Expansion Dynamics After Laser-Induced Cavitation in Liquid Tin Microdroplets
Dmitry Kurilovich, Tiago de Faria Pinto, Francesco Torretti, Ruben, Schupp, Joris Scheers, Aneta S. Stodolna, Hanneke Gelderblom, Kjeld S. E., Eikema, Stefan Witte, Wim Ubachs, Ronnie Hoekstra, Oscar O. Versolato

TL;DR
This study investigates how 15-ps laser pulses cause cavitation and expansion in liquid tin microdroplets, combining experiments and modeling to understand fragmentation and mass distribution relevant for EUV nanolithography.
Contribution
It introduces a combined experimental and fluid dynamic modeling approach to analyze cavitation-driven expansion and fragmentation of liquid tin microdroplets.
Findings
Good agreement between model and experiments across droplet sizes and laser energies.
Initial expansion velocity follows a power-law dependence on experimental parameters.
Late-time mass distributions are governed by a single parameter.
Abstract
The cavitation-driven expansion dynamics of liquid tin microdroplets is investigated, set in motion by the ablative impact of a 15-ps laser pulse. We combine high-resolution stroboscopic shadowgraphy with an intuitive fluid dynamic model that includes the onset of fragmentation, and find good agreement between model and experimental data for two different droplet sizes over a wide range of laser pulse energies. The dependence of the initial expansion velocity on these experimental parameters is heuristically captured in a single power law. Further, the obtained late-time mass distributions are shown to be governed by a single parameter. These studies are performed under conditions relevant for plasma light sources for extreme-ultraviolet nanolithography.
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