Optical models for thin layers

TL;DR

This paper systematically compares 3D, 2D, and linearized 2D optical models for thin layers, demonstrating the conditions under which each model is valid and their applications in analyzing optical responses.

Contribution

It introduces a comprehensive analysis of optical models for thin layers, including derivations of applicability conditions and generalizations to anisotropic and layered structures.

Findings

2D model agrees well with 3D model over broad spectral ranges

Linearized 2D model effective for weak optical responses

Analytical expressions for model applicability and accuracy

Abstract

We provide a systematic study of the optical models for thin layers: the 3D model, the 2D model and the linearized 2D model. We show that the 2D model is applicable for layers with small optical thicknesses. Excellent agreement of the 2D model with the 3D model is demonstrated over broad spectral ranges from DC to near UV for representative van der Waals atomic layers and thin metal layers. The linearized 2D model requires additionally weak optical response. Analytical expressions for the applicability and accuracies of the optical models are derived. We discuss the advantages and limitations of the models for the purpose of measuring their optical response functions. Further, we generalize the theory to take into account in-plane anisotropy, heterostructures, and stratified substrates. Implications of the 2D model for the correct analysis of transmission attenuation and implementations of half- and total-absorption layers are discussed.