Magnetohydrodynamics in graphene: shear and Hall viscosities
B. N. Narozhny, M. Sch\"utt

TL;DR
This paper provides a comprehensive calculation of shear and Hall viscosities in graphene, revealing how these viscosities depend on doping levels and magnetic fields, with implications for understanding hydrodynamic electron flow.
Contribution
It introduces a unified kinetic theory and renormalization group approach to compute viscosities in graphene across various doping levels and magnetic fields.
Findings
Hall viscosity vanishes at charge neutrality.
Shear viscosity decreases with magnetic field and saturates at high fields.
Viscosity behavior aligns with semiclassical predictions away from neutrality.
Abstract
Viscous phenomena are the hallmark of the hydrodynamic flow exhibited by Dirac fermions in clean graphene at high enough temperatures. We report a quantitative calculation of the electronic shear and Hall viscosities in graphene based on the kinetic theory combined with the renormalization group providing a unified description at arbitrary doping levels and non-quantizing magnetic fields. At charge neutrality, the Hall viscosity vanishes, while the field-dependent shear viscosity decays from its zero-field value saturating to a nonzero value in classically strong fields. Away from charge neutrality, the field-dependent viscosity coefficients tend to agree with the semiclassical expectation.
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Magnetohydrodynamics in graphene: Shear and Hall viscosities
B. N. Narozhny
Institut für Theorie der kondensierten Materie, Karlsruhe Institute of Technology, 76128 Karlsruhe, Germany
National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), 115409 Moscow, Russia
M. Schütt
Condensed Matter Theory Group, Paul Scherrer Institute, 5232 Villigen PSI, Switzerland
Department of Theoretical Physics, University of Geneva, 1211 Geneva, Switzerland
Institute for Theoretical Physics, ETH Zurich, 8093 Zurich, Switzerland
Abstract
Viscous phenomena are the hallmark of the hydrodynamic flow exhibited by Dirac fermions in clean graphene at high enough temperatures. We report a quantitative calculation of the electronic shear and Hall viscosities in graphene based on the kinetic theory combined with the renormalization group providing a unified description at arbitrary doping levels and nonquantizing magnetic fields. At charge neutrality, the Hall viscosity vanishes, while the field-dependent shear viscosity decays from its zero-field value saturating to a nonzero value in classically strong fields. Away from charge neutrality, the field-dependent viscosity coefficients tend to agree with the semiclassical expectation.
Hydrodynamic behavior of charge carriers in graphene has been the focus of considerable experimental Checkelsky and Ong (2009); Zuev et al. (2009); Abanin et al. (2011); Bandurin et al. (2016); Crossno et al. (2016); Moll et al. (2016); Ghahari et al. (2016); Krishna Kumar et al. (2017); Bandurin et al. (2018); Braem et al. (2018); Jaoui et al. (2018); Ella et al. (2019); Gallagher et al. (2019); Berdyugin et al. (2019) and theoretical efforts Hartnoll et al. (2007); Kashuba (2008); Müller et al. (2008); Fritz et al. (2008); Müller and Sachdev (2008); Bhaseen et al. (2009); Foster and Aleiner (2009); Müller et al. (2009); Torre et al. (2015); Narozhny et al. (2015); Briskot et al. (2015); Levitov and Falkovich (2016); Principi et al. (2016); Lucas et al. (2016); Falkovich and Levitov (2017); Guo et al. (2017); Seo et al. (2017); Ledwith et al. (2017); Shytov et al. (2018); Ho et al. (2018); Link et al. (2018a); Kiselev and Schmalian (2019); Xie and Levchenko (2019); Burmistrov et al. (2019) (recently reviewed in Refs. Narozhny et al., 2017; Lucas and Fong, 2018). Within linear response, the difference between an Ohmic current and a hydrodynamic flow is determined by the viscosity Bandurin et al. (2016); Krishna Kumar et al. (2017); Berdyugin et al. (2019); Levitov and Falkovich (2016); Guo et al. (2017); Torre et al. (2015); Briskot et al. (2015) (see Refs. Bandurin et al., 2018; Ella et al., 2019 on the issue of ballistic electrons).
In traditional hydrodynamics Landau and Lifshitz (1959), viscosity is a measure of mutual friction between the neighboring fluid elements moving with distinct velocities. From the viewpoint of the microscopic theory, viscosity is a fourth-rank tensor that can be defined as a “response function” relating the stress (or momentum flux) to the strain Bradlyn et al. (2012); Link et al. (2018a). In isotropic systems Landau and Lifshitz (1959), the viscosity tensor contains two independent coefficients, the shear and bulk viscosities. The latter is only important for physical phenomena associated with fluid compressibility and is known to vanish for monoatomic gases Landau and Lifshitz (1959), ultrarelativistic systems Khalatnikov (1956); Lifshitz and Pitaevskii (1981), and Fermi liquids Abrikosov and Khalatnikov (1959). Similarly, it’s been argued to vanish in graphene Müller et al. (2009); Briskot et al. (2015); Principi et al. (2016), at least to the leading approximation. In anisotropic systems the situation is more involved Link et al. (2018b).
Treating the shear viscosity as a linear response function, one can derive a Kubo formula Principi et al. (2016); Bradlyn et al. (2012); Link et al. (2018a) that can be related to the Kubo formula for electrical conductivity Bradlyn et al. (2012). In practice, Kubo-formula based calculations are typically perturbative and one can only use this approach to evaluate the viscosity either in doped graphene (i.e., in the so-called “Fermi-liquid” or “degenerate” limit) Principi et al. (2016) or in the high-frequency collisionless regime Link et al. (2018a). At charge neutrality, one typically turns to the kinetic theory Kashuba (2008); Müller et al. (2009) combined with the renormalization group Sheehy and Schmalian (2007).
The relation between the Kubo formulas for shear viscosity and conductivity Bradlyn et al. (2012) leads to certain expectations regarding the dependence of the viscosity tensor on the external magnetic field. In the simplest case Alekseev (2016); Scaffidi et al. (2017); Steinberg (1958), one finds the field-dependent shear viscosity and the newly appearing Hall viscosity to mimic the magnetoconductivity and Hall conductivity in the usual Drude theory, respectively, with the only difference that the scattering time is now provided by electron-electron interactions.
An experimental measurement of the electronic shear viscosity is a nontrivial task Tomadin et al. (2014). Based on nonlocal resistance measurements Bandurin et al. (2016), a related quantity – the kinematic viscosity Landau and Lifshitz (1959) – was estimated to have a “higher-than-in-honey” value m2/s at typical charge densities, cm*-2*, and temperatures, K. This value is of the same order of magnitude as the theoretical expectation Principi et al. (2016) for doped graphene and agrees with more recent measurements Krishna Kumar et al. (2017); Berdyugin et al. (2019). In contrast, the theoretical result for the shear viscosity in neutral graphene Kashuba (2008); Müller et al. (2009); Briskot et al. (2015) has not been tested experimentally. Hall viscosity has been studied in a recent experiment reported in Ref. Berdyugin et al., 2019. Again, the measurements were performed away from charge neutrality, where the shear and Hall viscosities follow the semiclassical field dependence Alekseev (2016); Scaffidi et al. (2017); Pellegrino et al. (2017).
The purpose of the present paper is to provide a consistent, unified calculation of the shear and Hall viscosities in graphene at arbitrary doping levels within the “hydrodynamic” temperature window Narozhny et al. (2017) and at arbitrary nonquantizing magnetic fields. In a companion paper Narozhny (2019), we have generalized the nonlinear hydrodynamic equations derived in Ref. Briskot et al., 2015 to include the external magnetic field. Here we report a quantitative calculation of the kinetic coefficients on the basis of the kinetic theory combined with the renormalization group approach. At neutrality and in the degenerate regime, the results can be obtained in a closed analytical form. For arbitrary carrier densities, the viscosities can be expressed in terms of certain “scattering rates” to be evaluated numerically.
The results of our calculations are in good agreement with available experimental evidence. In the absence of the magnetic field, we find the kinematic viscosity to depend rather weakly on the carrier density, remaining of the order of m2/s for all densities explored in the experiment of Ref. Bandurin et al., 2016. The field-dependent shear and Hall viscosities away from charge neutrality are qualitatively similar to the semiclassical expectations Berdyugin et al. (2019), reaching the standard Drude-like dependence at the experimental densities, cm*-2*. In contrast, the shear viscosity at the neutrality point in classically strong magnetic fields saturates to a nonzero value. Our results are illustrated in physical units in Figs. 5 and 7.
I From the microscopic theory to hydrodynamics
We begin with a brief review of the hydrodynamic approach and a discussion of the applicability of hydrodynamics to Dirac fermions in graphene. The ideas presented here were developed in full detail in Refs. Lifshitz and Pitaevskii, 1981; Hartnoll et al., 2007; Briskot et al., 2015; Narozhny, 2019 (see the recent review Lucas and Fong (2018) for a more detailed discussion and a complete set of references) and are included here to make the paper self-contained.
Hydrodynamics is a macroscopic manifestation of conservation laws in an interacting many-body system that is a fluid. Typically Landau and Lifshitz (1959), one considers conservation of the particle number (or, equivalently either mass or electric charge), energy, and momentum. The latter provides the most stringent restrictions on the applicability of hydrodynamics limiting one to systems with the only (or the dominant) scattering mechanism being due to interparticle collisions (e.g., electron-electron interaction) that conserve momentum. At first glance this rules out scattering with other types of excitations (e.g., electron-phonon or electron-magnon scattering) as well as microscopically varying external potentials (e.g., potential disorder). In a typical solid, such processes dominate the linear-response transport properties and while they can be accounted for using the Boltzmann kinetic theory Lifshitz and Pitaevskii (1981), a fully hydrodynamic description is not possible.
In recent years, a number of materials have been developed Bandurin et al. (2016); Crossno et al. (2016); Moll et al. (2016); Braem et al. (2018); Jaoui et al. (2018) which are, on one hand, clean enough, such that disorder scattering is important only at the lowest temperatures and on the other hand rigid enough, such that the electron-phonon interaction is relevant at much higher temperartures. This provides for a considerable intermediate temperature range Briskot et al. (2015); Narozhny et al. (2017) where the electron-electron interaction is the dominant scattering mechanism in the system. Mathematically, the above can be summarized by the inequality,
[TABLE]
where is the typical time scale associated with the electron-electron interaction, describes disorder scattering, – the electron-phonon interaction, and “etc” stands for any other scattering-related time scale in the problem (e.g., the “recombination” time , see below).
Assume that the condition (1) is sufficient to uphold the conservation laws in the electronic system. Then they can be expressed in terms of continuity equations, that can be either written down on symmetry grounds Landau and Lifshitz (1959) or can be obtained by integrating the kinetic equation Lifshitz and Pitaevskii (1981). The first of these equations is the standard continuity equation reflecting charge conservation
[TABLE]
The second equation reflects energy conservation. In the case of charge carriers, this equation differs Narozhny et al. (2017); Lucas and Fong (2018) from its textbook counterpart Landau and Lifshitz (1959); Lifshitz and Pitaevskii (1981) by an extra term describing Joule’s heat
[TABLE]
Here and are the energy density and current, is the electric field, and is the electron charge.
The third equation describes momentum conservation. In contrast to the corresponding equation for a neutral fluid Landau and Lifshitz (1959); Lifshitz and Pitaevskii (1981), this equation takes into account the effect of electromagnetic fields. Moreover, for reasons that will become clear below, we include a small [as required by Eq. (1)] disorder-scattering term Narozhny et al. (2015); Briskot et al. (2015)
[TABLE]
Here is the momentum density, is the momentum flux (or stress tensor), and is the magnetic field.
The continuity equations (2a) - (2c) are valid for any electronic system satisfying Eq. (1). In the particular case of graphene, one may neglect scattering processes that change the number of particles in each individual band (e.g., the Auger processes, three-particle collisions, electron-phonon interaction, etc.) such that the number of particles in each band should be conserved separately. As a result, one finds another continuity equation Foster and Aleiner (2009); Narozhny et al. (2017); Lucas and Fong (2018)
[TABLE]
where and are the so-called “imbalance” (or total quasiparticle) density and currents that are related to the particle number densities, , and currents, , in the two bands as
[TABLE]
The kinetic derivation Lifshitz and Pitaevskii (1981); Briskot et al. (2015) of the continuity equations (2) has the advantage of providing “microscopic” definitions of all macroscopic quantities in Eqs. (2) in terms of the quasiparticle distribution function. In graphene (or any other two-band system), one may label the single-particle (band) states by the band index, , and the momentum, . Denoting the distribution function by , we define the above densities and currents as
[TABLE]
[TABLE]
[TABLE]
[TABLE]
[TABLE]
[TABLE]
Here is the degeneracy factor. The second equality in Eq. (3f) is specific to the Dirac spectrum in graphene and represents a crucial difference between the electron fluid in graphene and the usual (massive) fluids. Indeed, assuming the Dirac form of the quasiparticle spectrum Katsnelson (2012)
[TABLE]
one immediately finds the following relations between velocity and momentum (where denotes the unit vector in the direction indicated by the subscript)
[TABLE]
Inserting Eqs. (5) into Eqs. (3g) and (3f), one concludes that (i) the momentum density in graphene is equivalent to the energy flux, and (ii) the hydrodynamic flow in graphene describes the energy flow in contrast to the standard hydrodynamics describing the mass flow of a conventional fluid. Moreover, conservation of momentum leads to the conclusion that the energy flux in graphene is not relaxed by electron-electron interaction. The system can only reach the steady state by means of (weak) disorder scattering Narozhny et al. (2015); Briskot et al. (2015) described by the last term in Eq. (2c).
II Ideal hydrodynamics in graphene
The true equilibrium state (in the absence of the external fields) is described by the Fermi-Dirac distribution function yielding constant densities and zero currents, such that each term in Eqs. (2) vanishes. Applying weak external fields one drives the system weakly out of equilibrium. This can be described either by means of the perturbative linear-response theory Narozhny et al. (2015), or, if the condition (1) is fulfilled, by the hydrodynamic theory Narozhny et al. (2017); Lucas and Fong (2018). The latter approach requires two additional assumptions.
First, one assumes the spatial and temporal variations of the external fields and the resulting currents and density inhomogeneities to be small [ultimately, in the sense of Eq. (1) or the equivalent relation of the corresponding length scales], such that the electron-electron scattering processes may maintain local equilibrium. The latter is described by the distribution function Hartnoll et al. (2007); Briskot et al. (2015); Narozhny et al. (2017); Lucas and Fong (2018); Narozhny (2019)
[TABLE]
where , , and are the local chemical potential, local temperature, and hydrodynamic (or “drift”) velocity, respectively.
Using the distribution function (3), one finds the expressions for the equilibrium hydrodynamic quantities as well as the thermodynamic pressure, , and enthalpy, , listed in Appendix A. Substituting these quantities into the continuity equations (2), one obtains the (ideal) hydrodynamic equations. In particular, expressing the continuity equation (2c) for the momentum density in terms of the hydrodynamic velocity, , we obtain the generalized Euler equation Landau and Lifshitz (1959)
[TABLE]
Equation (7) was suggested in Ref. Müller et al., 2009 in the absence of electromagnetic fields and weak disorder (terms due to the electric field were discussed in Ref. Briskot et al., 2015). In comparison to the standard Euler equation, the generalized equation (7) contains two extra terms: (i) the time derivative of pressure that can be interpreted as a reminder of the relativistic nature Hartnoll et al. (2007); Lucas and Fong (2018) of the quasiparticle spectrum in graphene, Eq. (4), and (ii) the disorder scattering term necessary to establish a steady state Narozhny et al. (2015); Briskot et al. (2015); Narozhny (2019).
Away from charge neutrality, the Euler equation (7) allows for a homogeneous, steady flow Narozhny et al. (2015) that is equivalent to the usual Ohmic current [using Eqs. (37) - (41) with and ]
[TABLE]
characterized by the standard Drude-like expressions for the longitudinal and Hall resistivities
[TABLE]
where is the Hall coefficient.
The complete set of the equations of ideal hydrodynamics in graphene includes the generalized Euler equation (7), the continuity equations (2a), (2b), and (2d), as well as the Poisson’s equation relating the charge density to the electric field and the (thermodynamic) equation of state Hartnoll et al. (2007); Briskot et al. (2015), see Eqs. (41),
[TABLE]
This equation has the thermodynamic nature and represents the second assumption needed to build the hydrodynamic theory, namely, that thermodynamic quantities and their relations are not affected by the dissipative corrections to the ideal hydrodynamics Lifshitz and Pitaevskii (1981).
III Generalized Navier-Stokes equation in graphene
Taking into account dissipative processes modifies the macroscopic quantities and turns the ideal Euler equation into the Navier-Stokes equation, the central equation of the hydrodynamic theory Landau and Lifshitz (1959). Following the standard approach Landau and Lifshitz (1959); Lifshitz and Pitaevskii (1981); Narozhny et al. (2017); Lucas and Fong (2018), we focus on the velocity-independent kinetic coefficients. In graphene, these include the viscosity and “quantum conductivity” (cf. the thermal conductivity in the traditional hydrodynamics Landau and Lifshitz (1959)).
In the usual hydrodynamics Landau and Lifshitz (1959); Briskot et al. (2015); Lucas and Fong (2018); Narozhny (2019), viscosity is defined as the coefficient in the leading term of the gradient expansion of the dissipative correction to the stress tensor
[TABLE]
where , , and are the field dependent shear Alekseev (2016); Scaffidi et al. (2017); Steinberg (1958) and Hall Alekseev (2016); Scaffidi et al. (2017); Steinberg (1958); Bradlyn et al. (2012); Pellegrino et al. (2017); Narozhny (2019) viscosities (the latter appears only in the presence of magnetic field; bulk viscosity in graphene vanishes, at least to the leading approximation Briskot et al. (2015); Narozhny et al. (2017); Lucas and Fong (2018)). While the sign of is fixed by thermodynamics Landau and Lifshitz (1959); Lifshitz and Pitaevskii (1981), the sign of is not. Similarly to Ref. Berdyugin et al., 2019, we adopt the convention where the Hall viscosity is positive for electrons Narozhny (2019) (and negative for holes).
Substituting Eqs. (9) into the continuity equation (2c) and repeating the steps leading to the Euler equation (7), we obtain the generalized Navier-Stokes equation Narozhny (2019)
[TABLE]
Comparing the first terms in the left- and right-hand sides of Eq. (10), we define the kinematic viscosity
[TABLE]
with the dimensionality of the diffusion constant (m2/s).
The second set of the kinetic coefficients describes the dissipative corrections to the quasiparticle currents Briskot et al. (2015); Narozhny (2019) with (in the presence of disorder, the energy current acquires a dissipative correction of its own):
[TABLE]
The “imbalance” chemical potential is relevant for thermoelectric effects Foster and Aleiner (2009), which will be considered elsewhere. In this paper we disregard the possibility of the temperature gradients and set (or ).
At charge neutrality, the matrix is block diagonal, i.e., the electric current decouples from the energy and imbalance currents. For , the total current is given by the dissipative correction which remains finite even in the absence of disorder, ,
[TABLE]
Here is known as the “quantum” or “intrinsic” conductivity of graphene Kashuba (2008); Müller et al. (2008); Schütt et al. (2011); Briskot et al. (2015); Lucas and Fong (2018); Narozhny (2019). Within the electronic hydrodynamics in graphene, this quantity appears instead of the usual thermal conductivity due to the special relation between the energy current and momentum, see Eq. (3f) and the discussion following Eq. (5).
Together with the continuity equations (2) and the equation of state (8), the generalized Navier-Stokes equation (10) forms a closed system of hydrodynamic equations that can be solved in arbitrary geometries (see Ref. Kiselev and Schmalian, 2019 for the appropriate boundary conditions). Away from charge neutrality, these equations have to be solved together with the electrostatics equations similarly to the usual Vlasov self-consistency Lifshitz and Pitaevskii (1981); Briskot et al. (2015). In free (e.g., suspended) graphene the latter is given by the Poisson’s equation. In gated structures used in the majority of experiments Bandurin et al. (2016); Krishna Kumar et al. (2017); Bandurin et al. (2018); Berdyugin et al. (2019) the electrostatics is dictated by the gate Aleiner and Shklovskii (1994); Alekseev et al. (2015), simplifying the relation between the charge density and the electric field.
IV Kinetic calculation of electronic viscosity in graphene
In this section we report the kinetic theory results for the electronic viscosity in graphene. The calculation method was outlined in Ref. Briskot et al., 2015, but unfortunately involves some tedious algebra yielding the viscosity coefficients in terms of rather cumbersome multidimensional integrals, see Appendix B. In the simple limiting cases (e.g., at charge neutrality and in the degenerate, “Fermi-liquid” regime), analytical results can be obtained. Otherwise, for arbitrary doping levels the shear and Hall viscosities, see Eqs. (42), are computed numerically. These results are illustrated in Figs. 1 - 3. Details of the derivation are published in Ref. Narozhny, 2019.
The kinetic theory is formally valid only in the weak coupling limit. In particular, the “collinear” (or “three-mode”) approximation Briskot et al. (2015); Fritz et al. (2008); Narozhny (2019) that allows us to solve the kinetic equation is formally justified in the limit ( is the coupling constant in graphene). Therefore, in order to obtain experimentally relevant numerical values for the viscosity coefficients we supplement the kinetic theory calculation with the renormalization group analysis described in the following section.
IV.1 Shear viscosity at charge neutrality
At charge neutrality, the general expressions (42) simplify and can be evaluated analytically Müller et al. (2009); Briskot et al. (2015) (up to a multiplicative numerical factor). The Hall viscosity vanishes identically (due to the exact electron-hole symmetry), while the shear viscosity exhibits the following behavior.
In zero magnetic field, we recover the well-known result Müller et al. (2009) (the parametric dependence follows from the fact that the only energy scale in neutral graphene is )
[TABLE]
The numerical coefficient was first evaluated in Ref. Müller et al., 2009 reporting the value . Although not explicitly discussed Müller et al. (2009), this result was obtained using the “bare” Coulomb interaction, i.e., neglecting screening effects. Such an approach is formally valid for asymptotically low temperatures Fritz et al. (2008); Kashuba (2008); Schütt et al. (2011) where the coupling constant is expected to have been renormalized to a small enough value (see below for the discussion of the renormalization group approach). Indeed, evaluating the integrals (44) for the “scattering rates” with unscreened Coulomb interaction numerically, we find , where the deviation stems from the systematic differences between various numerical methods. The small difference between the above result and that of Ref. Müller et al., 2009 is due to the fact that our calculation takes into account only the direct interaction, while the exchange term is small Kashuba (2008); Schütt et al. (2011) in .
In magnetic field, the shear viscosity decreases but remains finite in classically strong fields (due to the aforementioned decoupling of the charge mode)
[TABLE]
where
[TABLE]
and, again neglecting screening effects, and . The field dependence of the shear viscosity at charge neutrality is illustrated in Fig. 1.
IV.2 Viscosity away from charge neutrality
Away from charge neutrality, the shear viscosity (42a) has to be evaluated numerically, with the exception of the so-called “Fermi-liquid” or degenerate regime, . In that limit, the momentum integral in Eq. (44) is dominated by the momenta [for definition of the dimensionless variables see Eq. (48)] and can be evaluated analytically. For example (here ),
[TABLE]
Unscreened Coulomb interaction corresponds to (see below for a discussion of the screening effects).
Evaluating the momentum integral for unscreened Coulomb interaction in the limit yields
[TABLE]
which together with the rest of the integrals (44) leads to the following expression for the shear viscosity
[TABLE]
where . The numerical factors in the denominator represent small corrections to the leading behavior that have to be taken into account since otherwise the matrix of the scattering rates (43f) is degenerate.
Once the magnetic field is applied, the shear viscosity (42a) decreases, while the Hall viscosity (42b) becomes nonzero. In classically strong fields both viscosities vanish (in contrast to the behavior at ). In the degenerate regime, the field dependence of the viscosity coefficients follows the simple semiclassical expectation Berdyugin et al. (2019); Alekseev (2016); Scaffidi et al. (2017) (similarly to the Drude conductivity tensor):
[TABLE]
The field dependence (18) was suggested in Refs. Steinberg, 1958; Alekseev, 2016 for a single-component Fermi liquid. In graphene in the degenerate limit, essentially only the single band contributes to physical observables and hence one expects to recover the single-band results. The kinetic calculation allows us to give a precise definition to the scattering rate appearing in Eqs. (18). Indeed, this rate differs Principi et al. (2016); Briskot et al. (2015) from the transport scattering rate Schütt et al. (2011); Narozhny et al. (2012), determining the electrical conductivity as well as from the “quantum” scattering rate Schütt et al. (2011) determining the quasiparticle lifetime.
In Figs. 2 and 3 we compare the results of the numerical evaluation (with unscreened Coulomb interaction, for simplicity) of the shear viscosity (42a) and Hall viscosity (42b) with the asymptotic expressions (18). Qualitatively, the shape of the field dependence is the same for all values of the chemical potential. The semiclassical dependence (18) becomes indistinguishable from the full result at .
V Renormalization group approach
Quantitative evaluation of the shear and Hall viscosities (42a) and (42b) in physical units requires the knowledge of the coupling constant . Following Refs. Sheehy and Schmalian, 2007; Müller et al., 2009; Link et al., 2018b we treat this constant as a running coupling constant in the sense of the renormalization group (RG). The final values for physical observables are then obtained by combining the RG with the scaling laws for these quantities.
The one-loop Kadanoff-Wilson RG approach to interacting Dirac fermions in graphene was suggested in Refs. Sheehy and Schmalian, 2007; González et al., 1999, 1994. The idea is to relate physical observables to their counterparts at the specifically chosen renormalization scale, where the renormalized theory is characterized by weak coupling and the kinetic theory is justified.
The renormalized carrier density obeys the relation Sheehy and Schmalian (2007)
[TABLE]
Here and are the solutions of the RG equations. The latter are only valid in the low-temperature quantum limit, , where is related to the bandwidth. Choosing the renormalization condition for and , one finds , leading to the zero-temperature carrier density Sheehy and Schmalian (2007)
[TABLE]
For the nondegenerate system, , the renormalization condition is essentially the same as at criticality Millis (1993) (e.g., neutral graphene), , leading to
[TABLE]
For general and , the leading behavior is captured by
[TABLE]
where is a dimensionless function of ratio that can be read off Eq. (37a) (for ). The ratio does not change under the RG, hence only the explicit dependence on the velocity is renormalized Kashuba (2008). At the same time, the renormalized coupling constant is
[TABLE]
The “bare” coupling constant in suspended graphene is (corresponding to the “bare” velocity m/s), while for graphene encapsulated in boron nitride Bandurin et al. (2016) this reduces to (here is the effective dielectric constant). Assuming the value K, see Refs. Sheehy and Schmalian, 2007; Peres et al., 2006, and we estimate the effective coupling constant in neutral graphene
[TABLE]
Even assuming a smaller, “Fermi-liquid” coupling constant, , derived from earlier measurements Kozikov et al. (2010); Titov et al. (2013), we find the renormalized value of at the lowest temperatures and in the hydrodynamic range.
For realistic values of the carrier density in graphene in the degenerate regime Bandurin et al. (2016); Krishna Kumar et al. (2017); Bandurin et al. (2018); Berdyugin et al. (2019), the logarithmic renormalization (20) is appreciable, see Fig. 4. For K, the dimensionful prefactor in Eq. (20) has the value
[TABLE]
Neglecting the renormalization factor in Eq. (20) and using the “Fermi-liquid” asymptotics, , we estimate the chemical potential corresponding to the typical density, cm*-2*, as
[TABLE]
Restoring the renormalization factor, we find increased values for the chemical potential, see Fig. 4 (the values shown in the figure were evaluated for ). For the same carrier density we find
[TABLE]
with the corresponding renormalized coupling constant
[TABLE]
For the smaller “bare” coupling constant, , the above values change to
[TABLE]
Neither renormalization factor is negligible leading to a strong enhancement of the results of the kinetic theory.
Similarly to Eq. (19), the viscosity renormalizes as Müller et al. (2009); Link et al. (2018b)
[TABLE]
where is the magnetic field. Representing the weak-coupling kinetic-theory result (42a) as
[TABLE]
one finds Kashuba (2008); Müller et al. (2009) that the product doesn’t renormalize. This leads to the conclusion Sheehy and Schmalian (2007) that the kinetic expression for the shear viscosity at charge neutrality, Eq. (14), provides the correct low temperature result for interacting Dirac fermions in graphene (for ). Implicit to this argument is the assumption of the large screening length Kashuba (2008). Indeed, static screening is determined by the real part of the polarization operator, , which for small enough momenta is well approximated by the density of states Narozhny et al. (2012),
[TABLE]
where , see Eq. (43b). The scaling of the density of states was derived in Refs. Sheehy and Schmalian, 2007; Hwang et al., 2007.
The quantities are defined similarly to Eq. (18c)
[TABLE]
where the dimensionless functions can be read off Eqs. (18c) and (44).
Finally, the kinematic viscosity (11) is a combination of the shear viscosity, renormalized velocity, and energy density. The latter renormalizes as the free energy Sheehy and Schmalian (2007)
[TABLE]
which yields
[TABLE]
The kinematic viscosity (11) can be obtained by combining Eqs. (23) and (26) with the equation of state (8). The result is given by
[TABLE]
The results of the one-loop RG approach reviewed in this section should be treated with care. Ultimately, this is a perturbative calculation that is formally valid for weak coupling. Strictly speaking, this is not the case in real graphene (see the above estimates for the effectiv coupling constant) and hence the kinetic coefficients, such as viscosity, should be considered phenomenologically and assigned the experimentally measured values Lucas and Fong (2018). Nevertheless, it is instructive to evaluate the expressions for kinetic coefficients with the corresponding renormalizations to obtain a quantitative theoretical expectation for physical observables.
VI Quantitative results for electronic viscosity in graphene
In this section we report the results of the numerical evaluation of the shear and Hall viscosity in graphene (42) taking into account the renormalization and screening effects.
VI.1 Screening effects
The above analytical results were obtained for the bare Coulomb interaction and are valid only in the limit of the infinitesimal interaction strength, . For more realistic values of , screening effects have to be taken into account. Within the RPA approximation Schütt et al. (2011); Narozhny et al. (2012); Lucas and Fong (2018) the dynamically screened Coulomb interaction is given by
[TABLE]
where is the polarization operator (for a detailed calculation of the polarization operator see, e.g., Ref. Narozhny et al., 2012). In the dimensionless form of Eq. (16) one finds
[TABLE]
For analytical estimates in the degenerate regime one can use the usual Thomas-Fermi static screening Schütt et al. (2011); Narozhny et al. (2012)
[TABLE]
In full units the inverse screening length is . The use of the static screening in Eq. (16) can be justified by the fact that in this integral the contribution of the region is explicitly suppressed, while outside of this region for the polarization operator in graphene is well approximated by a constant Schütt et al. (2011); Narozhny et al. (2012).
Taking into account static screening, we find for the momentum integral in the opposite order of limits (first, , then )
[TABLE]
The first two terms are identical for all integrals (43f), so again we need to keep the subleading term. Combined with the rest of the integrals (44) this leads to the result
[TABLE]
where . The factor is kept in the denominator in order to emphasize that the logarithmic dependence on the coupling constant is only valid in the limit such that . For any practical value of the coupling constant Eq. (29) is negative and thus invalid. Instead of the limit , one has to consider the full expression for .
The leading parametric dependence in Eq. (29) (up to the correction, ) was first suggested in Ref. Principi et al., 2016. The numerical prefactor that can be found in Ref. Lucas and Fong, 2018 appears to be twice sa large as ours.
In gated structures screening is modified by the presence of the gate Aleiner and Shklovskii (1994). In particular, the “bare” Coulomb interaction should be replaced by
[TABLE]
where is the distance to the gate. This form assumes the single gate device. Note, that the experiments of Ref. Bandurin et al., 2016 were performed on double gate devices as well. In the latter case, the effective Coulomb interaction has a more complicated form. However, if the gate is placed far enough from the graphene sample (Ref. Bandurin et al., 2016 reports the thickness of the insulating layer to be about nm), such that , then the screening effect of the gate may be neglected.
VI.2 Kinematic viscosity in zero field
Kinematic viscosity in graphene as a function of the carrier density is shown in Fig. 5, where we plot our results in physical units taking into account the renormalizations (20) and (27) as well as the dynamical screening (28). The results are in a reasonably good agreement with the experimental data reported in Fig. 4 of Ref. Bandurin et al., 2016: the theoretical values are of the same order of magnitude, m2/s, as the experimental ones, the density dependence in the range cm*-2* is rather weak, and the overall value decreases slightly with the temperature increase from K to K.
Our results were obtained assuming the value for the “bare” coupling constant (as reported in the Supplemental Material to Ref. Bandurin et al., 2016). The “bare” velocity in graphene was taken as m/s. Then at K, the dimensionful prefactor in Eq. (27) has a value
[TABLE]
which ultimately determines the order of magnitude of the resulting kinematic viscosity.
Combining this prefactor with the asymptotic behavior of [which can be read off Eqs. (17) or (29) disregarding the logarithm] and [from Eq. (39)], we estimate the dominant temperature dependence of the kinematic viscosity (11) in the degenerate regime as
[TABLE]
This “naive” estimate neglects the temperature dependence arising from the renormalizations and the logarithmic factors in Eq. (17) [or Eq. (29)]. Nevertheless, the true temperature dependence is not far off as shown in Fig. 6 where we plot Eq. (31) together with the “Fermi-liquid” asymptotics for the kinematic viscosity (11) based on Eq. (16) and static screening (a reasonable approximation in the degenerate regime, see Fig. 5; the dashed curve is vertically shifted for clarity).
Similarly, we can estimate the temperature dependence of the kinematic viscosity at charge neutrality. Using Eq. (13) and the relation , we find
[TABLE]
Again, the true temperature dependence will be slightly different due to the renormalization factors (the screening length at charge neutrality is determined by temperature and hence does not lead to any additional temperature dependence).
For the higher temperature range shown in Fig. 6 the kinematic viscosity may be fitted Principi et al. (2016) by another power law, . However, this is an intermediate regime: for higher temperatures, K, the calculated temperature dependence shows clear deviations from this behavior.
Finally, typical theoretical values of the kinematic viscosity shown in Fig. 5 differ from those reported in Ref. Bandurin et al., 2016 by about a factor of . Our calculation does not involve any fitting parameters and does not take into account any particular features of the experimental device, e.g., screening by the gate and disorder scattering. As we have already mentioned, the renormalization group calculation leading to the factors of is approximate, so that we do not expect to find a perfect agreement with the data. A true test of the theory would be to calculate the quantities actually measured in the experiment (e.g., the nonlocal resistivity Bandurin et al. (2016), ) for realistic sample geometries. The results of such calculations will be reported in a subsequent publication.
VI.3 Hall viscosity
Defining the “kinematic” counterpart of the Hall viscosity similarly to Eq. (11),
[TABLE]
and using the same RG approach, we find that renormalizes similarly to Eq. (27)
[TABLE]
Here is defined according to Eq. (23). For K, T and neglecting renormalizations, the dimensionless quantity (in SI units) is given by
[TABLE]
The resulting values are shown in Figs. 7 and 8 in physical units. The former shows as a function of the external magnetic field for a fixed value of the charge density, cm*-2*. The results shown in Fig. 7 significantly exceed the experimental values shown in Fig. 3 of Ref. Berdyugin et al., 2019. The origin of this discrepancy is in the high power of the renormalization factor in Eqs. (34) and (24). Indeed, combining Eqs. (18b), (34), and (24), we find
[TABLE]
Here the dimensionless function is defined similarly to Eq. (24) with the dominant contribution coming from the scattering time [defined in Eq. (44)].
The temperature dependence of shown in Fig. 8 for weak magnetic fields, , and in the degenerate regime can be extracted from Eqs. (35) and (44),
[TABLE]
Similarly to Eqs. (31) and (32) this expression disregards additional temperature dependence from the renormalizations and screening [i.e., the logarithmic factors in Eqs. (17) or Eq. (29)]. Nevertheless, it accounts for the temperature dependence of the Hall viscosity in the degenerate regime rather well, see Fig. 8.
VII Summary
In conclusion, we have calculated the shear and Hall viscosities in graphene at arbitrary doping levels and classical (nonquantizing) magnetic fields using the kinetic theory approach combined with the RG analysis. The shear viscosity in graphene exhibits a monotonous growth as a function of carrier density (or chemical potential) from a small value at charge neutrality, see Eqs. (17) and (29). In contrast, the kinematic viscosity (11) remains of the same order of magnitude at all doping levels, see Fig. 5: decays from the initial value at and then passes through a minimum followed by a (initially weak) growth in the degenerate regime. This behavior follows from the nontrivial density dependence of the enthalpy (or equivalently, energy density). The appearance of the enthalpy in the definition of kinematic viscosity (11) is a characteristic feature of the electronic system in graphene (in contrast, the usual definition of the kinematic viscosity involves the mass density Landau and Lifshitz (1959)).
The field dependence of the shear and Hall viscosities shown in Figs. 2 and 3 can be expected on general grounds. In particular, the Hall viscosity vanishes at zero magnetic field as well as for classically strong fields and hence has to exhibit a maximum. In the degenerate regime, both viscosities are well described by the semiclassical expressions (18) first suggested in Ref. Alekseev, 2016. For smaller densities the shape of the field dependence of and deviates from Eqs. (18), but remains very similar. The only exception to this argument is the field dependence of the shear viscosity at charge neutrality, see Fig. 1, which remains finite in classically strong fields. This effect can be traced to the complete decoupling of the charge and energy currents at charge neutrality.
In the degenerate regime of large charge densities, our results are in a reasonably good agreement with the available experimental evidence. The quantitative discrepancies between the theoretical values shown in Figs. 5-8 and the results of Refs. Bandurin et al., 2016; Berdyugin et al., 2019 can be attributed to our use of the renormalization group resulting in relatively strong enhancement of the kinematic viscosity (11) and especially the kinematic Hall viscosity (33). Moreover, our calculation does not include sample-specific details such as screening by the gate and disorder scattering. The latter can be expected to reduce the viscosity values. In any case, a true test of the theory would be a calculation of several distinct quantities actually measured in the experiment for realistic sample geometries (using, e.g., the experimentally measured Siegel et al. (2011); Elias et al. (2011); Hwang et al. (2012) values for renormalized velocity). Such results will be reported elsewhere.
Acknowledgements.
We thank I.V. Gornyi, A.D. Mirlin, and J. Schmalian for fruitful discussions. This work was supported by the German Research Foundation DFG within FLAG-ERA Joint Transnational Call (Project GRANSPORT) and the MEPhI Academic Excellence Project, Contract No. 02.a03.21.0005 (BNN) and the European Union’s Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie Grant Agreement No. 701647 (MS).
Appendix A Local equilibrium quantities
Under the assumption of local equilibrium, the macroscopic quantities appearing in the hydrodynamic equations are given by
[TABLE]
[TABLE]
where is the polylogarithm,
[TABLE]
[TABLE]
[TABLE]
Appendix B General expressions for the viscosity coefficients
The general expressions for the shear and Hall viscosities in graphene
[TABLE]
with the following notations
[TABLE]
The “scattering rates” are obtained from the collision integral within the three-mode approximation Briskot et al. (2015) and are given by
[TABLE]
where
[TABLE]
These functions are expressed in terms of the integrals
[TABLE]
that are evaluated for either of the two functions
[TABLE]
The frequency and momentum are expressed in terms of the dimensionless variables
[TABLE]
Finally, the Coulomb interaction has the form
[TABLE]
where is the dielectric constant of the dielectric environment and the dimensionless factor accounts for screening.
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