Ground State Solutions of the Complex Gross Pitaevskii Equation Associated to Exciton-Polariton Bose-Einstein Condensates
Hichem Hajaiej, Slim Ibrahim, Nader Masmoudi

TL;DR
This paper proves the existence of ground state solutions for a Gross-Pitaevskii equation modeling exciton-polariton Bose-Einstein condensates, highlighting their macroscopic quantum nature and addressing mathematical challenges from pumping and damping terms.
Contribution
It introduces a novel mathematical analysis demonstrating ground state existence for a complex Gross-Pitaevskii equation with pumping and damping effects.
Findings
Existence of ground state solutions established
Condensation occurs under certain conditions
Solved the associated Cauchy problem and derived laws
Abstract
We investigate the existence of ground state solutions of a Gross-Pitaevskii equation modeling the dynamics of pumped Bose Einstein condensates (BEC). The main interest in such BEC comes from its important nature as macroscopic quantum system, constituting an excellent alternative to the classical condensates which are hard to realize because of the very low temperature required. Nevertheless, the Gross Pitaevskii equation governing the new condensates presents some mathematical challenges due to the presence of the pumping and damping terms. Following a self-contained approach, we prove the existence of ground state solutions of this equation under suitable assumptions: This is equivalent to say that condensation occurs in these situations. We also solve the Cauchy problem of the nonlinear Schroedinger equation and prove some corresponding laws.
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Ground State Solutions of the Complex Gross Pitaevskii Equation Associated to Exciton-Polariton Bose-Einstein Condensates
Hichem Hajaiej Slim Ibrahim & Nader Masmoudi
Abstract: We investigate the existence of ground state solutions of a Gross-Pitaevskii equation modeling the dynamics of pumped Bose Einstein condensates (BEC). The main interest in such BEC comes from its important nature as macroscopic quantum system, constituting an excellent alternative to the classical condensates which are hard to realize because of the very low temperature required. Nevertheless, the Gross Pitaevskii equation governing the new condensates presents some mathematical challenges due to the presence of the pumping and damping terms. Following a self-contained approach, we prove the existence of ground state solutions of this equation under suitable assumptions: This is equivalent to say that condensation occurs in these situations. We also solve the Cauchy problem of the nonlinear Schrödinger equation and prove some corresponding laws.
1 Introduction
The first realization of condensation has been obtained experimentally in a system consisting of about half million alkali atoms cooled down to nano-Kelvin temperature. Thus, a considerable obstacle in the study of (BEC) is the very low temperature required to create the condensate. Completely aware that it is extremely important to explore what kind of condensates can undergo condensation at higher temperatures, huge efforts have been undertaken by scientists to overcome this difficulty right after the first experimental realization of the first (BEC) in 1995. During the last years, a new kind of condensates has attracted the attention of many scientists. Very recently, it turned out that an excellent candidate is a system of exciton-polaritons, which are bosonic quasiparticles that exist inside semiconductor micro-cavities, consisting of a superposition of an exciton and a cavity photon. Above a threshold density, the polaritons macroscopically occupy the same quantum state, forming a condensate. The temperatures that are usually used to form exciton-polariton BECs are around T=10K, far higher than the nano-Kelvin temperatures required for atomic BECs. They are immensely promising in terms of new quantum technologies since quantum effects can appear on a macroscopic level, unlike most systems where quantum effects are rather easily destroyed by temperature and decoherence. As Boson particles are composed of quantum well excitons and optical cavity photons, microcavity exciton-polaritons possess unique intrinsic features: reminiscent excitonic nature leads to important interaction dynamics among exciton-polaritons. Polariton-polariton repulsive interactions are indeed crucial to stimulate scattering processes in order to relax into the ground state Bose-Einstein condensates (BECs). Since the temperature of condensation is inversely proportional to the mass of the particles, the exciton-polariton systems afford relatively high temperatures of condensation. The first drawback of these new condensates is their very short lifetime (approximately 1 ps), inherited also from their photonic component, so that polariton thermalization could be problematic. In fact the polariton gas can become fully thermalized, as a result of strong polariton-polariton interaction caused by their excitonic component. The second important inconvenient comes from the fact that the excitons disappear with the recombination of the electron-hole pairs through emission of photons. One way to overcome these problems is to introduce a polariton reservoir: polaritons are “cooled”and “pumped”from this reservoir into the condensate. At the same time, a low density level is kept in order to reduce the interactions between polaritons. Different mathematical models have been suggested for this new condensate. In this paper we consider the one proposed in [16], called complex Gross-Pitaevski equation. For a more detailed account of these aspects, see [23] and references therein.
In [23], the authors addressed the nature of radially symmetric standing wave-type solutions of the following nonlinear Gross-Pitaevskii equation:
[TABLE]
where is a complex-valued function defined on , is the Laplace operator on , is the harmonic potential, and .
To achieve their goals, they have developed a numerical collocation method but they did not provide any theoretical justification of their claims. The main objective of this paper is to rigorously prove the existence of ground state solutions of the Gross-Pitaevskii equation under study. We believe that this is a challenging and immensely important scientific question. The principle challenge comes from the fact that all classical methods do not seem to be applicable to discuss the existence of stationary solutions to (GPPD). This is essentially due to the simultanous presence of the dissipation and pumping terms simultaneously. Let us note that the establishment of ground state solutions avoids costly and very difficult experiments in the “classical”BEC. To achieve this goal, let us first introduce some important quantities associated to (GPPD).
Recall that the mass , the Hamiltonian , the action ( and the functional associated to the equation (GPPD) are given by:
[TABLE]
respectively. Observe that
[TABLE]
and
[TABLE]
Identity (1.5) shows that, at least formally, the mass and the energy are pumped into the system through the term involving the parameter and they are nonlinearly damped by the term involving the parameter . Contrarily to the complex Ginzburg-Landau equation (when a dissipatif term of the form is added to the RHS of (GPDP)), one cannot obtain time-uniform estimates of the solution in the energy space. The complex Gross-Pitaevski equation reflects the non-equilibrium dynamics described above by adding pumping and decaying terms to the GP equation.
Before going any further, we recall a few results about the linear equation without dissipation and pumping. The equation then reads
[TABLE]
We define the energy space , endowed with the -scalar product , by
[TABLE]
Also, define the dual space of as follows. For any , there exists a unique such that with the norm on given by
[TABLE]
Recall that is the norm in . It is well known that the unbounded operator defined on
[TABLE]
is self-adjoint. Moreover, the lowest eigenvalue of denoted by is simple with eigenfunction . Notice that can be constructed variationally as
[TABLE]
In particular, for any , we have
[TABLE]
For more details, we refer for example to [15].
When the chemical potential is complex , solitary wave solution would grow exponentially fast as which can be bad for the analysis as well as for numerics and experiments. Assuming that , yields the following stationary problem for :
[TABLE]
Multiplying (-) by and integrating gives the following identity.
[TABLE]
The condition for the chemical potential of being real is then equivalent to the fact that is a zero of .
It is important to emphasize that due to the presence of the dissipation and pumping mechanisms, we find it hard to apply the standard variational or PDE methods to construct soliton-type solutions of (GPPD) (i.e. a solution of (-)). In this paper, our idea to construct a solution of (-) with real chemical potential goes along a perturbative way by introducing a small parameter factor in the dissipation and pumping term. More precisely, for all , consider
[TABLE]
and its corresponding stationary equation
[TABLE]
The object is to construct a solution in the form
[TABLE]
where the approximate solution will be given explicitly, and is the error term that needs to be found. To define , we need to introduce some notation and state a few preliminary useful results. The first Theorem of this paper reads as follows:
Theorem 1.1**.**
Let be a continuous nontrivial function. There exist and a positive small such that, for any and , the complex Gross-Pitaevkii equation () has a solitary wave solution with solving -.
Remark 1.1**.**
It would be very desirable to extend the branch of standing wave solutions we constructed for small to all values of . Unfortunately, so far we were not able to do so given the non-equilibrium structure of the model.
Our second result concerns the Cauchy problem associated to (GPPD). We have.
Theorem 1.2**.**
Assume , and . For any , there exists a unique global solution of (GPPD) with . Moreover, for any , we have
[TABLE]
The paper is organized as follows: In the next section, some preliminary results are proven. This will prepare the field to the establishment of ground state solutions. In section 3, we will present our self-contained proof built up to prove the existence of ground state solutions. The last section of this paper is dedicated to the Cauchy problem. We show the existence and uniqueness of solutions for a large class of damping and pumping terms. We also discuss the non-conservation of some important functionals associated to the Schrödinger equation.
2 Preliminaries
Here we focus on the problem without pumping and decay of the energy, that is when . We start by recalling a few known facts about the space , for which the proof can for example be found in Kavian-Weissler [15].
Lemma 2.1**.**
The Hilbert space is compactly embedded in for any .
Throughout this paper, we suppose that is nontrivial continuous and is in function.
Lemma 2.2**.**
For any , there exists a unique solving the following constrained variational problem:
[TABLE]
In addition, is non-negative, radial and radially decreasing.
Proof.
It is sufficient to show the existence of a minimizer of . The uniqueness of the minimizer follows directly from the strict convexity of the functional .
Now let us fix , let be a minimizing sequence of , i.e., and . Then
[TABLE]
Therefore, we can find such that
[TABLE]
This implies that
[TABLE]
Consequently, there exists such that
[TABLE]
This implies, thanks to Lemma 2.1, that in and . Thus, we certainly have that implying that is non-trivial, and by the lower semi-continuity, we can write:
[TABLE]
Therefore, . On the other hand, let be the unique minimizer of , then is a non-negative function in since
[TABLE]
Furthermore, by rearrangement inequalities [12, 13], we have:
[TABLE]
[TABLE]
[TABLE]
[TABLE]
Combining these identities, it follows that
[TABLE]
∎
The next Lemma, addresses the regularity of the Hamiltonian , as well as the map .
Lemma 2.3**.**
The Hamiltonian is in . Moreover, for all we have
[TABLE]
and the function
[TABLE]
Proof.
The proof of (i) follows from standard arguments. For example, we refer to reference [14], and we just prove (ii).
Fix . Let be a sequence of positive real numbers such that . We will first prove that
[TABLE]
Let be a sequence such that and By (2.1), we can find such that
[TABLE]
Now let , then and
[TABLE]
for any .
Therefore, we can find such that
[TABLE]
for any .
It follows from (i) that there exists a constant such that for all such that .
Thus, for all ,
[TABLE]
Consequently,
Then and then
[TABLE]
Now let us prove that if , then
[TABLE]
For all , there exists a sequence of functions in such that and
[TABLE]
Combining the proof of (2.1) and (2.4), we can find such that for all . Setting , we have that and
[TABLE]
Thus, following the proof of (2.4), we certainly get:
[TABLE]
Consequently, we have:
[TABLE]
yielding as desired. ∎
Proposition 2.4**.**
Let , and be a sequence of positive real numbers such that . Denote by the unique minimizer of , and the unique minimizer of . Then
[TABLE]
and
[TABLE]
Proof.
We will first prove that there exists such that converges weakly in to . First obviously . Now noticing that
[TABLE]
one has
[TABLE]
Therefore, using (2.4), there exists a constant such that
[TABLE]
Thus, (up to a subsequence), there exists such that
[TABLE]
Now using Lemma 2.1, we have that
[TABLE]
In particular, . Thus,
[TABLE]
and then . This shows that is the unique minimizer of . To end the proof, we need to show that
[TABLE]
and
[TABLE]
To prove (2.5), it is sufficient to notice that and in , while (2.6) follows from the fact that in . ∎
3 Ground State Solutions
Always in the case , and within the class of minimizers we have just constructed, we would like to intersect it with the co-dimension one manifold characterized by the zeros of the functional . Before doing so, let us first fix our assumptions on the decay and pumping parameters.
First we deal with case i.e. the standard nonlinear Schrödinger equation in the absence of both the pumping and dissipation. Equation (-) then becomes
[TABLE]
The first preliminary result is the first iteration. We have the following result:
Proposition 3.1**.**
There exists a non-negative radial function and solving (-). Moreover, satisfies
[TABLE]
Remark 3.1**.**
* will be the first approximate solution in the iteration process to construct the full solution of (-).*
Proof of Proposition 3.1.
It is sufficient to prove that the functional changes sign when the mass of the ground state given by Lemma 2.2 varies. Then the conclusion will follow using Lemma 2.3. Now, because of the positivity of , first observe that for any nontrivial non-negative continuous function , we have . Moreover, on the one hand, by the Gagliardo-Nirenberg inequality, there is a constant such that for any , we have
[TABLE]
On the other hand, multiplying (-) by and integrating shows that any solution of (-) satisfies
[TABLE]
Thus, if we have
[TABLE]
This shows that when , we have and thus , for some positive constant . Now since is a nontrivial continuous function, there exists a nontrivial open set and a positive constant such that , for all . We have , for some small positive constant . This implies that as . Now, we need to show that becomes negative for large masses. In fact, first we will prove that
[TABLE]
If we let , then clearly
[TABLE]
Now, we will explicitly calculate
[TABLE]
where with the norm
[TABLE]
Let be a minimizing sequence of that is
[TABLE]
From the above bounds, let us just denote by (instead of ), an -weak limit of . Denote by . First we show that . Up to an extraction, we may assume that a subsequence of (also denoted by ) converges weakly to in the sense of distributions; that is for any (smooth and compactly supported function), we have
[TABLE]
To show strong convergence in , we observe that (see for example [8])
[TABLE]
where, for any subset , the function introduced by H. P. Rosenthal [22] is given by
[TABLE]
Using Hölder inequality and the above bounds (3.2), we have for any
[TABLE]
which clearly shows that , and thus and , as desired. Moreover, by the lower semi-continuity of the norms, we have
[TABLE]
If the estimate were strict that would contradict the minimality of . The convergence is therefore strong in , and at the minimum we have
[TABLE]
yielding
[TABLE]
and
[TABLE]
Now we mollify in order to get an upper bound for . Set
[TABLE]
Calculating shows that
[TABLE]
Moreover, similar calculation enables us to see that
[TABLE]
In summary, in virtue of (3.3) and (3.4), we have
[TABLE]
which implies, thanks to the fact that ,
[TABLE]
The above estimates automatically imply
[TABLE]
Indeed, if (3.6) does not hold, then there would exist a sequence , and satisfying
[TABLE]
and
[TABLE]
On the other hand, for all and
[TABLE]
Now choosing , gives the bound
[TABLE]
leading to a contradiction by taking .Clearly, (3.6) shows that becomes negative as which finishes the proof. ∎
Notice that to construct a nonlinear solution to (-), one can use several techniques. Variationnally, for any given amount of mass , we have shown that a radial positive solution to (-) can be constructed through the following minimizing problem
[TABLE]
Moreover, this family of solutions is included in the branch of solutions constructed using bifurcation arguments pioneered by Rabinowitz, and Crandall-Rabinowitz [7]. Indeed, is a solution to (-) if and only if , where , , and the operators , and are defined by
[TABLE]
[TABLE]
and
[TABLE]
Indeed, the following proposition shows that a branch of solutions of (-) emerging from the linear solution can be constructed. The proof of the proposition is included in the proof of the spectral assumption given in the Appendix. (See section 5).
Proposition 3.2**.**
There exists such that for all , a unique solution , of (-) exists such that
[TABLE]
with , and .
For the solution to (-) satisfying given by Proposition 3.1, denote by
[TABLE]
and
[TABLE]
The second preliminary result concerns the operators . We have the following important property of .
Proposition 3.3**.**
Let be the subspace of consisting of all functions -orthogonal to . Then we have
[TABLE]
Moreover, there exists such that for all ,
[TABLE]
The property of comes from the breakdown of the spatial translation symmetry due to the presence of the potential. We refer to the Appendix (Section 5) for the proof of proposition 3.3 .
We have
[TABLE]
Since , then thanks to Proposition 3.3, one can uniquely define by
[TABLE]
Observe that given the smoothness and the decay of , we have . Moreover, we have
[TABLE]
Now, define and by
[TABLE]
and
[TABLE]
The bijectivity of enables us to determine , and again the regularity of shows that . Thus it only remains to determine the coefficient , and . They are determined by the orthogonality condition
[TABLE]
Indeed, substituting (given by inverting (3.9)) into (3.10) gives
[TABLE]
Now since , then clearly
[TABLE]
which insures that is uniquely determined in terms of , which were already defined. Then follows by inverting using the orthogonality . Now, set
[TABLE]
The main result of this section is the following.
Theorem 3.1**.**
For a heaviside function and , there exists such that for all , equation () has a solution that can be decomposed as
[TABLE]
with satisfying
[TABLE]
Proof of Theorem 3.1.
First, we write an equation for being a solution of (-). We start by further decomposing and observe that
[TABLE]
Substituting this in equation (-) and splitting the real and imaginary parts, we obtain
[TABLE]
and
[TABLE]
respectively. The identity coming from the real part can be rewritten in the following way.
[TABLE]
where is given by
[TABLE]
and can be explicitly computed. In particular it satisfies
[TABLE]
The identity coming from the imaginary part can be rewritten in the following way.
[TABLE]
where is given by
[TABLE]
and can be explicitely computed. In particular it satisfies
[TABLE]
Now we define a map by
[TABLE]
where, solves
[TABLE]
Now the purpose is to show that there are positive constants and such that the above map is a contraction on the ball
[TABLE]
for sufficiently small. The ball is endowed with the norm
[TABLE]
Thanks to the equation on and the invertibility of , we can write
[TABLE]
Plugging the above identity in the equation on , we obtain
[TABLE]
Since,
[TABLE]
then the choice of
[TABLE]
makes
[TABLE]
,which enables us to invert and thus calculate :
[TABLE]
Let
[TABLE]
[TABLE]
and
[TABLE]
To show that is a contraction, consider and in the ball and denote by and their respective images through the map . We have
[TABLE]
[TABLE]
and
[TABLE]
Estimating , and using the above bounds on and yields
[TABLE]
showing the contraction of the map ∎
4 The Cauchy Problem
In this section, we study the Cauchy problem:
[TABLE]
We will first assume that , we set .
Definition 4.1**.**
A pair is admissible if and
[TABLE]
Recall the following Strichartz estimates for the Schrödinger equation with potential are due to [4].
Proposition 4.1**.**
Let .
For any admissible pair , there exists such that
[TABLE] 2. 2.
Denote
[TABLE]
For all admissible pairs and , there exists such that
[TABLE]
for all and .
Proposition 4.2**.**
There exists such that if and are such that
[TABLE]
then (4.1) has a unique solution
[TABLE]
Proof of Proposition 4.2.
Let
[TABLE]
In view of Duhamel’s formula, and for , introduce the map
[TABLE]
From Strichartz inequalities
[TABLE]
By choosing sufficiently small, the right hand side does not exceed is stable under the action of . For the contraction, let :
[TABLE]
Up to decreasing again, the factor on the right hand side does not exceed and is a contraction on . This proves the existence part of the proposition. The uniqueness part readily follows from the remark that if , then can be split finitely many times on intervals where
[TABLE]
so uniqueness on can be deduced. ∎
Theorem 4.1**.**
Let . Then (4.1) has a unique, maximal solution
[TABLE]
Moreover, in :
[TABLE]
It is maximal in the sense that if is finite, then
[TABLE]
Proof.
Since , the homogeneous Strichartz inequality (2.1) implies , hence
[TABLE]
Moreover, Proposition 4.2 yields a local solution satisfying (4.1). For the notion of maximality, we proceed as in [2]. Suppose that , with finite, and that cannot be extended to larger time. Let and . Duhamel’s formula implies
[TABLE]
In view of the same inequality as in the proof of Proposition 5.1.
[TABLE]
The right hand side is less than if is close to . Proposition 4.3 shows that can be extended after , in contradiction with the definition of . ∎
Corollary 4.2**.**
If and , then , and for all ,
[TABLE]
Proof.
Form (5.1)
[TABLE]
hence
[TABLE]
and
[TABLE]
Therefore, for all finite,
[TABLE]
hence in Theorem 4.1. ∎
Corollary 4.3**.**
If and , then (4.1) has a unique, global solution , such that
[TABLE]
The analogue of Proposition 4.2 becomes, if we just assume :
Proposition 4.7. There exists such that if and are such that
[TABLE]
then (4.1) has a unique solution
[TABLE]
The proof is similar to the proof of Proposition 4.2, by working in
[TABLE]
and estimating
[TABLE]
Now, we still have (5.1), hence
[TABLE]
Therefore, the solution is global again.
5 Appendix: Proof of Proposition 3.3
Proof.
We start by proving (i). Consider the minimizing problem
[TABLE]
and observe that since , then .
On the one hand, arguing as in the proof of proposition 3.1, one can easily show that a minimizer of the above problem exists. Next, for any test function , we have
[TABLE]
That is
[TABLE]
Since is arbitrary and can have any sign, then we deduce that
[TABLE]
and therefore is an eigenvector of corresponding to the first (and simple) eigenvalue . On the other hand, it follows from Theorem 11.8 in [19] that the minimizer is unique and up to a phase change, we can take a positive minimizer with . Now, to conclude it suffices to show that . We see from that
[TABLE]
yielding (given that and are positive) . This finishes the proof.
Now we prove (ii). The proof of the bijectivity goes through several steps. First we prove Proposition 3.2. Set
[TABLE]
Then reads as
[TABLE]
Now we can decompose , where is the first simple eigenfunction of the operator , denotes an element of the vector space -orthogonal to , and is a scalar. Therefore, we have
[TABLE]
Now let us define the projection by: Thus, (5.2) can be rewritten in the following way
[TABLE]
and
[TABLE]
We will first solve (5.3) using the implicit function theorem.
First, we notice that for , and satisfying:
[TABLE]
,we have is a solution of (5.3). On the other hand,
[TABLE]
is invertible for . Thus, using the implicit function theorem, there exists a unique solving (5.3). Now we are going to solve (5.4) for .
We have , which after expansion, leads to
[TABLE]
that in partcicular yields
[TABLE]
by an appropriate choice of .
In summary, we can assert that there exists such that for all , there exist a unique solution solving (5.3)-(5.4). finishing the proof of Proposition 3.2.
Second, we consider the eigenvalue problem of the linearized operator around
[TABLE]
and track how the zero eigenvalue of moves for small values of . Note that since (and hence ) decays exponentially fast in space, the operator has a discrete spectrum with the same asymptotic of the eigenvalues as the Harmonic oscillator. Recalling that and with , equation (5.6) is rewritten as
[TABLE]
with , and .
When , we have , , and is a simple isolated eigenvalue of .
Taking the derivative with respect to , we obtain at :
[TABLE]
Multiplying the identity (5.7) by and taking the scalar product, we get
[TABLE]
(5.8) is strictly negative by identity (5.5). Therefore, \displaystyle\frac{d\lambda}{d\eta}\Big{|}_{\eta=0}<0.
Third, we show that for small masses , the ground state minimizing given by Lemma 2.2 is indeed equal to the unique given in proposition (3.2) by choosing . More precisely, it is sufficient to show that and , as where and .
To prove the latter assertion, let us first notice that
[TABLE]
This implies that as .
Additionally, (5.9) implies that is bounded in and satisfies
[TABLE]
Taking the weak limit in the latter inequality, we deduce that in as . Hence, choosing small enough; so that is in a neighborhood of in .
In the last part of the proof, we choose
[TABLE]
for yielding that is a zero of the functional .
∎
**Acknowledgement: ** S.I. was supported by NSERC grant (371637-2014). N. M was partially supported by NSF grant DMS-1716466. The authors would like to thank Peter Markowich for proposing them this problem, and are grateful to staff of King Abdullah University of Science and Technology for their great hospitality.
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