Coupled spin and electron-phonon dynamics at the relativistic Tl/Si(111) surface

TL;DR

This study reveals how the unique spin textures at the Tl/Si(111) surface influence electron-phonon interactions, leading to exceptionally strong coupling near the Γ point due to spin polarization effects.

Contribution

The paper demonstrates, through first-principles calculations, that spin patterns significantly modulate electron-phonon coupling strength at the Tl/Si(111) surface, highlighting the role of spin-orbit interaction.

Findings

Electron-phonon coupling is weakened near K and K' valleys due to spin polarization.

Near the Γ point, electron-phonon coupling is exceptionally strong with λ ~ 1.4.

Spinor overlaps explain the modulation of electron-phonon interactions.

Abstract

We investigate the role played by the electron spin and the spin-orbit interaction on the exceptional electronphonon coupling at the Tl/Si(111) surface. Our first-principles calculations demonstrate that the particular spin pattern of this system dominates the whole low-energy electron-phonon physics, which is remarkably explained by forbidden spin-spin scattering channels. In particular, we show that the strength of the electron-phonon coupling appears drastically weakened for surface states close to the K and K' valleys, which is unambiguously attributed to the spin polarization through the associated modulation due to the spinor overlaps. However, close to the {\Gamma} point, the particular spin pattern in this area is less effective in damping the electron-phonon matrix elements, and the result is an exceptional strength of electron-phonon coupling parameter {\lambda} ~ 1.4. These results are rationalized by a simple model for the electron-phonon matrix elements including the spinor terms.