# Direct photoluminescence probing of ferromagnetism in monolayer   two-dimensional CrBr3

**Authors:** Zhaowei Zhang, Jingzhi Shang, Chongyun Jiang, Abdullah Rasmita, Weibo, Gao, and Ting Yu

arXiv: 1902.07446 · 2019-05-22

## TL;DR

This paper demonstrates intrinsic ferromagnetism in monolayer CrBr3 using polarization-resolved magneto-photoluminescence, revealing persistent magnetization at 34 K and insights into magnetic domain structures, advancing 2D spintronics research.

## Contribution

It provides direct optical evidence of ferromagnetism in monolayer CrBr3 and explores its magnetic properties and domain behavior, a novel insight for 2D magnetic materials.

## Key findings

- Ferromagnetism persists in monolayer CrBr3 with a Curie temperature of 34 K.
- Magneto-photoluminescence reveals intrinsic magnetic properties.
- Layer-dependent hysteresis linked to magnetic domain structures.

## Abstract

Atomically thin magnets are the key element to build up spintronics based on two-dimensional materials. The surface nature of two-dimensional ferromagnet opens up opportunities to improve the device performance efficiently. Here, we report the intrinsic ferromagnetism in atomically thin monolayer CrBr3, directly probed by polarization resolved magneto-photoluminescence. The spontaneous magnetization persists in monolayer CrBr3 with a Curie temperature of 34 K. The development of magnons by the thermal excitation is in line with the spin-wave theory. We attribute the layer-number dependent hysteresis loops in thick layers to the magnetic domain structures. As a stable monolayer material in air, CrBr3 provides a convenient platform for fundamental physics and pushes the potential applications of the two-dimensional ferromagnetism.

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Source: https://tomesphere.com/paper/1902.07446