Counterflowing edge current and its equilibration in quantum Hall devices with sharp edge potential: Roles of incompressible strips and contact configuration
T. Akiho, H. Irie, K. Onomitsu, and K. Muraki

TL;DR
This study observes counterflowing edge currents in InAs quantum wells causing quantum Hall effect breakdown at high magnetic fields, highlighting the roles of incompressible strips and contact configuration in edge state equilibration.
Contribution
It provides the first detailed measurement of counterflowing edge modes and their equilibration length in InAs quantum wells, emphasizing the influence of incompressible strips and contact setup.
Findings
Counterflowing edge channels cause QH breakdown at high fields.
Equilibration length increases exponentially with magnetic field.
Contact configuration significantly affects edge state transport.
Abstract
We report the observation of counterflowing edge current in InAs quantum wells which leads to the breakdown of quantum Hall (QH) effects at high magnetic fields. Counterflowing edge channels arise from the Fermi-level pinning of InAs and the resultant sharp edge potential with downward bending. By measuring the counterflow conductance for varying edge lengths, we determine the effective number of counterflowing modes and their equilibration length at bulk integer filling factor --. increased exponentially with magnetic field , reaching m for at ~T. Our data reveal important roles of the innermost incompressible strip with even filling in determining and and the impact of the contact configuration on the QH effect breakdown.…
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Counterflowing edge current and its equilibration in quantum Hall devices with sharp edge potential: Roles of incompressible strips and contact configuration
T. Akiho, H. Irie, K. Onomitsu, and K. Muraki
NTT Basic Research Laboratories, NTT Corporation, 3-1 Morinosato-Wakamiya, Atsugi 243-0198, Japan
Abstract
We report the observation of counterflowing edge current in InAs quantum wells which leads to the breakdown of quantum Hall (QH) effects at high magnetic fields. Counterflowing edge channels arise from the Fermi-level pinning of InAs and the resultant sharp edge potential with downward bending. By measuring the counterflow conductance for varying edge lengths, we determine the effective number of counterflowing modes and their equilibration length at bulk integer filling factor –. increased exponentially with magnetic field , reaching m for at T. Our data reveal important roles of the innermost incompressible strip with even filling in determining and and the impact of the contact configuration on the QH effect breakdown. Our results show that counterflowing edge channels manifest as transport anomalies only at high fields and in short edges. This in turn suggests that, even in the integer QH regime, the actual microscopic structure of edge states can differ from that anticipated from macroscopic transport measurements, which is relevant to various systems including atomic-layer materials.
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Understanding and controlling the electronic states at the edge of a two-dimensional system are becoming increasingly important. This is particularly true for topologically nontrivial systems, such as quantum Hall (QH) Halperin (1982); Streda et al. (1987); Büttiker (1988) and quantum spin Hall Kane and Mele (2005a, b) systems, where gapless edge states with distinct properties appear. Recent theories Lindner et al. (2012); Vaezi (2013); Clarke et al. (2013); Mong et al. (2014); Clarke et al. (2014) predict that, by coupling their edge states to superconductors, QH as well as quantum spin Hall systems can be exploited to engineer exotic quasiparticles with non-Abelian statistics, a building block for robust quantum computation Alicea (2012); Leijnse and Flensberg (2012). Semiconductor heterostructures comprising InAs, which can form transparent junctions with superconductors Knez et al. (2012); Pribiag et al. (2015); De Vries et al. (2018), are promising for such purposes. Theory further predicts that certain fractional QH edge states coupled through a superconductor may harbor even more exotic quasiparticles that would allow for universal topological quantum computation Lindner et al. (2012); Vaezi (2013); Clarke et al. (2013); Mong et al. (2014); Clarke et al. (2014). Motivated by these predictions, recently the quality of InAs-based heterostructures has been improved significantly Tschirky et al. (2017); Thomas et al. (2018), which has led to the observation of a fractional QH effect Ma et al. (2017).
In standard GaAs-based heterostructures, the edge potential is bent upward by the Fermi-level pinning in the band gap so that the electron density decreases monotonically toward the edge Halperin (1982); Chklovskii et al. (1992). This forms the basis for the common situation in QH systems where all edge channels have the same chirality, flowing in the same direction set by the magnetic field 111 In the fractional QH regime, electron correlation can lead to an edge state with a non-monotonic density profile and counterflowing modes, which is outside the scope of this work. See Ref. Lafont et al. (2019) and references therein. . In contrast, in InAs the surface pinning occurs in the conduction band Waldrop (1984); Noguchi et al. (1991), which implies that in heterostructures the edge potential is bent downward so the electron density increases near the edge. While this is advantageous for superconducting junctions, it gives rise to trivial edge conduction with no topological origin at zero magnetic field Nichele et al. (2016); Nguyen et al. (2016); Mueller et al. (2017); Mittag et al. (2017); De Vries et al. (2018). In a quantizing magnetic field, this suggests that the Fermi level can cross Landau levels extra times (see the inset to Fig. 1), where additional sets of edge channels running in the forward and counterflow directions form van Wees et al. (1995). As recently revealed in graphene Cui et al. (2016), a similar situation can also occur in a gated device due to electric-field focusing near the edge Silvestrov and Efetov (2008).
Counterflowing edge channels were first conceived by van Wees et al. van Wees et al. (1995), who observed in their InAs quantum well that QH effects collapsed when a negative gate voltage below a certain threshold ( V) was applied. The results were then explained using the Landauer-Büttiker model Büttiker (1988), taking into account the scattering between forward and counterflowing edge channels, which indicated a typical equilibration length in excess of m. However, it remains unknown what determines the equilibration length and how it depends on the parameters such as the magnetic field and filling factor. In this paper, we address these issues by systematically studying QH edge transport in InAs quantum wells using gated Hall-bar devices with only well-defined edges. We directly detect the upstream charge current using a three-terminal setup, which allows us to determine the effective number of counterflowing modes and their equilibration length. Our data reveal important roles of the innermost incompressible strip with even filling and the impact of the contact configuration for the counterflowing edge channels to manifest in transport. Our results provide new insights into microscopic details of QH edge states, which will be useful for understanding edge transport in various systems including atomic-layer materials and in superconducting junctions, not only in the QH but also in the quantum spin Hall setups.
The heterostructure studied was grown by molecular beam epitaxy on an -type GaSb (001) substrate. The layer structure comprises a 20-nm-thick InAs quantum well sandwiched between Al0.7Ga0.3Sb barriers, with no intentional doping to supply carriers. The center of the well is located nm below the surface of the 5-nm-thick GaSb cap. The heterostructure was processed into -m-wide Hall bars as shown in the inset of Fig. 1 by wet etching. We fabricated devices with ten Ti/Au Ohmic electrodes and a Ti/Au gate on an atomic-layer-deposited 40-nm-thick Al2O3 insulator. The gate covers all the mesa edges and their interface with Ohmic contacts, so that all the edges are defined in the same way. The sample had sheet electron density of m*-2* and low-temperature mobility of m2/Vs. We used two samples fabricated from the same wafer, sample A with all edges having the same length of m and sample B with varying (–m). Measurements were done at K using a standard lock-in technique.
We first present results for sample A. Figure 1 shows the magnetic field () dependence of the longitudinal resistance () at front gate voltage V, measured using different pairs of voltage probes on the lower edge of the sample. At T, we observe normal behavior—Shubnikov-de Haas oscillations and well-developed QH effect at Landau-level filling factor —for all configurations. ( with the elementary charge and Planck’s constant). In contrast, anomalous behavior is seen at T, where the QH effects expected at and are not fully developed or completely missing, as seen by the non-vanishing . Interestingly, the values of the finite at and systematically depend on the field direction and probe position. At , measured with the lower-right probes () is much higher for than for . Opposite behavior is seen for measured with the lower-left probes (), which is much higher for . The lower-middle probes () gives intermediate values nearly symmetric for both field directions. Although not shown, measurements using the probes on the upper edge confirm similar behavior, but with the probe-position dependence rotated around the sample normal. We show below that this chiral breakdown behavior of the QH effect can be explained by the Landauer-Büttiker model that takes into account the scattering between forward and counterflowing edge channels.
We demonstrate the existence of counterflowing charge current using the three-terminal measurements as illustrated in Fig. 2(a), which in turn allowed us to directly determine the number of counterflowing modes () and their transmission probability () for individual edges. In order to examine the dependence of , we used sample B with varying (–m). A magnetic field was applied in the direction so that the chirality of the edge channels was clockwise. With this three-terminal setup, we detected charge current at the probe located on the upstream of the electrode from which current ( nA) was driven, in addition to normal forward current measured on its downstream. To check the conduction through the bulk, we also monitored current on the opposite side of the Hall bar. In the QH regime, where the current cannot flow through the bulk, the chirality requires and . As shown in Fig. 2(b), we observe that this holds only at – T. At T, is seen to be noticeably lower than at fields where is vanishing, accompanied by a significant increase in . This observation of upstream charge current in the QH regime provides direct evidence for the existence of counterflowing edge channels.
Using the voltage applied to drive and measured currents and in the QH regime, we define the conductance in the forward and counterflow directions as and for the edges on the downstream and upstream labeled and , respectively, in units of conductance quantum . In the Landauer-Büttiker model Büttiker (1988); van Wees et al. (1995) can be expressed as , where is the transmission probability of the counterflowing mode of the edge on the upstream labeled . Note that there are forward edge channels in the presence of counterflowing edge channels. Detailed balance requires for each edge 222 Detailed balance requires for each edge, where is the transmission probability of the forward modes on the th edge. By solving this for and pluging it into , we have . . In what follows, we therefore show only results for . We repeated similar three-terminal measurements using the same sample while sequentially changing the injector and detector contacts, which allowed us to evaluate for different edges. Figure 2(c) shows for different , obtained while sweeping at a fixed magnetic field of T. The top axis shows the bulk filling factor determined from the low-field Shubnikov-de Haas oscillations and Hall measurements at each . We note that oscillates with , but with the positions of the minima shifted from the bulk integer filling to lower 333 The fact that decreases as is slightly lowered from integer is consistent with the conjecture that the electron density in the vicinity of the mesa edge is higher than that in the bulk.
As Fig. 2(c) shows, decreases with increasing for all . In the following we restrict our analysis to the values at integer bulk filling [shown by symbols in Fig. 2(c)], where we confirmed the absence of bulk conduction. In Fig. 2(d), we plot () at T as a function of for –4. The data were then fitted with a single exponential function using and as fitting parameters. As is expected for , we see that . We therefore use instead of to represent the effective number of counterflowing modes deduced from the fitting. For , we obtain and m at T.
We performed similar measurements and analysis for a range of magnetic fields (–8 T). The results are summarized in Fig. 3, where and obtained for – are plotted as a function of . For all , monotonically increases with increasing [Fig. 3(a)] and hence (inset) 444 For and , only data for T, for which good fitting with the exponential function was obtained, are included. . This suggests that the distance between the forward and counterflowing edge channels increases with , which reduces the scattering between them. At high fields, for and reaches m, the value reported in Ref. van Wees et al., 1995. Interestingly, increases with and peaks out below for and , whereas it exceeds and then levels off below for and [Fig. 3(b)] 555 Note that is the effective number of counterflowing modes, not the actual number of counterflowing edge channels determined by the density profile and magnetic field. In addition, disorder may affect the value of ; potential fluctuation near the edge may cause to vary between and (or between and [math]) along the edge, making non-integer. .
To gain insight into the dependence of and the even-odd behavior of , we simulated the density profile near the mesa edge by solving the Poisson equation self-consistently within the semiclassical approach taking only Landau quantization into account 666The Poisson equation was solved in the two-dimensional plane perpendicular to the sample edge. We employed a simplified geometry, with a -nm-wide zero-thickness channel surrounded by -nm-thick insulator with a dielectric constant of and a metallic gate in all four directions. Effective mass of and -factor of 10 were used to calculate the energies of the Landau levels, which were then broadened by a Gaussian function with meV. Finite-temperature effects were not included. A fixed line charge of nm*-1* along the channel edge was assumed to obtain realistic density profiles. . In Fig. 4, we compare the density profiles for (a) and (b) at the same bulk density of m*-2*. In both cases, density increases toward the edge, where it drops sharply to zero. Notably, density varies in a stepwise manner due to the formation of compressible and incompressible strips Chklovskii et al. (1992). As the charge equilibration between adjacent edge channels occurs via scattering across the incompressible strip between them Alphenaar et al. (1990); Cui et al. (2016), its width is the important parameter determining the scattering rate. The width is determined by the density gradient at and the Landau-level energy separation at the strip Chklovskii et al. (1992), the latter being the cyclotron and Zeeman energy for even and odd local filling (), respectively. Our simulations reveal an important role played by the innermost incompressible strip with even . For odd bulk filling , the one with is the widest [Fig. 4(a)], reflecting the small density gradient (at ) and the large cyclotron gap, which then isolates one inner counterflowing channel from all other channels. The outer counterflowing channels are very close to the forward channels and easily equilibrated with them. This explains why only one counterflowing mode can transmit for odd . In contrast, for , the widest incompressible strip develops at [Fig. 4(b)], which isolates two inner counterflowing channels, allowing more than one counterflowing modes to transmit. The dependence of can be understood in terms of the incompressible-strip width, which we discuss later in detail.
Now we discuss the probe-position and field-direction dependence of the QH effect breakdown presented in Fig. 1. Using the Landauer-Büttiker model, we calculate as a function of for the configuration shown in Fig. 5(a). The current-voltage relation can be expressed as , where and with () the current (voltage) of the th contact (–) Cui et al. (2016). is a matrix with non-zero elements given by
[TABLE]
(), where is the transmission probability of the forward mode on the th edge. Scattering between forward and counterflowing modes is described by the detailed balance as . Since all the edges have the same length in the present case, we assume that they share the same and values. We then solved the above equations with , , and .
The dependence of calculated for and is shown in Fig. 5(b). For these calculations, we took , for comparison with the experiment at V [Fig. 3(b)]. The experimental data taken from Fig. 1 are plotted in Fig. 5(b) against [] calculated using for and at V [Fig. 3(a)]. Since the model predicts , we included in Fig. 5(b) the data for using this relation. The calculation reproduces the experimentally observed probe-position dependence, for , including the quantitative values. We note that at V the equilibration lengths for and ( and m, respectively) are comparable to (m). Hence, the counterflowing mode, being not fully equilibrated with the forward mode, carries charge to the electrode on the upstream and destroys the QH effect. In contrast, m for at V is much shorter than , implying a nearly full equilibration 777 Indeed, for yields .. This explains why the QH effect is well developed at V, despite the presence of the counterflowing edge channels.
The probe-position and field-direction dependence can be understood intuitively by considering hot spots Klaß et al. (1991); Komiyama et al. (2006). In the absence of counterflowing modes, the chemical potential of a forward mode just follows that of the current terminal on its upstream. Consequently, all the applied bias between the source and drain contacts is concentrated at the two corners where the forward mode meets the source and drain contacts (“hot spots”) [Fig. 5(a)]. In contrast, the chemical potential of the counterflowing mode follows primarily that of the electrode on its immediate downstream. Therefore, the largest chemical potential difference between the forward mode and counterflowing one occurs near the immediate upstream of the hot spots, yielding the chiral QH breakdown behavior.
We now turn to the dependence of . As shown in Fig. 3(a), increases exponentially with for both even and odd , with nearly the same slope. The inter-edge-channel scattering rate is governed by the wave function overlap between the states involved, which scales as , where is the inter-edge distance and is the magnetic length. If is given by the width of the innermost incompressible strip with even , it is proportional to the square root of the cyclotron energy Chklovskii et al. (1992) and hence scales as . Since in this case, one expects , with a constant Martin and Feng (1990). The experimentally observed dependence, , is different 888 Similar exponential dependence is known for co-propagating edge channels in GaAs, which was observed when was varied around integer fillings at a fixed density and explained by the increase in the inter-edge distance with decreasing Chklovskii et al. (1992). In the present case, drops more quickly with as is slightly reduced from integer values [Fig. 2(c)], suggesting that the inter-edge distance becomes smaller with decreasing , suggesting the relevance of multiple scattering with impurities Martin and Feng (1991).
Several differences between our results and the previous ones reported for InAs van Wees et al. (1995) and graphene Cui et al. (2016) are worth noting. In Ref. van Wees et al., 1995, (i) was non-zero only for V, and (ii) increased linearly up to with decreasing . In our experiment, does not show a monotonic dependence, being non-zero for both and , with the maximum value peaked out below . The chemical properties of the edge Mittag et al. (2017) and the relative distances of the bulk and edge to the gate 999 Although not shown here, our experiments suggest that the edge potential depends also on other factors such as the quantum well thickness, distance from the surface, and the history of gate sweep, which will be reported separately. may partly account for these differences. However, as our simulations show, the outer counterflowing channels are spatially very close to the forward channels, making it rather unlikely for many of them to transmit 101010 It is not clear whether the large values found in Ref. van Wees et al., 1995 originate from the various assumptions made in the analysis. Our approach, in which one directly measures the counterflowing charge current for each individual edge, provides reliable values for and . . In Ref. Cui et al., 2016, despite significant charge accumulation at the edges, QH effects were observed, but at gate voltages shifted from the integer bulk filling. In the edge-state picture, the transport quantization was explained as resulting from strong scattering between forward and counterflowing channels (i.e., short ) and their isolation from the conductive bulk by the incompressible strip 111111 This happens only when the incompressible strip isolates the bulk from Ohmic contacts. Whether this happens or not depends on the density profile near Ohmic contacts Dahlem et al. (2010). . The microscopic structure of the edge states is non-trivial also in this case, which must be taken into account when making a superconducting junction Amet et al. (2016); Lee et al. (2017).
In summary, we investigated counterflow edge transport in InAs quantum wells in the QH regime and clarified how it equibrates or manifests as transport anomaly depending on the magnetic field, filling factor, and contact configuration. Our results suggest that counterflowing edge channels can exist in various systems with sharp edge potential. Thus, even in the integer QH regime, the microscopic structure of edge states and hence the transport phenomena therein can be more complex than naively expected from the bulk-edge correspondence and should be carefully studied.
The authors thank Yasuhiro Tokura and Masayuki Hashisaka for fruitful discussions and Hiroaki Murofushi for processing the devices. This work was supported by JSPS KAKENHI Grant No. JP15H05854.
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