Magnetic Force Microscopy Imaging Using Geometrically Constrained Nano-Domain Walls

TL;DR

This paper introduces a novel magnetic force microscopy probe with a nanostructure that can switch between states, providing enhanced magnetic contrast and additional information about sample stray fields with minimal interference.

Contribution

The study presents a new geometrically constrained nano-domain wall probe for MFM, enabling switchable magnetic states and improved imaging contrast compared to standard probes.

Findings

Probes exhibit four magnetic states controlled by external magnetic fields.

Pinned domain walls produce strong stray fields for high contrast imaging.

Curl states provide complementary information about in-plane magnetization.

Abstract

Domain wall probes (DW-probes) were custom-made by modifying standard commercial magnetic force microscopy (MFM) probes using focused ion beam lithography. Excess of magnetic coating from the probes was milled out, leaving a V-shaped nanostructure on one face of the probe apex. Owing to the nanostructure's shape anisotropy, such probe has four possible magnetic states depending on the direction of the magnetization along each arm of the V-shape. Two states of opposite polarity are characterised by the presence of a geometrically constrained DW, pinned at the corner of the V-shape nanostructure. In the other two states, the magnetization curls around the corner with opposite chirality. Electron holography studies, supported by numerical simulations, demonstrate that a strong stray field emanates from the pinned DW, whilst a much weaker stray field is generated by the curling configurations. Using in situ MFM, we show that the magnetization states of the DW-probe can be easily controlled by applying an external magnetic field, thereby demonstrating that this type of probe can be used as a switchable tool with a low or high stray field intensity. We demonstrate that DW-probes enable acquiring magnetic images with a negligible interference with the sample magnetization, similar to that of commercial low moment probes, but with a higher magnetic contrast. In addition, the DW-probe in the curl state provides complementary information about the in-plane component of the sample's magnetization, which is not achievable by standard methods and provides additional information about the stray fields, e.g. as when imaging DWs.