Study and mitigation of spurious electron emission from cathodic wires in noble liquid time projection chambers

TL;DR

This study systematically investigates spurious electron emission from cathodic wires in noble liquid detectors, revealing surface quality as a key factor and demonstrating that surface treatments can significantly reduce emission rates, aiding future detector performance.

Contribution

It provides the first detailed analysis of emission patterns and surface effects, showing that surface treatment like nitric acid cleaning reduces electron emission in noble liquid detectors.

Findings

Emission observed at fields as low as 10 kV/cm

Surface treatments can reduce emission rates by at least an order of magnitude

No intrinsic threshold found at the metal-LXe interface

Abstract

Noble liquid radiation detectors have long been afflicted by spurious electron emission from their cathodic electrodes. This phenomenon must be understood and mitigated in the next generation of liquid xenon (LXe) experiments searching for WIMP dark matter or neutrinoless double beta decay, and in the large liquid argon (LAr) detectors for the long-baseline neutrino programmes. We present a systematic study of this spurious emission involving a series of slow voltage-ramping tests on fine metal wires immersed in a two-phase xenon time projection chamber with single electron sensitivity. Emission currents as low as $10^{-18}$ A can thus be detected by electron counting, a vast improvement over previous dedicated measurements. Emission episodes were recorded at surface fields as low as $\sim$10 kV/cm in some wires and observed to have complex emission patterns, with average rates of 10-200 counts per second (c/s) and outbreaks as high as $\sim$10$^6$ c/s. A fainter, less variable type of emission was also present in all untreated samples. There is evidence of a partial conditioning effect, with subsequent tests yielding on average fewer emitters occurring at different fields for the same wire. We find no evidence for an intrinsic threshold particular to the metal-LXe interface which might have limited previous experiments up to fields of at least 160 kV/cm. The general phenomenology is not consistent with enhanced field emission from microscopic filaments, but it appears instead to be related to the quality of the wire surface in terms of corrosion and the nature of its oxide layer. This study concludes that some surface treatments, in particular nitric acid cleaning for stainless steel wires, can bringing about at least order-of-magnitude improvements in overall electron emission rates, and this should help the next generation of detectors achieve the required electrostatic performance.