Radiative-capture cross sections for the $^{139}$La($n,\gamma$) reactionusing thermal neutrons and structural properties of $^{140}$La

TL;DR

This study measured thermal neutron-capture cross sections for $^{139}$La, providing new data on the reaction and nuclear structure of $^{140}$La, including improved decay scheme details and a neutron-separation energy.

Contribution

The paper presents new experimental cross section data for $^{139}$La(n,γ), along with refined nuclear structure information for $^{140}$La, enhancing existing knowledge of this reaction and decay scheme.

Findings

Total cross section for $^{139}$La(n,γ) is 9.36(74) b.

Neutron-separation energy $S_n$ is 5161.005(21) keV.

Proposes improvements to the $^{140}$La decay scheme.

Abstract

A set of prompt partial $\gamma$-ray production cross sections from thermal neutron-capture were measured for the $^{139}$La($n,\gamma$) reaction using a guided beam of subthermal (thermal and cold) neutrons incident upon a $^{\rm nat}$La$_{2}$O$_{3}$ target at the Prompt Gamma Activation Analysis facility of the Budapest Research Reactor. Absolute $^{140}$La cross sections were determined relative to the well-known comparator $^{35}$Cl($n,\gamma$) cross sections from the irradiation of a stoichiometric $^{\rm nat}$LaCl$_{3}$ sample. The total cross section for radiative thermal neutron-capture on $^{139}$La from the sum of experimentally measured cross sections observed to directly feed the $^{140}$La ground state was determined to be $\sigma_{0}^{\rm expt} = 8.58(50)$ b. To assess completeness of the decay scheme and as a consistency check, the measured cross sections for transitions feeding the ground state from levels below a critical energy of $E_{c} = 285$ keV were combined with a modeled contribution accounting for ground-state feeding from the quasicontinuum to arrive at a total cross section of $\sigma_{0} = 9.36(74)$ b. In addition, a neutron-separation energy of $S_{n} = 5161.005(21)$ keV was determined from a least-squares fit of the measured primary $\gamma$-ray energies to the low-lying levels of the $^{140}$La decay scheme. Furthermore, several nuclear structure improvements are proposed for the decay scheme. The measured cross-section and separation-energy results are comparable to earlier measurements of these quantities.