Anomalous Nonlocal Conductance as a Fingerprint of Chiral Majorana Edge States
Satoshi Ikegaya, Yasuhiro Asano, and Dirk Manske

TL;DR
This paper proposes a definitive experimental method to detect chiral Majorana edge states via anomalous nonlocal conductance measurements in a device with a chiral p-wave superconductor and ferromagnetic leads, highlighting their unique long-range and directional transport properties.
Contribution
It introduces a theoretical framework for a smoking-gun experiment to identify chiral Majorana edge states through nonlocal conductance signatures in a specific device setup.
Findings
Chiral Majorana edge states cause long-range nonlocal conductance.
Nonlocal conductance is sensitive to the chirality of edge states.
The proposed experiment can determine the direction of edge state propagation.
Abstract
Chiral -wave superconductor is the primary example of topological systems hosting chiral Majorana edge states. Although candidate materials exist, the conclusive signature of chiral Majorana edge states has not yet been observed in experiments. Here we propose a smoking-gun experiment to detect the chiral Majorana edge states on the basis of theoretical results for the nonlocal conductance in a device consisting of a chiral -wave superconductor and two ferromagnetic leads. The chiral nature of Majorana edge states causes an anomalously long-range and chirality-sensitive nonlocal transport in these junctions. These two drastic features enable us to identify the moving direction of chiral Majorana edge states in the single experimental setup.
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Anomalous Nonlocal Conductance as a Fingerprint of Chiral Majorana Edge States
Satoshi Ikegaya1
Yasuhiro Asano2,3,4
Dirk Manske1
1Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, D-70569 Stuttgart, Germany
2Department of Applied Physics, Hokkaido University, Sapporo 060-8628, Japan
3Center of Topological Science and Technology, Hokkaido University, Sapporo 060-8628, Japan
4Moscow Institute of Physics and Technology, 141700 Dolgoprudny, Russia
Abstract
Chiral -wave superconductor is the primary example of topological systems hosting chiral Majorana edge states. Although candidate materials exist, the conclusive signature of chiral Majorana edge states has not yet been observed in experiments. Here we propose a smoking-gun experiment to detect the chiral Majorana edge states on the basis of theoretical results for the nonlocal conductance in a device consisting of a chiral -wave superconductor and two ferromagnetic leads. The chiral nature of Majorana edge states causes an anomalously long-range and chirality-sensitive nonlocal transport in these junctions. These two drastic features enable us to identify the moving direction of chiral Majorana edge states in the single experimental setup.
pacs:
74.45.+c, 74.25.F-, 74.70.Pq
††preprint: APS/123-QED
Introduction and main idea.—Superconductors (SCs) with spin-triplet chiral -wave pairing symmetry have attracted intensive attention for the past two decades because they exhibit topologically protected chiral Majorana edge states (CMESs) having great potential applications to topological quantum computations green_00 ; ivanov_01 . According to a range of experimental maeno_94 ; maeno_98 ; ishida_98 ; maeno_04 ; maeno_06 and theoretical rice_95 ; yanase_03 ; wang_13 evidence, the perovskite superconductor Sr2RuO4 is the most promising candidate for the spin-triplet chiral -wave SCs. At present, finding a smoking-gun signature of CMESs in this compound is an on-going and central subject in both physics of topological condensed matter kane_r10 ; zhang_r11 ; sato_r17 and that of spin-triplet superconductivity maeno_r03 ; maeno_r12 ; kallin_r12 .
There have been three standard directions for the detection of CMESs. The first direction is by measurements of internal magnetic fields due to the spontaneous edge current sigrist_99 ; furusaki_01 ; stone_04 ; asano_16 . However, the scanning SQUID experiments for Sr2RuO4 did not detect the expected fields moler_05 ; nelson_07 because of either the screening currents in the bulk sigrist_99 or for other reasons sigrist_14 ; kallin_15 ; simon_15 . The second direction is by use of phenomena analogous to the quantum Hall effect in a two-dimensional electron gas with applied magnetic fields klitzing_80 ; thouless_82 : the spin quantum Hall effect fisher_99 and thermal quantum Hall effect vishwanath_01 . However, these effects have not been observed yet because of difficulties in spin and thermal transport measurements. The third direction studies anomalies in local charge transport of superconducting junctions, such as a zero-bias conductance peak in tunneling spectroscopy kashiwaya_97 and a low-temperature anomaly in Josephson currents asano_02 . However, roughly speaking, these anomalies can be induced by any type of mid-gap Andreev bound states and are not unique to the CMESs. Therefore, unfortunately, the zero-bias conductance peak observed in a planar tunneling experiment for Sr2RuO4 kashiwaya_11 cannot be the conclusive evidence for the CMESs.
To resolve this stalemate, in the present Letter, we propose a novel experiment that provide a smoking-gun signature of CMESs though charge transport measurements. The central ingredient of our scheme is that we measure nonlocal charge transport in the presence of CMESs beenakker_10 . We will use a setup as shown in Fig. 1, where two ferromagnetic (FM) leads are attached to an edge of a chiral -wave SC tserkovnyak_18 . The nonlocal conductance in a similar device with replacing the chiral -wave SC by a conventional -wave SC has been already studied deutscher_00 ; yamashita_03 . In such a device the nonlocal conductance is governed by two distinctive nonlocal transport processes yielding opposite contributions: an incident electron from one lead is scattered into another lead as an electron (elastic co-tunneling process) or a hole (crossed Andreev reflection process). The exchange potential in the FM leads is source of finite nonlocal conductance because it generates the imbalance between these two nonlocal transport processes deutscher_00 ; yamashita_03 . With conventional -wave SC, the subgap nonlocal conductance is strongly suppressed when the distance between the two leads exceeds the superconducting coherent length. This is because that incident electrons must tunnel from one lead to the other through evanescent waves of Bogoliubov quasi-particles in the superconducting segment. However, we expect that CMESs modify the situation drastically such that the CMESs moving in the direction from lead to mediate the nonlocal transport from lead to irrespective of the distance between the two leads, while it does not assist the nonlocal transport from lead to (See also Fig. 1). If we can capture such unusual anisotropy in the nonlocal transport processes, it can be a smoking-gun signature of the CMESs.
We calculate two types of nonlocal differential conductance and by using the lattice Green function technique. Here, is the current response in the FM lead due to the application of the bias voltage to the electrode attached to the FM lead , while the electrodes attached to the FM lead and superconductor are grounded. We will demonstrate that spectrum of and indeed exhibit the distinctive contrast reflecting the chiral motion of CMESs. Namely, when the CMESs move in the direction from the lead to , the nonlocal conductance becomes finite irrespective of the distance between the FM leads [See Fig. 2 (a)], while the nonlocal conductance becomes almost zero [See Fig. 2 (b)]. We can measure both and only by changing the lead wire to which the bias-voltage is applied. Therefore, we can identify the moving direction of the CMES in the single experimental setup. The remarkable advantage of our proposal is that we only need the obvious difference in and , where one of them is finite and the other is zero, to identify the CMESs in the chiral -wave superconductor conclusively.
Minimal model.—Let us consider the junction illustrated in Fig. 1 on a two dimensional tight-binding model with the lattice constant . A lattice site is indicated by a vector , where () is the vector in the () direction with . The chiral -wave SC occupies and , where its width is given by . In the direction, we apply the hard-wall boundary condition. The FM lead 1 (FM lead 2) is placed on and (), where its width is denoted by . The distance between the two FM leads is given by . The present device is described by the Bogoliubov-de Gennes Hamiltonian . In this paper, we phenomenologically describe the chiral -wave SC by using the standard minimal model
[TABLE]
where , , , and with () representing the creation (annihilation) operator of an electron at the site with spin ( or . The Pauli matrices in spin space are represented by for , and the unit matrix is denoted with . and respectively denote the nearest-neighbor hopping integral and chemical potential in the superconductor. The amplitude and chirality of the pair potential are represented by and ( or ), respectively. The pair potential for a spin-triplet pairing symmetry in momentum space is generally described as . In this Letter, we use the -vector of , which is the most probable one in Sr2RuO4 rice_95 ; yanase_03 ; maeno_r03 ; maeno_r12 ; kallin_r12 . Here, () represents the wave number along the () direction, and represents the unit vector in the -direction corresponding to the -axis of Sr2RuO4. The FM lead (, ) is described by
[TABLE]
where , . The nearest-neighbor hopping integral and chemical potential in the FM leads are respectively denoted and . The exchange potential in the FM lead is given by . In what follows, we fix several parameters as , , , , and . In the tight-binding model, the superconducting coherent length is given by lee_10 . With our parameter choice, we obtain . The chiral -wave SC hosts two CMESs originated from the two different spin-sectors. With , both of them move along the edge at in the direction from the FM lead 1 to 2.
We are interested in the nonlocal differential conductance and . On the basis of the Blonder-Tinkham-Klapwijk (BTK) formalism klapwijk_82 , the nonlocal conductance at zero temperature is given by deutscher_00 ; yamashita_03 ; pachos_08 ; pablo_15 ; mukerjee_17 ; alidoust_17 ; akhmerov_18 ; cheng_18
[TABLE]
with . The elastic co-tunneling (EC) and crossed Andreev reflection (CAR) coefficients at energy are respectively denoted by and , where the index () labels the outgoing (incoming) channel in the FM lead (FM lead ). These reflection coefficients are obtained by using the lattice Green function technique fisher_81 ; ando_91 (See Supplemental Material for the detailed calculation). In the BTK formalism, we assume that all currents following towards () in the superconductor (FM lead ) are absorbed into the ideal electrode which is not describe in the Hamiltonian explicitly. We note that the BTK formalism is quantitatively justified for bias voltages well below the superconducting gap.
Results on nonlocal conductance.—We first focus on the nonlocal conductance . In Fig. 2(a), we show as a function of the bias voltage and distance between the FM leads . We choose the parameters as and . We vary from to , where . For the FM leads, we consider the antiparallel magnetization along axis, where with . We find that for is almost independent of and is finite for . Specifically, at zero-bias voltage, we find irrespective of . The anomalously long-range nonlocal transport in the present junction suggests that wave functions in the two different FM leads are mediated not by evanescent waves but by the propagating waves of CMESs. We will later confirm this statement by analyzing the wave functions in the present junction. Next, we discuss the nonlocal conductance . In Fig. 2(b), we show as a function of the bias voltage and , where the parameters are chosen as same as those in Fig. 2(a). In contrast to , we find that with is almost zero for all . This suggests that the CMESs moving in the direction from the lead 1 to 2 cannot assist the nonlocal transport processes from the lead 2 to 1. In the BTK formalism, we assume that the CMESs moving towards is absorbed into the ideal electrode attached to the superconductor. To support this assumption, we also calculate the reflection and transmission probabilities at an ideal chiral -wave SC/normal-metal interface, and confirm that the incident CMESs are always scattered into the attached normal-metal(See Supplemental Material for the detailed calculation). We confirm that the spectrum of and that of are replaced each other by changing the sign of chirality from to . Thus, the distinctive contrast between and is indeed related with the moving direction of the CMESs. We can measure both and by changing the FM lead wire to which the bias voltage is applied. Therefore, by comparing and , we can test the sign of chirality, and therefore the moving direction of CMESs, in the single experimental setup.
We now discuss the exchange potential dependence of the nonlocal conductance. In Fig. 3(a), we show the nonlocal conductance at zero-bias voltage as a function of the exchange potential amplitude. We here consider either parallel or antiparallel alignment of magnetization along the -axis with and . With this representation, the parallel (antiparallel) alignments of the magnetization is described with (). We choose the parameters as , and . For the antiparallel () and parallel () magnetization, respectively becomes positive and negative finite, which leads to the relation of () with the antiparallel (parallel) magnetization. When the -vector in the superconductor is parallel or antiparallel to the magnetic moment in the FM leads, Andreev reflection occurs between electron and hole states with opposite spins, while normal reflection occurs between equal-spin electrons yoshida_99 ; hirai_01 ; hirai_03 . Therefore, the antiparallel magnetization in the FM leads suppresses the equal-spin scattering process of EC, while it does not damage the CAR process. On the other hand, the parallel magnetization in the FM leads does not damage the EC process, while it disturbs the spin flip in the CAR process. This roughly explains the relation of () with the antiparallel (parallel) magnetization. In the absence of the exchange potential (), the nonlocal conductance becomes zero due to the complete cancellation between the contributions from the EC and CAR processes (i.e., ). When exceeds , only the spin- states remain at the Fermi level in the FM lead 1 and the only spin- (-) states remain at the Fermi level in the FM lead 2 with the antiparallel (parallel) alignment of magnetization. Within such half-metallic limit (), we obtain with the antiparallel (parallel) magnetization. In Fig. 3(b), we show at zero-bias voltage for various directions of the magnetization. The exchange potentials in the FM lead 1 and FM lead 2 are respectively chosen as and with . By changing and , and are respectively rotated around the and axis. We choose the parameters as , and . Except for and , we obtain the finite nonlocal conductance . The sign of is determined by , where . The maximum magnitude of is obtained when both and are directed along either or . We also confirm that the nonlocal conductance is zero irrespective of and for . Therefore, we can find the distinctive contrast in and , which is the evidence for the CMESs, for the various alignments of the magnetization.
Majorana wave functions.—The anomalously long-range nonlocal transport in the present junction implies that an incident electron from one lead is transmitted through the superconducting segment as the CMESs, and is scattered into another leads. To confirm this statement directly, we here analyze the quasi-particle wave functions contributing to the CAR process from the FM lead 1 to 2. Specifically, we calculate the wave function at zero energy, where labels the incoming channel having the largest contribution to (i.e., have the largest value of among all ). Details for the calculation are given in Supplemental Material. To discuss the most comprehensible case, we assume the half-metallic ferromagnets with the anitiprallel magnetization along -axis, where with . With this specific choice of magnetization, consists of only spin- electron component and spin- hole component , while . Moreover, the local Andreev reflection in the FM lead 1 and EC from the FM lead 1 to 2 are absent. In Fig. 4(a) and (b), we respectively show the spatial profile of electron component amplitude and that of hole component amplitude . We choose the parameters as , , and . In the lead 1, we find the finite which corresponds to the incident electron wave and normal-reflected electron wave. In the lead 2, we find the finite corresponding to the crossed Andreev reflected hole wave. There are no propagating hole (electron) waves in the lead 1 ( lead 2) due to the absence of the local Andreev reflection (EC) process. For the superconducting segment, most importantly, we find that the wave function localized at the edge of the superconductor mediates the wave functions in the two different FM leads. To examine this in more detail, in Fig. 4(c), we show the ratio of at the edge of the superconductor (). We find that holds between the two FM leads (). Therefore, the wave function bridging the two FM leads indeed corresponds to a Majorana edge excitation described by the superposition of an electron wave and a hole wave with equal amplitude.
Discussion—Here we highlight the most significant advantage of our proposal that we can identify the CMESs thorough the obvious difference in and , where one of them is finite and the other is zero. In real experiments, several perturbations such as the tilt of -vector, and spin-orbit coupling potentials in the vicinity of junction interface, may induce additional spin-flip scattering processes and may decrease the amplitude of the finite nonlocal conductance. Even so, our proposal is still valid in the presence of such perturbations because we only need the contrast between finite and zero nonlocal conductance for detecting the CMESs. Actually, we have confirmed that the significant contrast between and is preserved for the broad range of magnetization alignments as shown in Fig. 3(b).
In summary, we have discussed the nonlocal conductance in the junction consisting of a chiral -wave SC and two FM leads. The CMESs cause the the anomalously long-range and chirality-sensitive nonlocal transport and generate the drastic contrast in and . On the basis of these numerical results, we have proposed a smoking-gun experiment to detect the CMESs in chiral -wave superconductors and have discussed the advantage of our proposal. We hope that our work will motivate further experiments on nonlocal transport measurements for recently fabricated ferromagnetic-SrRuO3/Sr2RuO4 hybrid systems maeno_16 .
Acknowledgements.
We are grateful to J. Annett and D. Schlom for fruitful discussions. YA is supported by “Topological Materials Science” (Nos. JP15H05852 and JP15K21717) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan, JSPS Core-to-Core Program(A. Advanced Research Networks), Japanese-Russian JSPS-RFBR project (Nos. 2717G8334b and 17-52-50080), and the Ministry of Education and Science of the Russian Federation (Grant No. 14Y.26.31.0007).
I Recursive Green Function Technique
I.1 Reflections Coefficients
In this section we explain the lattice Green function technique used for calculating the reflection coefficients in Eq. (4) in the main text. For later convenience, we introduce several integer numbers as (see also Fig. 5)
[TABLE]
and indicate a lattice site by a vector . The chiral -wave superconductor (SC) occupies and and the ferromagnetic (FM) lead (-) occupies and . We rewrite the Bogoliubov-de Gennes (BdG) Hamiltonian in the main text into the appropriate form for the numerical calculation as
[TABLE]
where
[TABLE]
and
[TABLE]
We represents , , , and matrices by , , and , respectively. The zero matrix is represented by . The matrix () occupies from the -th row to the -th row of matrix (), while other components of () are zero.
With this representation, the BdG equation describing the present junction is given by
[TABLE]
with . For the FM lead with , we can separate the BdG equation into the two Schrödinger equations as
[TABLE]
where Eqs. (83) and (84) respectively describe the electron and hole states in the FM lead . For the SC segment with , we obtain
[TABLE]
By following the method shown in Ref. [ando_91, ], we will derive an useful equation for solving the scattering problem. As a preliminary step, we calculate the linearly independent solutions for Eqs. (83), (84) and (86). We first focus on the Eqs. (83) and (84) describing the FM lead . In the presence of translational symmetry in the -direction, the solution of Eqs. (83) and (84) respectively satisfy
[TABLE]
By substituting Eq. (87) into Eq. (83), and substituting Eq. (88) into Eq. (84), we obtain
[TABLE]
By using Eqs. (87) and (89), and using Eqs. (88) and (90), we obtain the eigen equations
[TABLE]
By solving Eq. (97) numerically, we obtain the eigenstates, where of them are right-going (left-going) eigenstates [] belonging with eigenvalue [] for -. The right-going (left-going) propagating channel is characterized with and (), where represents the group velocity of the electron state given by
[TABLE]
The right-going (left-going) evanescent channel is characterized with (). By using the eigenstates and eigenvelues of Eq. (97), we define two matrices
[TABLE]
As in the similar manner, we define two matrices by using the eigenstates and eigenvelues of Eq. (104)
[TABLE]
where [] represents the right-going (left-going) eigenstates corresponding to the eigenvalue [] for -. The right-going (left-going) propagating channel satisfies and () with representing the group velocity of the hole state given by
[TABLE]
while the right-going (left-going) evanescent channel satisfies (). Any left-going and right-going electron (hole) states can be described by the linear combination of []. We here denote the left- and right-going electron states at with
[TABLE]
and denote the left- and right-going hole states at with
[TABLE]
where and are expanding coefficients. For , we can describe the left- and right-going states by
[TABLE]
Next, we calculate the the linearly independent solutions for Eq. (86) describing the SC segment. As similar to the analysis for the FM leads, we introduce the eigen equation
[TABLE]
By using the eigenstates and eigenvalues of of Eq. (125), we construct the matrices
[TABLE]
where [] represents the right-going (left-going) eigenstates belonging with eigenvelue [] for -. The right-going (left-going) states are characterized by () or () with , where represents the group velocity as
[TABLE]
We here represent the left- and right-going wave functions at as
[TABLE]
where is the expanding coefficient. For , the wave function is given by
[TABLE]
Let us now consider the scattering problem that electron states incident from the FM leads to the SC. The electron wave function in the FM lead at is represented as . For , we obtain
[TABLE]
By substituting Eq. (133) into Eq. (83), we deform the Schrödinger equation for the electron states at as
[TABLE]
For , the wave function for the hole states consists of only left-going waves as . Thus the hole wave function at is deformed as
[TABLE]
By substituting Eq. (136) into Eq. (84), we deform the Schrödinger equation for the hole states at as
[TABLE]
For the SC segment with , the wave function consists of only the right-going waves as . Thus the wave function at is written as
[TABLE]
By substituting Eq. (138) into Eq. (86), the BdG equation at is deformed as
[TABLE]
By using Eqs. (134) , (137) and (139), we obtain a motion of equation for
[TABLE]
where is the zero vector with lines. On the basis of this equation, we define the Green function obeying
[TABLE]
To calculate the reflection and transmission coefficients, we only need and . These matrix components can be easily calculated by using the recursive Green function technique as fisher_81
[TABLE]
where
[TABLE]
We here calculate the reflection coefficients. By using Eqs. (111) and (113), the wave function at is written by
[TABLE]
From Eq. (178), we also obtain
[TABLE]
By combining Eqs. (213) and (230), we obtain
[TABLE]
By using the matrices
[TABLE]
we obtain
[TABLE]
where () occupies from -th to -th line and from -th to -th row of (). From Eq. (259), we find
[TABLE]
The normal (Andreev) reflection coefficients for the incident electron in the lead belonging with the channel and the reflected electron (hole) in the lead belonging with the channel is given by
[TABLE]
We next calculate the transmission coefficients. From Eq. (131), the wave function at is rewritten as
[TABLE]
From Eq. (178), we also find
[TABLE]
By using Eqs. (280) and (286), we obtain
[TABLE]
where represents zero matrix. The matrix occupies from the -th row to -th row of the matrix . From Eq. (289), we obtain the relation
[TABLE]
The transmission coefficient for the incident electron in the FM lead belonging with the channel and the out-going Bogoliubov quasiparticle in the SC belonging with the channel is given by
[TABLE]
These reflection and transmission coefficients satisfy the conservation low of
[TABLE]
To calculate the nonlocal conductance in the main text, we use the elastic co-tunneling and crossed Andreev reflection coefficients respectively given by and with .
I.2 Wave functions
In this section, we explain the calculation method for the spacial profile of wave functions shown in Fig. 4 in the main text. From Eqs. (115), (117) and (213), the wave function in the FM segment is described as
[TABLE]
By using Eq. (259), we obtain
[TABLE]
From Eqs. (131) and (280), the wave function for the SC segment is written by
[TABLE]
By using Eq (289), we find
[TABLE]
Let us focus on the wave function belonging with the incoming channel in the FM lead . To calculate , we set the expanding coefficient as
[TABLE]
with . By substituting Eqs. (337) into Eq. (330) and (334), we finally obtain
[TABLE]
where
[TABLE]
In the main text, we show at zero energy belonging with the incoming channel having the largest value of among all .
II Transmission and Reflection Probabilities
at a Chiral -wave Superconductor/Normal-metal Interface
In the Blonder-Tinkham-Klapwijk formalism, we assume that the charge currents carried by the chiral Majorana edge states moving towards the inside of the superconducting segment () are absorbed into the ideal electrode attached to the superconductor. In this section, to support this assumption, we calculate the reflection and transmission probabilities in a chiral -wave superconductor/normal-metal (SN) junction as shown in Fig. 6(a). We consider the present junction on the two-dimensional lattice model with the lattice constant . A lattice site is indicated by a vector , where () is the vector in the () direction with . The chiral -wave superconductor (normal-metal) occupies () and . In the direction, we apply the hard-wall boundary condition. The present junction is described by the Bogoliubov-de Gennes Hamiltonian
[TABLE]
where () represents the creation (annihilation) operator of an electron at the site , denotes the nearest-neighbor hopping integral, and is the chemical potential. The amplitude and chirality of the pair potential in the superconducting segment are represented by and ( or ), respectively. In what follows, we fix several parameters as , , , and . With , the chiral Majorana edge states of the chiral -wave superconductor incident from the lower edge () of the superconducting segment to the SN interface as shown in Fig. 6(a). By using the lattice Green functions technique, we calculate the reflection and transmission probabilities defined as
[TABLE]
The reflection coefficient at energy is given by , where the index labels the incident channel from the superconducting segment and the index labels the outgoing channel in the superconductor. The transmission coefficient from the quasi-particle states in the superconductor to the electron (hole) states in the normal segment is represented by , where the index labels the outgoing channel in the normal-metal segment. With the energy below the superconducting gap (i.e., ), there is only one incident channel corresponding to the chiral Majorana edge state at the lower edge. Therefore, the reflection probability with corresponds to the scattering processes that the incident chiral Majorana edge states are reflected to the superconducting segment as the backward chiral Majorana edge states at the upper edge as shown Fig. 6(a). In Fig. 2(b), we show , and as a function of energy of incident states from the superconducting segment. With , we find the important relations of and , which imply that the incident chiral Majorana edge states are always scattered into the attached normal-metal. Although the normal-metal does not describe the ideal electrode straightforwardly, this result strongly support the assumption of the BTK formalism that the chiral Majorana edge states moving toward are always absorbed into the ideal electrode and never circle around the edge of superconductor.
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