# Tracking the ultrafast motion of an antiferromagnetic order parameter

**Authors:** Christian Tzschaschel (1), Takuya Satoh (2), Manfred Fiebig (1), ((1) Department of Materials, ETH Zurich, Switzerland, (2) Department of, Physics, Kyushu University, Japan)

arXiv: 1903.08604 · 2019-09-06

## TL;DR

This study demonstrates direct measurement of the ultrafast dynamics of an antiferromagnetic order parameter using time-resolved optical techniques, revealing its temporal evolution and enabling better control of AFM spin states.

## Contribution

The paper introduces a novel method to directly track the ultrafast motion of an AFM order parameter via time-resolved SHG, overcoming previous measurement challenges.

## Key findings

- Direct observation of AFM order parameter dynamics in the time domain.
- Separation of electron and spin dynamics through symmetry analysis.
- General applicability of the method to other coherent excitations.

## Abstract

The unique functionalities of antiferromagnets offer promising routes to advance information technology. Their compensated magnetic order leads to spin resonances in the THz-regime, which suggest the possibility to coherently control antiferromagnetic (AFM) devices orders of magnitude faster than traditional electronics. However, the required time resolution, complex sublattice interations and the relative inaccessibility of the AFM order parameter pose serious challenges to studying AFM spin dynamics. Here, we reveal the temporal evolution of an AFM order parameter directly in the time domain. We modulate the AFM order in hexagonal YMnO$_\mathrm{3}$ by coherent magnon excitation and track the ensuing motion of the AFM order parameter using time-resolved optical second-harmonic generation (SHG). The dynamic symmetry reduction by the moving order parameter allows us to separate electron dynamics from spin dynamics. As transient symmetry reductions are common to coherent excitations, we have a general tool for tracking the ultrafast motion of an AFM order parameter.

## Full text

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## Figures

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## References

34 references — full list in the complete paper: https://tomesphere.com/paper/1903.08604/full.md

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Source: https://tomesphere.com/paper/1903.08604