2D Semiconductor Nonlinear Plasmonic Modulators
Matthew Klein, Bekele H. Badada, Rolf Binder, Adam Alfrey, Max McKie,, Michael R. Koehler, David G. Mandrus, Takashi Taniguchi, Kenji Watanabe,, Brian J. LeRoy, and John R. Schaibley

TL;DR
This paper introduces the first 2D semiconductor nonlinear plasmonic modulator using WSe2 monolayer, achieving significant transmission change and ultralow switching energy through strong exciton-SPP coupling.
Contribution
It demonstrates a novel 2D semiconductor-based nonlinear plasmonic modulator with high modulation depth and ultralow energy, advancing plasmonic device technology.
Findings
73% change in transmission achieved
Modulation depth of 4.1% demonstrated
Ultralow switching energy of 40 aJ estimated
Abstract
A plasmonic modulator is a device that controls the amplitude or phase of propagating plasmons. In a pure plasmonic modulator, the presence or absence of a pump plasmonic wave controls the amplitude of a probe plasmonic wave through a channel. This control has to be mediated by an interaction between disparate plasmonic waves, typically requiring the integration of a nonlinear material. In this work, we demonstrate the first 2D semiconductor nonlinear plasmonic modulator based on a WSe2 monolayer integrated on top of a lithographically defined metallic waveguide. We utilize the strong coupling between the surface plasmon polaritons, SPPs, and excitons in the WSe2 to give a 73 percent change in transmission through the device. We demonstrate control of the propagating SPPs using both optical and SPP pumps, realizing the first demonstration of a 2D semiconductor nonlinear plasmonic…
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