Fractional Angular Momenta, Gouy and Berry phases in Relativistic Bateman-Hillion-Gaussian Beams of Electrons
Robert J. Ducharme, Irismar Gon\c{c}alves da Paz, Armen G. Hayrapetyan

TL;DR
This paper presents a relativistic Gaussian electron beam solution to the Dirac equation, revealing fractional angular momenta linked to Berry and Gouy phases, with implications for spin-orbit coupling and beam focusing.
Contribution
It introduces a new relativistic Gaussian beam solution accounting for beam waist position, highlighting fractional angular momenta and their relation to Berry and Gouy phases beyond the paraxial limit.
Findings
Fractional angular momenta are related to Berry phase.
Gouy phase is connected to Berry phase and affects beam focusing.
Differences between Laguerre-Gaussian and Bessel beams in phase properties.
Abstract
A new Bateman-Hillion solution to the Dirac equation for a relativistic Gaussian electron beam taking explicit account of the -position of the beam waist is presented. This solution has a pure Gaussian form in the paraxial limit but beyond it contains higher order Laguerre-Gaussian components attributable to the tighter focusing. One implication of the mixed mode nature of strongly diffracting beams is that the expectation values for spin and orbital angular momenta are fractional and are interrelated to each other by \textit{intrinsic spin-orbit coupling}. Our results for these properties align with earlier work on Bessel beams [Bliokh \textit{et al.} Phys. Rev. Lett. \textbf{107}, 174802 (2011)] and show that fractional angular momenta can be expressed by means of a Berry phase. The most significant difference arises, though, due to the fact that Laguerre-Gaussian beams naturally…
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Fractional Angular Momenta, Gouy and Berry phases in Relativistic Bateman-Hillion-Gaussian Beams of Electrons
Robert Ducharme1
Irismar G. da Paz2
Armen G. Hayrapetyan3,4,5
1 2112 Oakmeadow Pl., Bedford, TX 76021, USA
2 Departamento de Física, Universidade Federal do Piauí, Campus Ministro Petrônio Portela, CEP 64049-550, Teresina, PI, Brazil
3 d-fine GmbH, Bavariafilmplatz 8, 82031 Grünwald, Germany
4 Mathematical Institute, University of Oxford, Radcliffe Observatory Quarter, Woodstock Rd, Oxford OX2 6GG, UK
5 Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Str. 38, 01187 Dresden, Germany
Abstract
A new Bateman-Hillion solution to the Dirac equation for a relativistic Gaussian electron beam taking explicit account of the -position of the beam waist is presented. This solution has a pure Gaussian form in the paraxial limit but beyond it contains higher order Laguerre-Gaussian components attributable to the tighter focusing. One implication of the mixed mode nature of strongly diffracting beams is that the expectation values for spin and orbital angular momenta are fractional and are interrelated to each other by intrinsic spin-orbit coupling. Our results for these properties align with earlier work on Bessel beams [Bliokh et al. Phys. Rev. Lett. 107, 174802 (2011)] and show that fractional angular momenta can be expressed by means of a Berry phase. The most significant difference arises, though, due to the fact that Laguerre-Gaussian beams naturally contain Gouy phase, while Bessel beams do not. We show that Gouy phase is also related to Berry phase and that Gouy phase fronts that are flat in the paraxial limit become curved beyond it.
pacs:
41.85.-p, 03.65.Pm, 03.65.Vf,42.50.Tx
Introduction.— In the past decade, there has been considerable progress towards solving the Dirac equation (DE) for the purpose of unveiling detailed properties of electron vortex beams carrying both spin and orbital angular momenta. The earliest of this work has modelled Bessel beams as a linear superposition of Dirac or Dirac-Volkov Bliokh:11 ; Hayrapetyan-Karlovets plane waves in contrast to non-relativistic Laguerre-Gaussian (LG) Bliokh:07 and Bessel beams Schattschneider:11 acting as solutions to paraxial and non-paraxial wave equations, respectively. More recently, the attention has been focused on investigating symmetry properties of relativistic electrons to better understand the nature of their vortex formation Bliokh:17 ; Karlovets:18 and to construct other types of wave packets Karlovets:18 ; BB (see also the debate in Refs. BB ; SMB ; BB-comment ).
A 3-vector position in space is not form invariant under Lorentz transformations. For fully relativistic calculations it is therefore necessary to replace points using point events (4-positions) so that a beam front with velocity u that reaches the waist at time T will have time for any other point at a distance before or after the waist. The use of point events as energy-momentum waypoint markers has precedent in the derivation of Lienard-Wiechert potentials SR and constraint mechanics AK ; CA . Beam solutions that incorporate a 4-position beam waist have been shown to reduce to traditional beam models RD1 ; RD2 ; RD3 in the non-relativistic limit. Beam solutions that zero out the beam waist as the origin of the beam coordinate system thus carry a hidden non-relativistic 3-vector.
In a typical electron microscope assembly, a Gaussian beam passes from an electron gun to a magnetic lens that focuses it to a small waist diameter. Assuming a modest current of energetic electrons ( 100keV), the average separation between them will be large enough so that electron repulsion can be ignored. Under these conditions, the expected diameter of the beam waist will be about a hundred times the wavelength of the electrons unless corrective measures are taken to reduce the strong spherical and chromatic aberration, which is a normal feature of magnetic lenses RE . Such transmission electron microscopes are by far the only tool to produce electron vortex beams EVB-exp , which are nowadays widely used in various physical setups review-EVB . This includes vortices in external fields EVB-in-external-fields , scattering EVB-with-scattering , atomic processes EVB-with-radiation and indicates a further possible application for electron beams to trap (sub)nanoparticles in a close analogy with optical trapping via light vortices manipulation-via-twist .
Over the course of last two-three decades, advances in optical instrumentation have made it possible to produce light vortex beams, which typically carry an integer number of orbital angular momentum (OAM) quanta review-twisted-light ; twisted-light-other . This led to an elucidation of the nature of fractional OAM (fOAM) including its clear understanding in terms of Berry phase FOAM ; FOAM-exp .
Our intention here is to build on existing work both on optical and electron vortices to calculate fractional – spin and orbital – angular momenta for a tightly focused relativistic Gaussian beam of electrons, which contains higher order LG modes. Taking proper account of the 4-position of the beam waist, we evaluate the total energy-momentum of relativistic electrons and derive a fundamental property called the Gouy phase gouy1 ; gouy2 , accumulated along the propagation direction as a result of the transverse localization of the beam feng2001-yang2006 . We demonstrate the interplay of the Gouy phase and the fractional angular momenta, quantified by an intrinsic spin-orbit interaction (SOI) term, with the Berry geometric phase. In view of this, we parameterize the total shift of the Gouy phase in a relativistic Gaussian beam, from far field to far field, in terms of the Berry phase. We shall also calculate beyond the paraxial limit to show that Gouy phase fronts that have generally thought to be planar are actually curved.
Exact Bateman-Hillion-Gaussian beams from Dirac equation.— In order to achieve our goal, we develop a theory that incorporates Lorentz invariance of relativistic Gaussian solutions of wave equations known as Bateman-Hillion (BH) solutions (BA-PH, ; BS-APK, ) that also take proper account of the beam waist position. We use the BH ansatz to solve the Klein-Gordon equation (KGE) then convert it to a solution of the full DE. Our solutions build on existing approaches for relativistic LG beams Karlovets:18 ; BB . It must be recognized, however, that our inclusion of the beam waist 4-position matters since it brings a resolution to a well known problem of BH Gaussian beams that electrons move in both directions BB additional to certain other benefits that include Lorentz invariance and correspondence to accepted beam models in the non-relativistic and paraxial limits.
Consider a beam of electrons each having a mass of , a -position and a -momentum , where and is the speed of light in vacuum. It follows the particle has an energy and 3-momentum at world time and world position . Let us also assume that each electron passes through a beam waist with a -position , where is the world position of the beam waist at world time . Note that we introduce two different time coordinates since the equality is not form preserving under Lorentz transformations.
The dynamics of each of the electrons in the beam is then given by the DE expressed as PAMD
[TABLE]
Here, is the canonical -momentum operator, are the Dirac matrices, is the reduced Planck’s constant, while represents a bi-spinor wave function of each individual electron, where “” stand for spin-up and -down states, respectively. Equation (1) also has two negative-energy bi-spinor solutions that we will not consider since they describe anti-particles. The DE (1) can be simplified using the substitution
[TABLE]
with , being two-component spinors, a scalar function, the Pauli matrices (), and where the inner product and the superscript T means “transposed”. Combining Eqs. (1) and (4) leads to the KGE for
[TABLE]
The clear understanding here is that the bi-spinor solution satisfies the DE provided that the scalar function acts as a solution of the KGE, a procedure that is also applied in Ref. BB for constructing relativistic wave packets with non-zero OAM.
The solution to the KGE (5) for the Gaussian beam has been developed in two recent papers RD1 ; RD2 . For our purposes, we start from the BH based ansatz
[TABLE]
where is a constant number, is the -position of the electron relative to the beam waist, is the wave -vector and is a scalar function incorporating non-trivial vortex and both space- and time-dependent phase structures of the electron beam.
Following Ref RD2 , we insert the BH ansatz (6) into the KGE (5) and solve the resulting equation for by utilizing the ‘radial’ and ‘azimuthal’ coordinates. This leads to the LG solution
[TABLE]
with and . Furthermore, represent the generalized Laguerre polynomials in terms of the radial, , and the azimuthal indices, ,
[TABLE]
is the Gouy phase and . The solution (7) also contains the complex parameter
[TABLE]
whose modulus, , characterizes the beam radius, such that represents the beam radius at the waist. Note that the Gouy phase (8) depends on both the space and time variables in sharp contrast to only a time-dependent Gouy phase of Ref. Karlovets:18 . Our setup considers a beam confined in the transverse -plane and propagating in the longitudinal direction, chosen to be the -axis, meaning that the beam spreads as a function of and time . This confinement in two dimensions can be experimentally designed by spherical lenses complementing the one-dimensional case realized by cylindrical lenses. The difference of expressions in round parentheses ( in Eq. (8) and of Ref. Karlovets:18 ) is a consequence of an altered scenario, when the beam is confined in three dimensions Karlovets:18 , a situation which is yet to be experimentally generated.
Equations (4), (6) and (7) constitute an exact BH solution to the DE for LG modes of the electron beam. We shall, however, focus our attention only on the Gaussian wave packets leaving a treatment of more general LG modes for future work as relevant physical conclusions can be drawn already from relativistic Bateman-Hillion-Gaussian (BHG) beams, i.e., when . Inserting, therefore, into Eq. (4) leads to
[TABLE]
where will be referred to as the effective wave vector of the electron beam,
[TABLE]
. We have omitted the arguments for brevity. Equation (10) is the exact solution to the DE for the lowest order (Gaussian) bi-spinor mode of electron beam. In the paraxial and semi-relativistic limit (, ), we recover Barnett’s solution SMB .
The constant in Eq.(6) can be determined from the Dirac current using the normalization condition, footnote1 , which implies and gives the expected velocity of the beam front where is distance traveled. We now eliminate the elapsed time in Eq. (8) using the previous expression to give
[TABLE]
for where represents the Rayleigh range. To recover the standard LG beam formulae we shall instead set consistent with the paraxial approximation , inserting this into Eqs. (8) and (9) yields the traditional paraxial beam formula
[TABLE]
The beam radius determines an important relation
[TABLE]
between the angular divergence of the beam, , the longitudinal component of the wave vector and the beam radius at the waist. Figure 1 shows a comparison of curved non-paraxial to planar paraxial Gouy phase fronts calculated using Eqs. (11) and (12) respectively.
In order to estimate the magnitude of terms in the solution (10), we evaluate the averaged probability density:
[TABLE]
where we use to confirm . The cross terms vanish here since the products of the bi-spinors are identically zero. It now follows that
[TABLE]
owing to current imperfections in magnetic lenses that limit to values of about or greater. For our further purposes, it is therefore reasonable to drop the negligible term in Eq. (10) giving to be
[TABLE]
and holding to a very high degree of accuracy. Equation (16) completes the solution of the DE for the relativistic BHG beam of electrons and enables evaluation of linear and angular momenta in the beam.
Momentum and energy of the beam.— Some of relativistic beam solutions, such as Bessel Bliokh:11 and Volkov-Bessel modes Hayrapetyan-Karlovets , although reasonable in other respects, actually carry an infinite beam energy. BHG solutions, similar to LG modes, do not share this ‘problem’. In particular, the expectation values for the -momentum in a beam are determined to be . Inserting this result into the dispersion relation we obtain the averaged total energy of a single Dirac particle in a Gaussian beam
[TABLE]
where and denote the square values of radial and axial momentum respectively. Equation (17) has been obtained elsewhere for a Klein-Gordon particle in a Gaussian beam, see Ref. RD2 , which also connects the stored kinetic energy in the beam to the Bohm potential PRH1 .
Fractional angular momenta and non-trivial phase structure of the beam.— Expected values for angular momenta of an electron parallel to the beam axis can be calculated if the explicit forms of the spin angular momentum (SAM), , and OAM operators, , are employed. Direct evaluation of corresponding integrals leads to
[TABLE]
where , while
[TABLE]
represents the intrinsic SOI term. There is a little need for us to dwell on these expressions since they look like a special case () of more general relations but derived from relativistic Bessel-beam solutions to the DE Bliokh:11 (c.f., footnote2 ).
Nonetheless, there are two subtle differences in the SOI terms for Bessel and BHG beams. (i) The Bessel-type solutions naturally contain non-paraxiality as a key feature, which is quantified by means of a parameter called opening angle similarly appearing in the sine function Bliokh:11 . In our case of Eq. (19), we have the divergence angle instead, that carries more information about the beam radius (at the waist) via Eq. (14). (ii) It is true that in the non-relativistic regime () SOI terms vanish for both types of beams. Due to the transverse localization of Gaussian modes, moreover, the first term of the SOI parameter depends explicitly on the beam radius at the waist by virtue of Eq. (17). Combining these yields an explicit connection between the SOI term and the beamwidth, which can be simplified to
[TABLE]
for existing experimental setups, i.e., when for pm. As seen, the SOI term vanishes for large beam radii independent of the longitudinal momentum , or else, for very small divergence angles (c.f., Eqs. 14 and 19).
Another implication of expected angular momenta is that the focusing of relativistic Gaussian modes with bi-spinor structure will cause a fraction of angular momentum, , to convert from the expected SAM to OAM and vice versa (see the left panel of Fig. 2 for ). At the same time, the total angular momentum (TAM) of the beam, with , is conserved along the propagation direction as depicted by the straight green dash-dotted line. As the divergence angle increases from [math] to , the stake starts disappearing from the SAM and reappearing as fOAM resulting in the fractional spin-to-orbit conversion. For , the fractional SAM (fSAM) and fOAM parts contribute in the conserved TAM with the shares and , respectively. Depending on the electron kinetic energy, the spin-to-orbit conversion occurs either fully (for ), so that the shares by angular momenta are equal, or partially (e.g., for ) due to the gradual decrease of the SOI term.
Variations in the beamwidth over the infinite length of the beam axis represent an adiabatic cycle in the sense that the beam divergence beyond the waist undoes the convergence occurring ahead of the waist. Such an adiabatic cycle, being inherently characterized by the divergence angle, contributes in the SOI due to the tight focusing of the BHG beam by means of non-zero higher mode bi-spinors proportional to and (see Eq. (10)). Over the course of such a cyclic adiabatic process, the beam accumulates also a Berry (geometric) phase from these higher mode bi-spinors. The Berry phase can be evaluated exactly in the same manner as for relativistic Bessel beams by making use of the so-called Foldy-Wouthuysen momentum representation Bliokh:11 . Following Bliokh et al. we may therefore write the Berry phase as gained due to the non-trivial fOAM as .
For a tightly focused BHG beam, the expected Gouy phase
[TABLE]
is larger than would be the case for a pure Gaussian beam owing to the SOI. The total Gouy phase shift from far field to far field in the beam is therefore given by
[TABLE]
showing that the Gouy phase as well as the fOAM increase in direct proportion to the Berry phase, while the fSAM decreases. The right panel of Fig. 1 illustrates the growth of both phases dependent on the divergence angle and the electron kinetic energy. The Berry phase rises as the SOI term increases and retains its maximum value along with the Gouy phase at . The presence of non-vanishing expectation values for the transverse components of the linear momentum implies that the relevant phase angle to consider in this case is not the azimuth phase associated with the fOAM but the Gouy phase feng2001-yang2006 . It thus appears from our results that the Berry phase for this cycle is not the baseline Gouy phase for the paraxial beam but the fractional increase in the Gouy phase above the baseline value that can be explicitly attributed to the adiabatic cycle. Our evidence for this assertion being the direct proportionality between the Gouy phase and the fOAM value is shown in Eq. (21).
Discussion.— Dirac published his quantum theory of the electron in 1928 PAMD . Some ninety years later, it is now being extensively applied to understand the effects of transverse localization on electron beams. A significant progress has been made in this direction by deriving (either exact or approximated) solutions to the DE for Bessel Bliokh:11 ; Hayrapetyan-Karlovets and LG beams Karlovets:18 ; BB ; SMB . In our paper, we derive a new and exact BHG solution to the DE, which possesses the full relativistic nature of the beam propagation as it takes into account the -position of the beam waist footnote3 . This has enabled us to calculate the energy-momentum, fractional angular momenta and the Gouy phase in the beam and demonstrate the presence of the intrinsic SOI leading to the fractional spin-to-orbit conversion. Remarkably, both the fOAM and the Gouy phase are directly proportional to the Berry phase. This both corroborates the earlier finding of Bliokh et al. Bliokh:11 for fOAM and takes it a step further with our inclusion of Gouy phase into the evolving understanding of the role geometric phase has to play in relativistic electron beams, predicted earlier for a non-relativistic Gaussian beam SM and demonstrated recently for optical rays Malhotra:18 . Additionally, we have found that Gouy phase fronts that have traditionally thought to be planar are in fact curved. This curvature is most apparent in the far fields of strongly diffracting beams.
Acknowledgements.
I. G. da Paz thanks Grant No. 307942/2019-8 from CNPq.
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