Non-hermitian Hamiltonian description for quantum plasmonics: from dissipative dressed atom picture to Fano states

TL;DR

This paper develops effective non-Hermitian Hamiltonians to model the dynamics of a dipolar emitter coupled to a metal nanoparticle, accounting for losses and radiative leakages, and introduces Fano states and Lindblad equations for a comprehensive description.

Contribution

It introduces a unified framework using non-Hermitian Hamiltonians and Fano states to describe dissipative quantum plasmonic systems with varying particle sizes.

Findings

Effective non-Hermitian Hamiltonian models for small particles dominated by absorption.

Fano Hamiltonian including plasmon leakages for large particles.

Lindblad equations and collective dissipators describing system dynamics.

Abstract

We derive effective Hamiltonians for a single dipolar emitter coupled to a metal nanoparticle (MNP) with particular attention devoted to the role of losses. For small particles sizes, absorption dominates and a non hermitian effective Hamiltonian describes the dynamics of the hybrid emitter-MNP nanosource. We discuss the coupled system dynamics in the weak and strong coupling regimes offering a simple understanding of the energy exchange, including radiative and non radiative processes. We define the plasmon Purcell factors for each mode. For large particle sizes, radiative leakages can significantly perturbate the coupling process. We propose an effective Fano Hamiltonian including plasmon leakages and discuss the link with the quasi-normal mode description. We also propose Lindblad equations for each situation and introduce a collective dissipator for describing the Fano behaviour.