Phase-controlled Fourier-transform spectroscopy

TL;DR

This paper introduces a phase-controlled Fourier-transform spectroscopy method that significantly increases spectral acquisition rates to over 10,000 spectra per second, enabling rapid, high-resolution, broadband measurements with incoherent light sources.

Contribution

The authors develop a dynamic phase-control technique that allows high-speed Fourier-transform spectroscopy at Nyquist limits, expanding its application to rapid and continuous measurements.

Findings

Achieved spectral acquisition rates over 10,000 spectra per second.

Maintained high spectral resolution and broad bandwidth.

Demonstrated passive operation with incoherent light sources.

Abstract

Fourier-transform spectroscopy (FTS) has been widely used as a standard analytical technique over the past half-century. FTS is a simple and robust autocorrelation-based technique that is compatible with both temporally coherent and incoherent light sources, which functions as an active or passive spectrometer. However, this technique has been mostly used for static measurements due to the low scan rate imposed by technological restrictions. This has impeded its application to continuous rapid measurements, which would be of significant interest for a variety of fields, especially when monitoring of non-repeating/transient complex dynamics is desirable. Here, we demonstrate highly efficient FTS operating at a high spectral acquisition rate with a simple delay line based on a dynamic phase-control technique. The independent adjustability of phase and group delays allows us to achieve the Nyquist-limited spectral acquisition rate over 10,000 spectra per second, while maintaining a large spectral bandwidth and high resolution. In addition, we demonstrate the ability of this passive spectrometer working with an incoherent light source.