Precise measurement of $\alpha_K$ and $\alpha_T$ for the 39.8-keV $E$3 transition in $^{103}$Rh: Test of internal-conversion theory

TL;DR

This study precisely measures internal conversion coefficients for a specific nuclear transition in $^{103}$Rh, testing and refining theoretical models by including atomic vacancy effects and revealing a small M4 component.

Contribution

The paper provides the first precise experimental measurements of $ ext{K}$-shell and total internal conversion coefficients for the 39.8-keV $E$3 transition in $^{103}$Rh, challenging existing theory and suggesting a small M4 mixing.

Findings

Measured $ ext{K}$-shell and total internal conversion coefficients: 141.1(23) and 1428(13).

Results disagree with vacancy-ignoring Dirac-Fock calculations.

Indicates a small M4 component with mixing ratio $ ext{δ} = 0.023(5)$.

Abstract

Neutron-activated sources of $^{103}$Ru and $^{103}$Pd both share the isomeric first-excited state in $^{103}$Rh as a daughter product. From independent measurements of both decays, we have measured the $K$-shell and total internal conversion coefficients, $\alpha_K$ and $\alpha_T$, for the 39.8-keV $E$3 transition, which de-excites that state in $^{103}$Rh, to be 141.1(23) and 1428(13), respectively. When compared with Dirac-Fock calculations, our new results disagree with the version of the theory that ignores the $K$-shell atomic vacancy, which is consistent with our conclusion drawn from a series of measurements on high multipolarity transitions in nuclei with higher $Z$. Calculations that include the atomic vacancy indicate that the transition actually has a small $M$4 component with mixing ratio $\delta$ = 0.023(5).