Enhanced Gilbert Damping in Re doped FeCo Films: A Combined Experimental and Theoretical Study

TL;DR

This study investigates how Re doping in FeCo thin films affects their magnetic properties, showing increased damping and decreased magnetization, supported by both experimental measurements and first principles calculations.

Contribution

It provides a combined experimental and theoretical analysis of Re doping effects on magnetic damping and saturation magnetization in FeCo films, highlighting the microscopic origin of damping enhancement.

Findings

Saturation magnetization decreases with Re doping.

Gilbert damping parameter increases with Re doping.

Theoretical and experimental damping values are in good agreement.

Abstract

The effects of rhenium doping in the range 0 to 10 atomic percent on the static and dynamic magnetic properties of Fe65Co35 thin films have been studied experimentally as well as with first principles electronic structure calculations focusing on the change of the saturation magnetization and the Gilbert damping parameter. Both experimental and theoretical results show that the saturation magnetization decreases with increasing Re doping level, while at the same time Gilbert damping parameter increases. The experimental low temperature saturation magnetic induction exhibits a 29 percent decrease, from 2.31 T to 1.64 T, in the investigated doping concentration range, which is more than predicted by the theoretical calculations. The room temperature value of the damping parameter obtained from ferromagnetic resonance measurements, correcting for extrinsic contributions to the damping, is for the undoped sample 0.0027, which is close to the theoretically calculated Gilbert damping parameter. With 10 atomic percent Re doping, the damping parameter increases to 0.0090, which is in good agreement with the theoretical value of 0.0073. The increase in damping parameter with Re doping is explained by the increase in density of states at Fermi level, mostly contributed by the spin-up channel of Re. Moreover, both experimental and theoretical values for the damping parameter are observed to be weakly decreasing with decreasing temperature.