$\mathcal{P}\mathcal{T}$-Symmetric Coherent Perfect Absorber with Graphene
Mustafa Sarisaman, Murat Tas

TL;DR
This paper explores how integrating graphene sheets into $ ext{PT}$-symmetric coherent perfect absorbers enhances absorption, reduces gain requirements, and offers potential for improved CPA laser design through analytic modeling.
Contribution
It provides exact analytic expressions for $ ext{PT}$-symmetric CPAs with graphene, highlighting how graphene parameters optimize absorption and reduce gain thresholds for CPA lasers.
Findings
Graphene enhances absorption in CPA systems.
Optimal parameters reduce the gain needed for CPA.
Graphene's resonance effects improve CPA performance.
Abstract
We investigate -symmetric coherent perfect absorbers (CPAs) in the TE mode solution of a linear homogeneous optical system surrounded by graphene sheets. It is revealed that presence of graphene sheets contributes the enhancement of absorption in a coherent perfect absorber. We derive exact analytic expressions, and work through their possible impacts on lasing threshold and CPA conditions. We point out roles of each parameter governing optical system with graphene and show that optimal conditions of these parameters give rise to enhancement and possible experimental realization of a CPA laser. Presence of graphene leads the required gain amount to reduce considerably based on its chemical potential and temperature. We obtain that relation between system parameters decides the measure of CPA condition. We find out that graphene features contributing to resonance effect in…
| Spectrally Singular Waves | Time Reversed Waves | CPA Waves | ||
|---|---|---|---|---|
| Region | ||||
| Region |
| with Graphene | without Graphene | |||||||
|---|---|---|---|---|---|---|---|---|
| 1.9053 | 1.8883 | 1.7817 | ||||||
| and | and | |||||||
|---|---|---|---|---|---|---|---|---|
| 1.6713 | 1.6324 | 1.6591 | ||||||
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-Symmetric Coherent Perfect Absorber with Graphene
Mustafa Sarısaman1
Department of Physics, Istanbul University, 34134 Istanbul, Turkey
Murat Tas2
Department of Physics, Gebze Technical University, 41400 Kocaeli, Turkey
Abstract
We investigate -symmetric coherent perfect absorbers (CPAs) in the TE mode solution of a linear homogeneous optical system surrounded by graphene sheets. It is revealed that presence of graphene sheets contributes the enhancement of absorption in a coherent perfect absorber. We derive exact analytic expressions, and work through their possible impacts on lasing threshold and CPA conditions. We point out roles of each parameter governing optical system with graphene and show that optimal conditions of these parameters give rise to enhancement and possible experimental realization of a CPA laser. Presence of graphene leads the required gain amount to reduce considerably based on its chemical potential and temperature. We obtain that relation between system parameters decides the measure of CPA condition. We find out that graphene features contributing to resonance effect in graphene sheets are rather preferable to build a better coherent perfect absorber.
Pacs numbers: 03.65.Nk, 42.25.Bs, 42.60.Da, 24.30.Gd
I Introduction
The coherent perfect absorbers (CPAs), or antilasers, antilaser1 ; antilaser2 ; antilaser2-1 ; antilaser2-2 ; antilaser2-3 ; antilaser3 ; antilaser4 ; antilaser5 are fascinating optical constructs that furnish in principle the absorption of certain incident coherent waves by the optical potential, but yet they basically act as a theoretical design today. Since they operate as time reversal case of regular lasers, they are inherently expressed by the time reversal symmetry of spectral singularities naimark ; naimark-1 ; naimark-2 ; naimark-3 ; naimark-4 , which are used as a tool to render the best way of examining lasing threshold condition silfvast in a laser. Thus, complex conjugate of the optical potential that supports a spectral singularity engenders a CPA-laser action jpa-2012 . Accordingly, it is intriguing to consider a -symmetric potential that endorses both a spectral singularity and CPA concurrently. This is rather interesting because it functions as a laser emitting coherent waves unless it is subject to incident coherent waves with appropriate amplitude and phase in which case it acts as an absorber lastpaper . Although recent experimental realizations of CPAs have been carried out CPAexp ; CPAexp-1 ; CPAexp-2 , basically they still stand as theoretical structures awaiting experimental advancement, see also antilaser5 for a recent review of CPAs.
Since its debut, symmetry has found considerable interest in optics and related fields due to its smoothness to realize experimental investigations and immediate applications. A generic -symmetric Hamiltonian in optics is vested with a potential whose peculiar property is bender ; bender-1 ; bender-2 ; bender-3 ; bender-4 ; PT4 ; PT5 , which corresponds to switching gain and loss components in conserved potential. Complex optical -symmetric potentials are realized by the formal equivalence between quantum mechanical Schrödinger equation and optical wave equation derived from Maxwell equations. By exploiting optical modulation of the refractive index in the complex dielectric permittivity plane and engineering both optical absorption and amplification, -symmetric optical systems can lead to a series of intriguing optical phenomena and devices, such as dynamic power oscillations of light propagation, CPA-lasers lastpaper ; CPA ; CPA-1 ; CPA-2 ; CPA-3 ; pra-2015d , spectral singularities naimark ; naimark-1 ; naimark-2 ; naimark-3 ; naimark-4 ; p123 ; pra-2012a ; longhi4 ; longhi3 and unidirectional invisibility bender ; bender-1 ; bender-2 ; bender-3 ; bender-4 ; PT6 ; PT7 ; pra-2017a ; prb-2018 .
Emergence of CPA-lasers is among the most notable applications of -symmetric potentials in optics. In the context of -symmetry, the condition for appearance of a spectral singularity coincides with that of its time-reversal longhi2010 . This makes -symmetric CPA-lasers as one of the primary examples in the study of -symmetric optical structures mostafazadeh2012 . This elegant finding motivates new insight towards solving the problem of constructing a CPA with appropriate amplitudes and phases of incoming waves. In view of this motivation, here we examine feasibility of realizing a CPA-laser in a homogeneous -symmetric optical slab system covered by graphene sheets. Our aim in using the graphene sheets is to enhance the adjustment of absorption in entire system graphene ; graphene-1 ; graphene-2 ; graphene-3 ; graphene-4 ; graphene-5 .
Physical properties of graphene has been profoundly unveiled and thus its numerous applications in condensed matter physics and optics have attracted interest of researchers for over a decade gr1 ; gr2 ; gr3 ; gr4 . Since its early discovery, a voluminous literature has arisen and plenty of applications have been realized especially in the fields of sensor based transport phenomena gr5 ; gr5-1 ; gr5-2 ; gr5-3 ; gr5-4 ; gr5-5 ; gr5-6 , impurity invisibility gr6 , electron optics with p-n junctions gr7 , and invisibility cloaking gr8 ; gr9 ; naserpour . The idea that graphene interact with electromagnetic waves in anomalous and exotic ways, providing new phenomena and applications, gives rise to the study of CPA phenomenon in -symmetric optical structures with graphene. Especially recent works in this field lastpaper ; graphene ; graphene-1 ; graphene-2 ; graphene-3 ; graphene-4 ; graphene-5 fashion up essential motivation for this study, which will use whole competency of the transfer matrix method in a scattering formalism which grounds its power on Maxwell equations. Furthermore, see referee1 ; referee2 ; referee3 ; referee4 for some relevant studies of graphene based light modulation and optical gain.
In a scattering problem the transfer matrix is used to encapsule all the scattering data prl-2009 . Its composition property makes it more practical and preferable than scattering matrix. Moreover, its components involve necessary information to reveal spectral singularities, CPA and invisibility of electromagnetic fields interacting with an optically active medium lastpaper ; CPA ; CPA-1 ; CPA-2 ; CPA-3 ; pra-2015d . See also transmat1 ; transmat2 ; transmat3 for the use of transfer matrix formalism belonging to the scattering of layered structures containing graphene.
Our analysis fulfils oblique incidence lastpaper ; jones1 , considering that desired phenomena may be angle dependent. Hence, we conduct a comprehensive study of spectral singularities which yields lasing threshold condition and CPAs in the oblique TE mode of a -symmetric system with graphene to unveil the intriguing traits of transfer matrix as complementary to lastpaper . Our system is depicted in Fig. 1.
Our analysis demonstrates all possible configurations of the system leading to spectral singularity and CPA solutions. We find out complete solutions and schematically demonstrate their behaviors using various parameter choices. Among all possible parameters of the system which provide valuable information about the CPA-lasers, only optimal ones lead to achieve performing an efficient CPA. In particular, we obtain analytic expressions for the spectral singularity and CPA configurations, and examine behaviors of practically most desirable choices of parameters corresponding to TE waves. We reveal that optimal control of graphene parameters, such as gain coefficient, incidence angle, slab thickness, temperature, and chemical potential, gives rise to a desired outcome for achieving enhancement of absorption, and computing correct amplitude and phase contrasts in a CPA-laser. Thus, we provide a concrete ground that restrict the mentioned parameters of graphene in certain ranges. Optimal values of these parameters should be adjusted in a given system if one desires the experimental realization of CPA.
II TE Mode Solution of a Planar Bilayer Slab System with Graphenes
Consider a one-dimensional linear homogeneous and optically active parallel pair of slab system whose exterior planar surfaces are covered by graphene layers as depicted in Fig. 1. Suppose that entire optical system is immersed in air and regions and are respectively filled with gain and loss materials having constant complex refractive indices and . Let this system be exposed to external time harmonic electromagnetic waves with electric and magnetic fields. Maxwell equations describing interaction of the electromagnetic waves with the slab system have the form:
[TABLE]
where the index represents the regions sketched in Fig. 1, and are the electric and magnetic fields in corresponding regions. They are connected to and fields via the constitutive relations
[TABLE]
and are respectively the permeability and permittivity of the vacuum. We defined complex quantity
[TABLE]
such that the subindex correspond to vacuum at which , represent respectively the gain and loss components of the slab, and stands for coordinates in the specified -th region as depicted in Fig. 1. In Maxwell equations (1) and (2), and respectively denote the free charge and conductivity present on the graphene sheets and therefore expressed as
[TABLE]
where and are respectively the free charge and conductivity on the -th layer of graphene, with . Notice that and are associated to each other by the continuity equation
[TABLE]
for the electric current density . Conductivity of graphene sheets has been determined within the random phase approximation in conductivity-graphene ; conductivity-graphene-1 ; conductivity-graphene-2 as the sum of intraband and interband contributions, i.e. , where
[TABLE]
Here , , is electron charge, is reduced Planck’s constant, is Boltzmann constant, is temperature, is the scattering rate of charge carriers, is the chemical potential, and is the photon energy naserpour . In time harmonic forms, and fields are respectively given by and . Thus, Maxwell equations corresponding to transverse electric (TE) wave solutions yield the following form of Helmholtz equation
[TABLE]
where , is the wavenumber, is the speed of light in vacuum, and is the impedance of vacuum. We stress out that TE waves correspond to the solutions of (6) for which is parallel to the surface of the slabs. In our geometrical setup, they are aligned along the -axis. Suppose that in region , incident wave adapts a plane wave with wavevector in the - plane, specified by
[TABLE]
where and are respectively the unit vectors along the -, - and -directions, and is the incidence angle (See Fig. 1). For convenience we introduce the scaled variables
[TABLE]
Thus, the electric field corresponding to TE waves is given by
[TABLE]
where is solution of the Schrödinger equation
[TABLE]
for the potential . Here we define
[TABLE]
The fact that potential is constant in regions of interest gives rise to a solution in relevant regions
[TABLE]
where and , with , are -dependent complex coefficients, and
[TABLE]
In particular, is given by the right-hand side of (12) with generally different choices of constants and . These coefficients are related to each other via appropriate boundary conditions: tangential components of and are continuous across the surface while the normal components of have a step of unbounded surface currents across the interface of graphenes. Table 1 displays corresponding set of boundary conditions. Quantities are defined as
[TABLE]
III Transfer Matrix and Spectral Singularities
Right outgoing waves could be associated to the left ones by means of the transfer matrix. Transfer matrix is favored over the scattering matrix by virtue of its composition property, which helps being articulated the scattering properties of any optical system. For our two-layer optical system furnished by -symmetry with graphene sheets, total transfer matrix can be obtained as the product of transfer matrices of gain and loss regions. If individual transfer matrices corresponding to the gain and loss regions of the slab are denoted by and respectively, then total transfer matrix satisfies composition property , and is expressed by
[TABLE]
Spectral singularities match up to real zeros of component of , which is computed explicitly as
[TABLE]
where we identify
[TABLE]
It is apparent that -symmetry implies the following relations
[TABLE]
Thus it amounts that currents on the left and right graphene sheets flow in opposite directions by virtue of symmetry. Spectral singularities correspond to real values of the wavenumber such that . Hence, (20) gives rise to explicit form of the spectral singularity condition
[TABLE]
We note that quantities involve the effect of graphene in the spectral singularities as given by identity (14). Provided that graphene layers are removed by setting , (22) generates the spectral singularity condition given in lastpaper .
IV Spectral Singularities in -Symmetric Configurations
Spectral singularities corresponding to our optical setup in (22) describe the lasing threshold condition. This is in fact a complex expression screening behavior of system parameters. Thus, it can be explored in detail by means of relevant quantities containing significant physical consequences. In view of symmetry relations given in (21), we obtain the following relations
[TABLE]
Refractive index and are expressed in real and imaginary parts as follows
[TABLE]
Most of the materials safely satisfy the condition . In particular, this practical restriction of materials leads and to be expressed in terms of and leading order of as
[TABLE]
We next introduce the gain coefficient and its threshold value at resonance frequency
[TABLE]
where corresponds to the resonance wavelength. In the light of (23), (24), (25) and (26), the spectral singularity condition (22) yields the following set of equations in the leading order of
[TABLE]
where we define and for convenience as follows
[TABLE]
In practice, Eqs. (27) and (28) control the lasing behavior of our system in such a way that the most appropriate system parameters should be accounted for the emergence of optimal impacts. Graphene effect on the lasing occurrence is revealed by the presence of real and imaginary parts of . Thus, a comprehensive analysis of the involvement of system parameters is required to observe final outcome in the presence of graphene sheets. For this purpose we exhibit general behaviors of system parameters through the gain coefficient plots. We employ Nd:YAG crystals in -symmetric bilayer slab system with following specifications
[TABLE]
and graphene sheets with characterizations
[TABLE]
In Fig. 2, appearance of graphene sheets is distinguished in the plot of gain coefficient as a function of incidence angle . We use the parameters as given in (29) for the slab, and in (30) for the graphene component. It is obvious that graphene triggers the gain value to reduce considerably, depending upon the properties of graphene sheets. As the incidence angle approaches to , graphene effect gets trivial and amount of the gain coefficient survives at a finite value as distinct from an individual layer case alone.
Figure 3 reflects essential behavior of curves in the plane of slab thickness and gain once the graphene sheets are inserted into the system. Gain values slightly drop off especially more at smaller thicknesses of micron sizes.
It turns out that characteristics of graphene layers manifest themselves in determining the rate of gain decrement. Fig. 4 displays attitudes of temperature and chemical potential of graphene sheets. It is revealed that optimal reduction of gain amount is achieved by employing as much lower temperatures and chemical potentials as possible. In particular, chemical potentials less than about meV are favorable for the best effect. This is the case . Around the resonance of graphene where the relation holds, the required gain amount for lasing rises and then proceeds to decay to when . Lastly, we remark that temperature (also chemical potential) dependence of the refractive indices is ignored safely since it yields a negligible effect (about 0.001%) within the temperature limits of interest temp ; temp2 , which guarantees validity of our results.
V Presence of Dispersion Content
We now assume that there exist a dispersion in the refractive index , and investigate its possible impacts on the spectral singularities. For this purpose, we include wavenumber dependence of . We assume that active part of our optical system composing the gain ingredient is formed by doping a host medium of refractive index , and its refractive index satisfies the following dispersion relation
[TABLE]
Here , , , is the resonance frequency, is the damping coefficient, and is the plasmon frequency. The can be described in leading order of the imaginary part of at the resonance wavelength , by the expression pra-2011a . After inserting this relation into (31), employing the first expression of (24), and ignoring quadratic and higher order terms in , we obtain the real and imaginary parts of the refractive index as CPA ; CPA-1 ; CPA-2 ; CPA-3
[TABLE]
At resonance wavelength , the can be written as , see (26). Substituting this relation in (32) and making use of (24) and (22), we can determine and values for the spectral singularities. These are explicitly shown in the - plane in Fig. 5 for our setup with slab and graphene properties listed in (29) and (30), and for the incidence angle . Furthermore, Nd:YAG crystals which form the slab material hold the following value for given and values silfvast
[TABLE]
It appears that graphene sheets with associated parameters lead to shift down in the location of spectral singularity points. This verifies our findings explored in the previous section. Again at temperatures close to absolute zero and chemical potentials much lower values, the spectral singularity points move faster down in the - plane.
VI CPA Laser Action
Our -symmetric optical slab encrusted by graphene sheets serves as a CPA provided that time reversed system is fulfilled once the spectral singularities are prevalent. This phenomenon happens to exist only if correct phase and amplitude of incoming waves are originated. Thus, incoming waves are perfectly absorbed by the optical system that gives rise to a CPA-laser, see Fig. 6 for a pictorial demonstration of the phenomenon.
Spectral singularities displayed in the left panel of Fig. 6 describe purely outgoing waves. Time reversed case is just obtained by complex conjugation of waves outside the slab such that gain and loss parts are interchanged. To make a CPA-laser, we switch the gain and loss parts of time reversed case so that desired incoming waves can entirely be obtained as shown in the right panel of Fig. 6. For a required phenomena, waves outside the active part of the optical slab can be expressed as in Table 2 in terms of solutions of Maxwell equations in the exterior regions as given in (9) and (12).
CPA-laser operates once the incoming waves emergent by angle are absorbed perfectly so that full destructive interference occurs. This can be measured by the ratio of complex amplitude of incoming waves for and . In view of amplitudes given in Table 2, this is expressed as
[TABLE]
In fact, can be denominated in terms of by employing the spectral singularity condition. We recall that spectral singularities correspond to purely outgoing waves such that
[TABLE]
This, together with the boundary conditions in Table 1 and spectral singularity condition in (22), leads to
[TABLE]
Thus, it is easy to show that incoming waves are perfectly absorbed provided that ratio of incoming amplitudes specified by satisfies
[TABLE]
Hence, ratio of amplitudes and phase factors of the waves incoming from left- and right-hand sides are characterized by and respectively, and the latter is quantified as
[TABLE]
Consequently, the CPA-laser action can outrightly be obtained once the and of incoming waves from the left and right-hand sides are tuned in according to expressions (36) and (37) respectively. Pictorial representation of how these quantities are influenced by parameters of the optical system are clearly shown in Figs. 7, 8 and 9. Note that in these figures the parameters assume the values given in (29) and (30).
Figure 7 displays dependence of and on incidence angle . We set the gain amount to , nm, and meV. We notice that and oscillate with angle such that peaks in the presence of graphene case slightly shift with respect to without graphene case, especially for small incidence angles, and they almost coincide for large incidence angles. It is obvious that presence of graphene requires larger compared to without graphene case for small and moderate incidence angles, and this influence decreases as gets larger. This means that amplitude of wave coming from the left side should be adjusted to have a little higher value compared to the amplitude of waves coming from the right side. In a similar manner, phase difference factor for graphene shifts slightly, and could get any value for small incidence angles, and graphene induces this phase difference to rise significantly as the incidence angle increases. This amounts to that graphene mostly yields almost destructive interference. Graphene effect is not felt much for the angles close to right angles. See the last row of Fig. 7 for overall view of incidence angle dependence.
In Figs. 8 and 9, one explicitly realizes the effect of graphene for obtaining a CPA-laser. We employ the incidence angle , gain value , and wavelength nm. Figure 8 demonstrates how chemical potential variation of graphene sheets impacts on the ratio of amplitudes and phase difference corresponding to different temperatures. We observe that chemical potentials less than about meV give more and relatively small phase difference, especially at smaller temperatures. When increases till about 0.028 eV, the decreases and increases. The point eV corresponds to resonance value of graphene so that it is felt at small temperatures as noticed in the figure. When chemical potential gets values higher than eV, starts to scale up to get asymptotic value of about while reduces to get a value around . These findings are verified in Fig. 9, i.e. the effect of graphene is perceived at considerably small temperatures, and temperatures giving rise to the resonance effect particularly for small chemical potentials such that increases whereas decreases as temperature decreases from , and decreases to minimum value and increases to maximum value in temperature range . It is understood that temperature and chemical potential values close to resonance effect of graphene are favorable in order to get a well-adjusted CPA-laser.
Table 3 demonstrates some parameter values belonging to our optical system with and without graphene to realize a CPA-laser as an instructive guide for the experimental attempts. Properties of graphene sheets are specified by temperature , chemical potential of eV and meV. Table 4 explicitly presents values necessary to build a graphene based CPA-laser corresponding to graphene parameter values and eV (left board), and and eV (right board).
VII Concluding Remarks
This study benefits the idea that a CPA-laser is the time reversal construct of a regular laser which could be expressed by means of the spectral singularities. Nowadays, experimental realization of CPA-lasers is the main challenge due to difficulties in adjusting exact amplitude and phase factors of incoming waves. Current studies exploit various techniques in order to measure the quantities pointing CPA actions. In this work, we employed an optical system which respects the property of -symmetry accompanied by graphene containment. In lastpaper , necessary and sufficient conditions for implementing a CPA-laser based on the feature of -symmetry are given, and in this current study we performed a comprehensive analysis aiming to find the conditions for CPA-laser action based on graphene sheets. Hence, the results of this study guide experimental attempts for realization of -symmetric CPA phenomenon with graphene.
We made use of distinctive traits of the transfer matrix formalism and determined the spectral singularities, which give rise to lasing threshold condition reflecting the presence of graphene in a -symmetric optical system. The transfer matrix approach grounds the power of boundary conditions arising from the solutions coming directly from Maxwell equations. Table 1 reveals the presence of graphene sheets in boundary conditions in the form of complex function , see Eq. (14). We derived exact expressions for the conditions of lasing threshold in (22) and of coherent perfect absorber in (36) and (37). We employ a perturbative approach to obtain optimal conditions arising from the system parameters.
We require that graphene coatings respect overall symmetry which leads to formation of currents flowing in opposite directions. We emphasize that symmetry enables the emergence of lasing and CPA conditions due to its power to control the system parameters as distinct from non--symmetric structures. In particular, we find out that graphene insertion into a -symmetric optical system leads lower gain values depending upon the graphene features, especially temperature and chemical potential. At this point, resonance occurrence of graphene plays a significant role which happens to exist at meV at absolute zero temperature, and slightly shifts up with increasing temperature. In general, below the resonance point, the lower temperature and chemical potential of graphene sheets are, the less gain amount is. The results of spectral singularities and in turn lasing threshold conditions facilitate the path towards obtaining a CPA because of coincidence of both phenomena at the same points.
We observe that efficiency of a CPA-laser could be improved once the parameters of the optical system together with graphene features are well-adjusted. We consider -symmetry to achieve computational and thus experimental accessibility of the optical system by tuning appropriate parameters of the system. Accordingly, we place graphene sheets at the ends of -symmetric slab system just to realize that optimal conditions for the CPA-laser action can be obtained by computing appropriate intensity and phase contrasts. In order to get a lower intensity and higher phase contrast that yield an almost destructive interference, one should opt for lower temperatures and chemical potentials for the graphene sheets at which the resonance effect occurs. Also, small incidence angles provide relatively lower intensities in the presence of graphene, which lead to larger phase difference as desired. This is the main reason to use graphene sheets in the optical system.
In view of our findings, one can shape a reliable CPA equipment provided that parameters specifying the graphene and bilayer slab system are well-adjusted. In Tables 3 and 4 we provide explicit values of parameters in order to build a concrete CPA. Our primary purpose in placing graphene is to improve absorption of waves and utilize arrangement of parameters. We explored that this is achieved at values especially around the resonance effect of graphene. Furthermore, it is observed that graphene causes the necessary gain amount to lessen. In this respect, we infer that presence of graphene gives valuable information about enhancement of absorption in a CPA, which helps building a better CPA. This suggests even a more effective material could be used instead of graphene to make a unity ratio of amplitudes and smooth phase contrast to make a perfect destructive interference. In this direction recently some prominent candidates have been intensely studied like Weyl semimetals may be in the limelight to build a better CPA.
As a final note, it would be interesting to describe the role of surface plasmon polaritons (SPPs) in our system. But, no surface modes should exist at the interface between the slab and graphene since we focused on TE polarization solutions. SPPs exist only for TM polarization. Maier .
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