Anisotropic hybridization in a new Kondo lattice compound CeCoInGa$_3$

TL;DR

This study investigates the anisotropic hybridization and heavy-fermion behavior in the new Kondo lattice compound CeCoInGa$_3$, combining experimental measurements and theoretical calculations to reveal coherence effects and hybridization anisotropy.

Contribution

It provides a comprehensive experimental and theoretical analysis of CeCoInGa$_3$, highlighting anisotropic hybridization and coherence phenomena in a new Kondo lattice compound.

Findings

Onset of coherence at about 50 K

Large Sommerfeld coefficient indicating heavy-fermion behavior

Anisotropy in hybridization gap and magnetic susceptibility

Abstract

We report a detailed and comparative study of the single crystal CeCoInGa$_3$ in both experiment and theory. Resistivity measurements reveal the typical behavior of Kondo lattice with the onset temperature of coherence, $T^*\approx 50\,$K. The magnetic specific heat can be well fitted using a spin-fluctuation model at low temperatures, yielding a large Sommerfeld coefficient, $\gamma\approx172\,$mJ/mol K$^2$ at 6 K, suggesting that this is a heavy-fermion compound with a pronounced coherence effect. The magnetic susceptibility exhibits a broad field-independent peak at $T_{\chi}$ and shows an obvious anisotropy within the $bc$ plane, reflecting the anisotropy of the coherence effect at high temperatures. These are compared with strongly correlated calculations combining first-principles band structure calculations and dynamical mean-field theory. Our results confirm the onset of coherence at about 50 K and reveal a similar anisotropy in the hybridization gap, pointing to a close connection between the hybridization strength of the low-temperature Fermi-liquid state and the high-temperature coherence effect.