# Isospin-phonon coupling and Fano-interference in spin-orbit Mott insulator Sr2IrO4

## TL;DR

This study investigates how lattice vibrations interact with electronic and magnetic properties in Sr2IrO4, revealing isospin-phonon coupling and Fano interference effects that are sensitive to magnetic ordering.

## Contribution

It provides new insights into the coupling between phonons, electronic excitations, and magnetic order in the spin-orbit Mott insulator Sr2IrO4 using Raman scattering.

## Key findings

- Anomalous phonon behavior below TN ~240 K.
- Fano lineshape in A1g mode at 560 cm-1 indicating electronic excitations.
- Strong isospin-phonon coupling related to Ir-O-Ir bond modulation.

## Abstract

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The strongest effect is detected for the A1g mode at 272 cm-1 associated with the modulation of the Ir-O-Ir bond angle. Additionally, the A1g mode at 560 cm-1 shows a Fano asymmetric lineshape sensitive to TN, supporting the existence of low-energy (~70 meV) electronic excitations that are renormalized by the magnetic order. These results reveal new aspects of the interaction between the crystal lattice and electronic degrees of freedom in this spin-orbit entangled Mott insulator.