Ultrafast light switching of ferromagnetism in EuSe

TL;DR

This study demonstrates ultrafast optical control of ferromagnetism in EuSe, where resonant light induces a giant spin polarization within picoseconds, enabling rapid and complete magnetization of the material.

Contribution

It reveals a novel photoinduced magnetization mechanism in EuSe driven by resonant light and large magnetic susceptibility enhancement due to competing magnetic interactions.

Findings

Light resonant with EuSe bandgap induces ferromagnetic alignment in picoseconds.

Generation of a supergiant spin polaron with nearly 6,000 Bohr magnetons.

Complete sample magnetization achieved by increasing light intensity.

Abstract

We demonstrate that light resonant with the bandgap forces the antiferromagnetic semiconducor EuSe to enter ferromagnetic alignment in the picosecond time scale. A photon generates an electron-hole pair, whose electron forms a supergiant spin polaron of magnetic moment of nearly 6,000 Bohr magnetons. By increasing the light intensity, the whole of the sample can be fully magnetized. The key to the novel large photoinduced magnetization mechanism is the huge enhancement of the magnetic susceptibility when both antiferromagnetic and ferromagnetic interactions are present in the material, and are of nearly equal magnitude, as is the case in EuSe.