Electroluminescence TPCs at the thermal diffusion limit

TL;DR

This study investigates how adding small amounts of molecular gases to xenon can reduce electron diffusion in electroluminescent TPCs, balancing diffusion reduction with energy resolution to optimize detector performance for neutrinoless double-beta decay searches.

Contribution

It provides experimental and simulation data on the effects of CO₂, CH₄, and CF₄ additives on EL yield and energy resolution, identifying CH₄ as the most promising additive for large xenon TPCs.

Findings

Electron diffusion reduced from 10 to 2.5 mm/√m with additives.

CF₄ yields highest EL but poor energy resolution.

CH₄ offers best energy resolution (~0.4%) at low concentrations.

Abstract

The NEXT experiment aims at searching for the hypothetical neutrinoless double-beta decay from the ${}^{136}$Xe isotope using a high-purity xenon TPC. Efficient discrimination of the events through pattern recognition of the topology of primary ionisation tracks is a major requirement for the experiment. However, it is limited by the diffusion of electrons. It is known that the addition of a small fraction of a molecular gas to xenon reduces electron diffusion. On the other hand, the electroluminescence (EL) yield drops and the achievable energy resolution may be compromised. We have studied the effect of adding several molecular gases to xenon (CO${}_{2}$, CH${}_{4}$ and CF${}_{4}$) on the EL yield and energy resolution obtained in a small prototype of driftless gas proportional scintillation counter. We have compared our results on the scintillation characteristics (EL yield and energy resolution) with a microscopic simulation, obtaining the diffusion coefficients in those conditions as well. Accordingly, electron diffusion may be reduced from about 10 mm/$\sqrt{\mathrm{m}}$ for pure xenon down to 2.5 mm/$\sqrt{\mathrm{m}}$ using additive concentrations of about 0.05%, 0.2% and 0.02% for CO${}_{2}$, CH${}_{4}$ and CF${}_{4}$, respectively. Our results show that CF${}_{4}$ admixtures present the highest EL yield in those conditions, but very poor energy resolution as a result of huge fluctuations observed in the EL formation. CH${}_{4}$ presents the best energy resolution despite the EL yield being the lowest. The results obtained with xenon admixtures are extrapolated to the operational conditions of the NEXT-100 TPC. CO${}_{2}$ and CH${}_{4}$ show potential as molecular additives in a large xenon TPC, CH${}_{4}$ showing the best performance and stability to be used in the NEXT-100 TPC, with an extrapolated energy resolution of 0.4% at 2.45 MeV for concentrations below 0.4%.