Microscopic description of fission in odd-mass uranium and plutonium nuclei with the Gogny energy density functional

TL;DR

This study uses the Gogny energy density functional within the HFB-EFA framework to analyze fission properties of odd-mass uranium and plutonium isotopes, providing detailed predictions of fission characteristics and lifetimes.

Contribution

It presents a systematic microscopic analysis of fission in odd-mass U and Pu nuclei using the Gogny D1M functional, including effects of pairing and quantum corrections, with insights into uncertainties.

Findings

Odd-mass U and Pu nuclei have larger fission half-lives than even-even neighbors.

Small changes in pairing strengths significantly affect predicted fission lifetimes.

Fission fragment properties and alpha-decay lifetimes are also characterized.

Abstract

The parametrization D1M of the Gogny energy density functional is used to study fission in the odd-mass Uranium and Plutonium isotopes with A=233,\ldots,249 within the framework of the Hartree-Fock-Bogoliubov (HFB) Equal Filling Approximation (EFA). Ground state quantum numbers and deformations, pairing energies, one-neutron separation energies, barrier heights and fission isomer excitation energies are given. Fission paths, collective masses and zero point rotational and vibrational quantum corrections are used to compute the systematic of the spontaneous fission half-lives t$_{SF}$, the masses and charges of the fission fragments as well as their intrinsic shapes. Although there exits a strong variance of the predicted fission rates with respect to the details involved in their computation, it is shown that both the specialization energy and the pairing quenching effects, taken into account fully variationally within the HFB-EFA blocking scheme, lead to larger spontaneous fission half-lives in odd-mass U and Pu nuclei as compared with the corresponding even-even neighbors. It is shown that modifications of a few percent in the strengths of the neutron and proton pairing fields can have a significant impact on the collective masses leading to uncertainties of several orders of magnitude in the predicted t$_{SF}$ values. Alpha-decay lifetimes have also been computed using a parametrization of the Viola-Seaborg formula.