Tunneling spin valves based on Fe$_3$GeTe$_2$/hBN/Fe$_3$GeTe$_2$ van der Waals heterostructures

TL;DR

This study demonstrates the creation of tunneling spin valves using vdW heterostructures with Fe3GeTe2 and hBN, revealing high magnetoresistance and surface-bulk magnetic property correlation.

Contribution

It reports the first realization and detailed investigation of vdW heterostructure-based tunneling spin valves with Fe3GeTe2 and hBN, highlighting their magnetic and transport properties.

Findings

Magnetoresistance of 160% at low temperature.

Spin polarization of Fe3GeTe2 is 0.66.

Surface magnetic properties reflect bulk behavior.

Abstract

Thin van der Waals (vdW) layered magnetic materials disclose the possibility to realize vdW heterostructures with new functionalities. Here we report on the realization and investigation of tunneling spin valves based on van der Waals heterostructures consisting of an atomically thin hBN layer acting as tunnel barrier and two exfoliated Fe3GeTe2 crystals acting as ferromagnetic electrodes. Low-temperature anomalous Hall effect measurements show that thin Fe3GeTe2 crystals are metallic ferromagnets with an easy axis perpendicular to the layers, and a very sharp magnetization switching at magnetic field values that depend slightly on their geometry. In Fe3GeTe2/hBN/Fe3GeTe2 heterostructures, we observe a textbook behavior of the tunneling resistance, which is minimum (maximum) when the magnetization in the two electrodes is parallel (antiparallel) to each other. The magnetoresistance is 160% at low temperature, from which we determine the spin polarization of Fe3GeTe2 to be 0.66, corresponding to 83% and 17% of majority and minority carriers, respectively. The measurements also show that, with increasing temperature, the evolution of the spin polarization extracted from the tunneling magnetoresistance is proportional to the temperature dependence of the magnetization extracted from the analysis of the anomalous Hall conductivity. This suggests that the magnetic properties of the surface are representative of those of the bulk, as it may be expected for vdW materials.