Effects of high energy proton irradiation on the superconducting properties of Fe(Se,Te) thin films

TL;DR

This study investigates how 3.5 MeV proton irradiation affects Fe(Se,Te) thin films, revealing minimal impact on critical temperature and fields but notable enhancement of critical current when irradiation occurs far from the film-substrate interface.

Contribution

It provides a systematic analysis of proton irradiation effects on Fe(Se,Te) thin films, highlighting substrate proximity as a key factor influencing superconducting properties.

Findings

Irradiation has a minor effect on Tc and Hc2.

Critical current density Jc can increase by up to 50% when irradiation is far from the film.

Proximity of irradiation to the film-substrate interface decreases Tc and Jc, increases resistivity and lattice strain.

Abstract

In this paper we explore the effects of 3.5 MeV proton irradiation on Fe(Se,Te) thin films grown on CaF2. In particular, we carry out a systematic experimental investigation with different irradiation fluences up to 7.30x10^16 cm^-2 and different proton implantation depths, in order to clarify whether and to what extent the critical current is enhanced or suppressed, what are the effects of irradiation on the critical temperature, the resistivity and the critical magnetic fields, and finally what is the role played by the substrate in this context. We find that the effect of irradiation on superconducting properties is generally small as compared to the case of other iron-based superconductors. Such effect is more evident on the critical current density Jc, while it is minor on the transition temperature Tc, on the normal state resistivity and on the upper critical field Hc2 up to the highest fluences explored in this work. In addition, our analysis shows that when protons implant in the substrate far from the superconducting film, the critical current can be enhanced up to 50% of the pristine value at 7 T and 12 K, while there is no appreciable effect on critical temperature and critical fields together with a slight decrease in resistivity. On the contrary, when the implantation layer is closer to the film-substrate interface, both critical current and temperature show a decrease accompanied by an enhancement of the resistivity and the lattice strain. This result evidences that possible modifications induced by irradiation in the substrate may affect the superconducting properties of the film via lattice strain. The robustness of the Fe(Se,Te) system to irradiation induced damage makes it a promising compound for the fabrication of magnets in high-energy accelerators.