Comparison of magnetic and structural properties of permalloy Ni80Fe20 grown by dc and high power impulse magnetron sputtering

TL;DR

This study compares the microstructure and magnetic properties of Ni80Fe20 thin films grown by HiPIMS and dcMS, revealing how deposition methods and parameters influence film density, roughness, and magnetic anisotropy.

Contribution

It provides a direct comparison of magnetic and structural properties of Ni80Fe20 films grown by two sputtering techniques under various conditions, highlighting the impact of adatom energy.

Findings

High adatom energy in HiPIMS yields dense films with low magnetic anisotropy.

Void-rich films from dcMS at high pressure show higher coercivity.

Surface roughness increases with pressure but minimally affects magnetic properties.

Abstract

We study the microstructure and magnetic properties of Ni80Fe20 thin films grown by high power impulse magnetron sputtering (HiPIMS), and compare with films grown by dc magnetron sputtering (dcMS). The films were grown under a tilt angle of 35{\deg} to identical thickness of 37 nm using both techniques, at different pressure (0.13-0.73 Pa) and substrate temperature (room temperature and 100 {\deg}C). All of our films display effective in-plane uniaxial anisotropy with square easy axis and linear hard axis magnetization traces. X-ray diffraction reveals that there is very little change in grain size within the pressure and temperature ranges explored. However, variations in film density, obtained by X-ray reflectivity measurements, with pressure have a significant effect on magnetic properties such as anisotropy field (Hk) and coercivity (Hc). Depositions where adatom energy is high produce dense films, while low adatom energy results in void-rich films with higher Hk and Hc. The latter applies to our dcMS deposited films at room temperature and high pressure. However, the HiPIMS deposition method gives higher adatom energy than the dcMS and results in dense films with low Hk and Hc. The surface roughness is found to increase with increased pressure, in all cases, however it showed negligible contribution to the increase in Hk and Hc.