100401 (2017) .
- 4(4) V. Gurarie and L. Radzihovsky, Ann. Phys. 322 , 2 (2007) .
- 5(5) J. Levinsen, N. R. Cooper, and V. Gurarie, Phys. Rev. A. 78 , 063616 (2008) .
- 6(6) D. Vollhardt and P. Wolfe, The Superfluid Phases Of Helium 3 (Taylor and Francis Ltd, N.Y., 2002).
- 7(7) C. A. Regal, C. Ticknor, J. L. Bohn, and D. S. Jin Phys. Rev. Lett. 90 , 053201 (2003).
- 8(8) J. Zhang, E. G. M. van Kempen, T. Bourdel, L. Khaykovich, J. Cubizolles, F. Chevy, M. Teichmann, L. Tarruell, S. J. J. M. F. Kokkelmans, and C. Salomon, Phys. Rev. A 70 , 030702 (2004) .
