Two-color phase-of-the-phase spectroscopy with circularly polarized laser pulses

TL;DR

This paper extends phase-of-the-phase spectroscopy to circularly polarized laser pulses, revealing a sharp phase-flip in photoelectron spectra sensitive to laser parameters and ionization potential, supported by numerical and analytical analysis.

Contribution

It introduces the application of phase-of-the-phase spectroscopy to circular polarization and derives an analytical expression for the phase-flip momentum.

Findings

Photoelectron spectra exhibit three-fold symmetry with circular polarization.

A sharp phase-flip occurs at a specific radial momentum.

The phase-flip is sensitive to laser parameters and ionization potential.

Abstract

Phase-of-the-phase spectroscopy using two-color colinearly polarized laser pulses has been introduced and experimentally applied to strong-field tunneling ionization in S. Skruszewicz et al., Phys. Rev. Lett. 115, 043001 (2015) and recently to multiphoton ionization in M. A. Almajid et al., J. Phys. B: At. Mol. Opt. Phys. 50, 194001 (2017). The idea behind phase-of-the-phase spectroscopy is to study in a systematic way the change in the photoelectron yield as a function of the relative phase between the strong fundamental field component (of carrier frequency $\omega$) and a weak, second color component (e.g., $2\omega$). The observable of interest is the photoelectron-momentum-dependent phase of the change in the electron yield with respect to the relative phase, hence the name "phase of the phase." In the present paper, phase-of-the-phase spectroscopy is extended to circularly polarized light. With a small, counter-rotating $2\omega$-component, photoelectron spectra have a three-fold symmetry in the polarization plane. The same is true for the corresponding phase-of-the-phase spectra. However, a peculiar, very sharp phase-flip by $\pi$ occurs at a certain radial momentum of the photoelectron that is sensitive to both laser parameters and the ionization potential. Results from the numerical solution of the time-dependent Schr\"odinger equation are compared to those from the strong-field approximation. An analytical expression for the momentum at which the phase-of-the-phase flipping occurs is presented.