Maltese Cross anisotropy in Ho0.8Lu0.2B12 antiferromagnetic metal with dynamic charge stripes

TL;DR

This study investigates the complex magnetic and electronic behaviors of Ho0.8Lu0.2B12, revealing a Maltese cross magnetic phase diagram and the role of dynamic charge stripes in its antiferromagnetic ground state.

Contribution

It uncovers the angular magnetic phase diagram as a Maltese cross and links charge stripe dynamics to symmetry lowering and magnetic phase diversity in Ho0.8Lu0.2B12.

Findings

Reconstructed magnetic phase diagram as a Maltese cross.

Identified charge stripe influence on magnetic symmetry.

Separated magnetoresistance contributions related to charge and spin fluctuations.

Abstract

The model strongly correlated electron system Ho0.8Lu0.2B12 which demonstrates a cooperative Jahn-Teller instability of the boron sub-lattice in combination with rattling modes of Ho(Lu) ions, dynamic charge stripes and unusual antiferromagnetic (AF) ground state has been studied in detail at low temperatures by magnetoresistance, magnetization and heat capacity measurements. Based on received results it turns out that the angular H-fi-T magnetic phase diagrams of this non-equilibrium AF metal can be reconstructed in the form of a Maltese cross. The dramatic AF ground state symmetry lowering of this dodecaboride with fcc crystal structure can be attributed to the redistribution of conduction electrons which leave the RKKY oscillations of the electron spin density to participate in the dynamic charge stripes providing with extraordinary changes in the indirect exchange interaction between magnetic moments of Ho3+ ions and resulting in the emergence of a number of various magnetic phases. It is also shown that the two main contributions to magnetoresistance in the complex AF phase, the (i) positive linear on magnetic field and the (ii) negative quadratic component can be separated and analyzed quantitatively, correspondingly, in terms of charge carrier scattering on spin density wave (5d) component of the magnetic structure and on local 4f-5d spin fluctuations of holmium sites.