# Interrupted Motility Induced Phase Separation in Aligning Active Colloids

## TL;DR

This study investigates the dynamics of phase separation in active Janus colloids, revealing how particle alignment interrupts the process and introduces new physics in active matter systems.

## Contribution

It provides the first large-scale experimental observation of phase separation kinetics in active colloids with alignment and short-range repulsions.

## Key findings

- Identification of three dynamical regimes during phase separation.
- Alignment between particles causes the interruption of phase separation.
- Characterization of structural ordering and cluster dynamics.

## Abstract

Switching on high activity in a relatively dense system of active Janus colloids, we observe fast clustering, followed by cluster aggregation towards full phase separation. The phase separation process is however interrupted when large enough clusters start breaking apart. Following the cluster size distribution as a function of time, we identify three successive dynamical regimes. Tracking both the particle positions and orientations, we characterize the structural ordering and alignment in the growing clusters and thereby unveil the mechanisms at play in these regimes. In particular, we identify how alignment between the neighboring particles is responsible for the interruption of the full phase separation. This experimental study, which provides the first large scale observation of the phase separation kinetics in active colloids, combined with single particle analysis of the local mechanisms, points towards the new physics observed when both alignment and short-range repulsions are present.